Lower Stratospheric Water Vapor Research Articles

Is there a solar signal in lower stratospheric water vapour?

Abstract. A merged time series of stratospheric water vapour built from the Halogen Occultation Instrument (HALOE) and the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) data between 60° S and 60° N and 15 to 30 km and covering the years 1992 to 2012 was analysed by multivariate linear regression, including an 11-year solar cycle proxy. Lower stratospheric water vapour was found to reveal a phase-shifted anti-correlation with the solar cycle, with lowest water vapour after solar maximum. The phase shift is composed of an inherent constant time lag of about 2 years and a second component following the stratospheric age of air. The amplitudes of the water vapour response are largest close to the tropical tropopause (up to 0.35 ppmv) and decrease with altitude and latitude. Including the solar cycle proxy in the regression results in linear trends of water vapour being negative over the full altitude/latitude range, while without the solar proxy, positive water vapour trends in the lower stratosphere were found. We conclude from these results that a solar signal seems to be generated at the tropical tropopause which is most likely imprinted on the stratospheric water vapour abundances and transported to higher altitudes and latitudes via the Brewer–Dobson circulation. Hence it is concluded that the tropical tropopause temperature at the final dehydration point of air may also be governed to some degree by the solar cycle. The negative water vapour trends obtained when considering the solar cycle impact on water vapour abundances can possibly solve the "water vapour conundrum" of increasing stratospheric water vapour abundances despite constant or even decreasing tropopause temperatures.

Balloon-borne observations of lower stratospheric water vapor at Syowa Station, Antarctica in 2013

Balloon-borne observations of lower stratospheric water vapor were conducted with the Cryogenic Frostpoint Hygrometer (CFH) in July, September, and November 2013 at Syowa Station (69.0oS, 39.6oE) in the Antarctic. High-precision and high vertical resolution data of water vapor concentration up to an altitude of about 28 km were obtained successfully except for a contamination in the observation of July 2013. A comparison between the CFH and coincident satellite (i.e., Aura/MLS) observations showed a good agreement within their uncertainty. A position of Syowa Station relative to the stratospheric polar vortex edge varied depending on both the observation date and altitude. Temperature and pressure histories of the observed air parcels were examined by 10-day backward trajectories. These analyses clearly demonstrated that most air parcels observed in the lower stratosphere above Syowa Station experienced final dehydration inside the polar vortex. On the other hand, a clear signature of rehydration or incomplete dehydration was also observed around a 25 hPa pressure level in the observation of July 2013.

Processes Controlling Tropical Tropopause Temperature and Stratospheric Water Vapor in Climate Models

Abstract A warm bias in tropical tropopause temperature is found in the Met Office Unified Model (MetUM), in common with most models from phase 5 of CMIP (CMIP5). Key dynamical, microphysical, and radiative processes influencing the tropical tropopause temperature and lower-stratospheric water vapor concentrations in climate models are investigated using the MetUM. A series of sensitivity experiments are run to separate the effects of vertical advection, ice optical and microphysical properties, convection, cirrus clouds, and atmospheric composition on simulated tropopause temperature and lower-stratospheric water vapor concentrations in the tropics. The numerical accuracy of the vertical advection, determined in the MetUM by the choice of interpolation and conservation schemes used, is found to be particularly important. Microphysical and radiative processes are found to influence stratospheric water vapor both through modifying the tropical tropopause temperature and through modifying upper-tropospheric water vapor concentrations, allowing more water vapor to be advected into the stratosphere. The representation of any of the processes discussed can act to significantly reduce biases in tropical tropopause temperature and stratospheric water vapor in a physical way, thereby improving climate simulations.

Impact of stratospheric major warmings and the quasi‐biennial oscillation on the variability of stratospheric water vapor

AbstractBased on simulations with the Chemical Lagrangian Model of the Stratosphere for the 1979–2013 period, driven by the European Centre for Medium‐Range Weather Forecasts ERA‐Interim reanalysis, we analyze the impact of the quasi‐biennial oscillation (QBO) and of Major Stratospheric Warmings (MWs) on the amount of water vapor entering the stratosphere during boreal winter. The amplitude of H2O variation related to the QBO amounts to 0.5 ppmv. The additional effect of MWs reaches its maximum about 2–4 weeks after the central date of the MW and strongly depends on the QBO phase. Whereas during the easterly QBO phase there is a pronounced drying of about 0.3 ppmv about 3 weeks after the MW, the impact of the MW during the westerly QBO phase is smaller (about 0.2 ppmv) and more diffusely spread over time. We suggest that the MW‐associated enhanced dehydration combined with a higher frequency of MWs after the year 2000 may have contributed to the lower stratospheric water vapor after 2000.

Water vapor observations up to the lower stratosphere through the Raman lidar during the Maïdo Lidar Calibration Campaign

Abstract. A new lidar system devoted to tropospheric and lower stratospheric water vapor measurements has been installed at the Maïdo altitude station facility of Réunion island, in the southern subtropics. To evaluate the performances and the capabilities of the new system with a particular focus on UTLS (Upper Troposphere Lower Stratosphere) measurements, the Maïdo Lidar Calibration Campaign (MALICCA) was performed in April 2013. Varying the characteristics of the transmitter and the receiver components, different system configuration scenarios were tested and possible parasite signals (fluorescent contamination, rejection) were investigated. A hybrid calibration methodology has been set up and validated to insure optimal lidar calibration stability with time. In particular, the receiver transmittance is monitored through the calibration lamp method that, at the moment, can detect transmittance variations greater than 10–15%. Calibration coefficients are then calculated through the hourly values of IWV (Integrated Water Vapor) provided by the co-located GPS. The comparison between the constants derived by GPS and Vaisala RS92 radiosondes launched at Maïdo during MALICCA, points out an acceptable agreement in terms of accuracy of the mean calibration value (with a difference of approximately 2–3%), but a significant difference in terms of variability (14% vs. 7–9%, for GPS and RS92 calibration procedures, respectively). We obtained a relatively good agreement between the lidar measurements and 15 co-located and simultaneous RS92 radiosondes. A relative difference below 10% is measured in the low and middle troposphere (2–10 km). The upper troposphere (up to 15 km) is characterized by a larger spread (approximately 20%), because of the increasing distance between the two sensors. To measure water vapor in the UTLS region, nighttime and monthly water vapor profiles are presented and compared. The good agreement between the lidar monthly profile and the mean WVMR profile measured by satellite MLS (Microwave Limb Sounder) has been used as a quality control procedure of the lidar product, attesting the absence of significant wet biases and validating the calibration procedure. Due to its performance and location, the MAIDO H2O lidar will become a reference instrument in the southern subtropics, insuring the long-term survey of the vertical distribution of water vapor. Furthermore, this system allows the investigation of several scientific themes, such as stratosphere–troposphere exchange, tropospheric dynamics in the subtropics, and links between cirrus clouds and water vapor.

Upper-troposphere and lower-stratosphere water vapor retrievals from the 1400 and 1900 nm water vapor bands

Abstract. Measuring water vapor in the upper troposphere and lower stratosphere is difficult due to the low mixing ratios found there, typically only a few parts per million. Here we examine near-infrared spectra acquired with the Solar Spectral Flux Radiometer (SSFR) during the first science phase of the NASA Airborne Tropical TRopopause EXperiment (ATTREX). From the 1400 and 1900 nm absorption bands we infer water vapor amounts in the tropical tropopause layer and adjacent regions between altitudes of 14 and 18 km. We compare these measurements to solar transmittance spectra produced with the MODerate resolution atmospheric TRANsmission (MODTRAN) radiative transfer model, using in situ water vapor, temperature, and pressure profiles acquired concurrently with the SSFR spectra. Measured and modeled transmittance values agree within 0.002, with some larger differences in the 1900 nm band (up to 0.004). Integrated water vapor amounts along the absorption path lengths of 3 to 6 km varied from 1.26 × 10−4 to 4.59 × 10−4 g cm−2. A 0.002 difference in absorptance at 1367 nm results in a 3.35 × 10−5 g cm−2 change of integrated water vapor amounts; 0.004 absorptance change at 1870 nm results in 5.50 × 10−5 g cm−2 of water vapor. These are 27% (1367 nm) and 44% (1870 nm) differences at the lowest measured value of water vapor (1.26 × 10−4 g cm−2) and 7% (1367 nm) and 12% (1870 nm) differences at the highest measured value of water vapor (4.59 × 10−4 g cm−2). A potential method for extending this type of measurement from aircraft flight altitude to the top of the atmosphere is discussed.

The Climate Impact of Past Changes in Halocarbons and CO2 in the Tropical UTLS Region

Abstract A chemistry–climate model coupled to an ocean model is used to compare the climate impact of past (1960–2010) changes in concentrations of halocarbons with those of CO2 in the tropical upper troposphere and lower stratosphere (UTLS). The halocarbon contribution to both upper troposphere warming and the associated increase in lower stratospheric upwelling is about 40% as large as that due to CO2. Trends in cold-point temperature and lower stratosphere water vapor are positive for both halocarbons and CO2, and are of about the same magnitude. Trends in lower stratosphere ozone are negative, due to the increased upwelling. These increases in water vapor and decreases in lower stratosphere ozone feed back onto lower stratosphere temperature through radiative cooling. The radiative cooling from ozone is about a factor of 2 larger than that from water vapor in the vicinity of the cold-point tropopause, while water vapor dominates at heights above 50 hPa. For halocarbons this indirect radiative cooling more than offsets the direct radiative warming, and together with the adiabatic cooling accounts for the lack of a halocarbon-induced warming of the lower stratosphere. For CO2 the indirect cooling from increased water vapor and decreased ozone is of comparable magnitude to the direct warming from CO2 in the vicinity of the cold-point tropopause, and (together with the increased upwelling) lowers the height at which CO2 increases induce stratospheric cooling, thus explaining the relatively weak increase in cold-point temperature due to the CO2 increases.

Interannual Variations of Stratospheric Water Vapor in MLS Observations and Climate Model Simulations

Abstract By analyzing the almost-decade-long record of water vapor measurements from the Microwave Limb Sounder (MLS) instrument on the NASA Aura satellite and by detailed diagnostic analysis of the results from state-of-the art climate model simulations, this study confirmed the conceptual picture of the interannual variation in equatorial stratospheric water vapor discussed in earlier papers (e.g., Geller et al.). The interannual anomalies in water vapor are strongly related to the dynamical quasi-biennial oscillation (QBO), and this study presents the first QBO composite of the time–height structure of the equatorial water vapor anomalies. The anomalies display upward propagation below about 10 hPa in a manner analogous to the annual “tape recorder” effect, but at higher levels they show clear downward propagation. This study examined these variations in the Model for Interdisciplinary Research on Climate (MIROC)-AGCM and in four models in phase 5 of the Coupled Model Intercomparison Project (CMIP5) that simulate realistic QBOs. Diagnostic budget analysis of the MIROC-AGCM data and comparisons among the CMIP5 model results demonstrate (i) the importance of temperature anomalies at the tropopause induced by the QBO for lower-stratospheric water vapor variations and (ii) that upper-stratospheric water vapor anomalies are largely driven by advection of the mean vertical gradient of water content by the QBO interannual fluctuations in the vertical wind.

Dry phase of tropical lower stratospheric water vapor: Role of BDC, convection and ozone variability

In the present paper, the relationship between dry phase of water vapor in the tropical lower stratosphere (TLS) and 100hPa temperatures (T100) has been examined. Role of various processes, such as Brewer–Dobson circulation (BDC), convective activities and seasonal minimum of ozone mixing ratio, has been quantified to explain the reason of low T100 over Indonesian-Australian western Pacific region (IAWPR). Aura MLS data show that low water vapor mixing ratio (WVMR) first appears over the western Pacific during northern hemisphere (NH) winters and directs the dry phase of TLS. Observations of low T100 (~188K), close association between WVMR and T100, slow transport of water vapor in TLS and saturation of air close to 82.5–100hPa over IAWPR indicate conditions favorable for 'freeze drying'. Present analysis has brought out several interesting features (a) in addition to BDC, convective activities and low ozone mixing ratio near the tropopause level seems to be contributing to the low T100 over IAWPR during NH winter/spring, (b) apart from the seasonal decrease, T100 over IAWPR is noted to be continually low throughout the year by ~1.2K than the zonal mean value where part of such decrease in T100 (i.e. ~0.7K) can be understood in terms of water vapor feedback process and (c) wave activity of different temporal scale and amplitude (~1–2K) also modulate T100 over IAWPR. MLS observations also provide an evidence of coupling between the surface and TLS processes, if the sea surface temperature over IAWPR is more than 301.7K.

Evaluation of aviation NOx-induced radiative forcings for 2005 and 2050

Aviation NOx emissions lead to the production of ozone (O3) and an OH increase in the troposphere and lower stratosphere. This OH increase results in a reduction of methane (CH4) which causes a longer-term reduction in O3 concentrations and lower stratospheric water vapor (SWV). Here we report new evaluations of a more comprehensive suite of aviation NOx-induced steady-state radiative forcing (RF) for 2006 aviation NOx emissions and for two different projections of 2050 NOx emissions and compare them with previously published analyses of aviation NOx-induced steady-state RFs. To do so, we evaluate the aviation NOx-induced steady-state RFs using the three-dimensional (3-D) global climate-chemistry Community Atmosphere Model (CAM), CAM4Chem. Moreover, we determine time dependent (transient) RFs for 2005 and the two 2050 emission scenarios by utilizing a parameterization based on specific RFs (steady-state RFs per unit of NOx emission) calculated in the 3-D model simulations, time-dependent NOx emissions data, and considering the lifetime of the perturbed species. For aviation NOx-induced effects we find that the net transient RFs differ from the linearly scaled steady-state RFs (specific steady-state RFs multiplied by NOx emissions) by +10%–36% for the different emission scenarios used in this study. These results indicate the importance of not using the transient and steady-state RF interchangeably, especially when comparing the aviation contribution in RF changes to contributions from other transportation sectors. Also, these results indicate that careful consideration is necessary when choosing whether to use the steady-state or transient RF when evaluating aviation NOx-induced RFs.

The potential impact of changes in lower stratospheric water vapour on stratospheric temperatures over the past 30 years

This study investigates the potential contribution of observed changes in lower stratospheric water vapour to stratospheric temperature variations over the past three decades using a comprehensive global climate model (GCM). Three case studies are considered. In the first, the net increase in stratospheric water vapour (SWV) from 1980–2010 (derived from the Boulder frost‐point hygrometer record using the gross assumption that this is globally representative) is estimated to have cooled the lower stratosphere by up to ∼0.2 K decade−1 in the global and annual mean; this is ∼40% of the observed cooling trend over this period. In the Arctic winter stratosphere there is a dynamical response to the increase in SWV, with enhanced polar cooling of 0.6 K decade−1 at 50 hPa and warming of 0.5 K decade−1 at 1 hPa. In the second case study, the observed decrease in tropical lower stratospheric water vapour after the year 2000 (imposed in the GCM as a simplified representation of the observed changes derived from satellite data) is estimated to have caused a relative increase in tropical lower stratospheric temperatures by ∼0.3 K at 50 hPa. In the third case study, the wintertime dehydration in the Antarctic stratospheric polar vortex (again using a simplified representation of the changes seen in a satellite dataset) is estimated to cause a relative warming of the Southern Hemisphere polar stratosphere by up to 1 K at 100 hPa from July–October. This is accompanied by a weakening of the westerly winds on the poleward flank of the stratospheric jet by up to 1.5 m s−1 in the GCM. The results show that, if the measurements are representative of global variations, SWV should be considered as important a driver of transient and long‐term variations in lower stratospheric temperature over the past 30 years as increases in long‐lived greenhouse gases and stratospheric ozone depletion.

Temperature trends in the tropical upper troposphere and lower stratosphere: Connections with sea surface temperatures and implications for water vapor and ozone

Satellite observations and chemistry‐climate model experiments are used to understand the zonal structure of tropical lower stratospheric temperature, water vapor, and ozone trends. The warming in the tropical upper troposphere over the past 30 years is strongest near the Indo‐Pacific warm pool, while the warming trend in the western and central Pacific is much weaker. In the lower stratosphere, these trends are reversed: the historical cooling trend is strongest over the Indo‐Pacific warm pool and is weakest in the western and central Pacific. These zonal variations are stronger than the zonal‐mean response in boreal winter. Targeted experiments with a chemistry‐climate model are used to demonstrate that sea surface temperature (hereafter SST) trends are driving the zonal asymmetry in upper tropospheric and lower stratospheric tropical temperature trends. Warming SSTs in the Indian Ocean and in the warm pool region have led to enhanced moist heating in the upper troposphere, and in turn to a Gill‐like response that extends into the lower stratosphere. The anomalous circulation has led to zonal structure in the ozone and water vapor trends near the tropopause, and subsequently to less water vapor entering the stratosphere. The radiative impact of these changes in trace gases is smaller than the direct impact of the moist heating. Projected future SSTs appear to drive a temperature and water vapor response whose zonal structure is similar to the historical response. In the lower stratosphere, the changes in water vapor and temperature due to projected future SSTs are of similar strength to, though slightly weaker than, that due directly to projected future CO2, ozone, and methane.

Modeling upper tropospheric and lower stratospheric water vapor anomalies

Abstract. The domain-filling, forward trajectory calculation model developed by Schoeberl and Dessler (2011) is used to further investigate processes that produce upper tropospheric and lower stratospheric water vapor anomalies. We examine the pathways parcels take from the base of the tropical tropopause layer (TTL) to the lower stratosphere. Most parcels found in the lower stratosphere arise from East Asia, the Tropical West Pacific (TWP) and Central/South America. The belt of TTL parcel origins is very wide compared to the final dehydration zones near the top of the TTL. This is due to the convergence of rising air due to the stronger diabatic heating near the tropopause relative to levels above and below. The observed water vapor anomalies – both wet and dry – correspond to regions where parcels have minimal displacement from their initialization. These minimum displacement regions include the winter TWP and the Asian and American monsoons. To better understand the stratospheric water vapor concentration we introduce the water vapor spectrum and investigate the source of the wettest and driest components of the spectrum. We find that the driest air parcels originate below the TWP, moving upward to dehydrate in the TWP cold upper troposphere. The wettest air parcels originate at the edges of the TWP as well as in the summer American and Asian monsoons. The wet air parcels are important since they skew the mean stratospheric water vapor distribution toward higher values. Both TWP cold temperatures that produce dry parcels as well as extra-TWP processes that control the wet parcels determine stratospheric water vapor.

Correction technique for Raman water vapor lidar signal-dependent bias and suitability for water vapor trend monitoring in the upper troposphere

Abstract. The MOHAVE-2009 campaign brought together diverse instrumentation for measuring atmospheric water vapor. We report on the participation of the ALVICE (Atmospheric Laboratory for Validation, Interagency Collaboration and Education) mobile laboratory in the MOHAVE-2009 campaign. In appendices we also report on the performance of the corrected Vaisala RS92 radiosonde measurements during the campaign, on a new radiosonde based calibration algorithm that reduces the influence of atmospheric variability on the derived calibration constant, and on other results of the ALVICE deployment. The MOHAVE-2009 campaign permitted the Raman lidar systems participating to discover and address measurement biases in the upper troposphere and lower stratosphere. The ALVICE lidar system was found to possess a wet bias which was attributed to fluorescence of insect material that was deposited on the telescope early in the mission. Other sources of wet biases are discussed and data from other Raman lidar systems are investigated, revealing that wet biases in upper tropospheric (UT) and lower stratospheric (LS) water vapor measurements appear to be quite common in Raman lidar systems. Lower stratospheric climatology of water vapor is investigated both as a means to check for the existence of these wet biases in Raman lidar data and as a source of correction for the bias. A correction technique is derived and applied to the ALVICE lidar water vapor profiles. Good agreement is found between corrected ALVICE lidar measurments and those of RS92, frost point hygrometer and total column water. The correction is offered as a general method to both quality control Raman water vapor lidar data and to correct those data that have signal-dependent bias. The influence of the correction is shown to be small at regions in the upper troposphere where recent work indicates detection of trends in atmospheric water vapor may be most robust. The correction shown here holds promise for permitting useful upper tropospheric water vapor profiles to be consistently measured by Raman lidar within NDACC (Network for the Detection of Atmospheric Composition Change) and elsewhere, despite the prevalence of instrumental and atmospheric effects that can contaminate the very low signal to noise measurements in the UT.

Relationships between Brewer-Dobson circulation, double tropopauses, ozone and stratospheric water vapour

Abstract. Statistical relationships between the variability of the area covered by double tropopause events (DTs), the strength of the tropical upwelling, the total column ozone and of the lower stratospheric water vapour are analyzed. The QBO and ENSO signals in the double tropopause and tropical upwelling as well as their influence on the statistical relationships are also presented. The analysis is based on both reanalysed data (ERA-Interim) and satellite data. Significant anticorrelations were found between the area covered by DTs and the total column ozone in the midlatitudes of the Northern Hemisphere. This relationship is confirmed by a large positive correlation between the areas covered by ozone laminae and double tropopause events as found in the HIRDLS satellite dataset. Significant anticorrelations were also found between the global area of double tropopause events and the near global (50° S–50° N) water vapour in the lower stratosphere. The correlations of DT variables with total column ozone and ozone laminae are both consistent with the poleward displacement of tropical air with lower ozone mixing ratio and with tropospheric intrusions of tropical tropospheric air into the lower extratropical stratosphere. The association of DTs with the poleward displacements of the tropical air is also consistent with a strong positive correlation between the area covered by DTs and the wave activity in the lower most stratosphere, between the first and second lapse rate tropopauses, as found in the ERA-Interim reanalysis. Finally, a significant anticorrelation was found between the tropical upwelling and the near global lower stratospheric water vapour. Moreover, the step like decrease in the lower stratospheric water vapour after 2001 is mirrored by a step like increase in the tropical upwelling.

Revisiting the lower stratospheric water vapour trend from the 1950s to 1970s

Previous work showed a near-continuous increase in stratospheric water vapour between the 1950s and 1990s from a variety of instruments, without recourse to fits between instruments. We reassess the trend from the earliest, the UK frost-point hygrometer, 1954–1976. An error in previous work omitted to transform values from ppmm to ppmv. When corrected, they fit more convincingly with measurements by later frost-point hygrometers. Minor instrument changes between the 1950s and 1970s do not introduce a potential bias to the trend but do increase its error. If the full 1970s data are included, the trend becomes 2.1 ± 0.8%/year (two-sigma). Copyright © 2011 Royal Meteorological Society

Ozone concentration changes in the Asian summer monsoon anticyclone and lower stratospheric water vapour: An idealised model study

[1] Satellite observations and model studies have previously established the impact of the Asian Summer Monsoon on the composition of the upper troposphere and lower stratosphere, where a region of enhanced water vapour and decreased ozone is found in the Monsoon anticyclone. We investigate a potential link between the magnitude of the Monsoon-induced ozone minimum and water vapour concentrations. In three idealised climate model experiments we prescribe ozone climatologies, decreasing or increasing ozone in the anticyclone region relative to the annual cycle during northern hemisphere summer. We discuss the modelled temperature and water vapour response. While water vapour decreases significantly when lower ozone is prescribed, it changes very little when higher ozone is prescribed, illustrating an important asymmetry between forcing and response.

A study of upper troposphere and lower stratosphere water vapor above the Tibetan Plateau using AIRS and MLS data

AbstractWe use water vapor data from Atmospheric Infrared Sounder (AIRS) and Aura Microwave Limb Sounder (MLS) combined with meteorological data from ECMWF Interim (ERA‐Interim) reanalysis, to study some aspects of stratosphere–troposphere exchange (STE) near the Tibetan Plateau. Apart from a distinctive region of high water vapor in the lower stratosphere (LS) in summer near the southern Tibetan Plateau (between 30°N and 35°N), the water vapor in the upper troposphere and lower stratosphere (UTLS) adjacent to the northern Tibetan Plateau (40°N–45°N) is found to be relatively higher than the surrounding regions of the same latitude in March and April. This relatively high water vapor in the northern Tibetan Plateau UTLS is proposed to be associated with approaching cold surges from the north and forced lifting of air by high orography. Another interesting feature detected in this study is the region of low water vapor values on the order of 5–7 ppmv, that is more pronounced from May to September at around 200 hPa and located at 30°N–40°N western Tibetan Plateau. This low water vapor region is found to be related to an anticyclone developed at the western Tibetan Plateau which causes sinking of dry air from the stratosphere resulting lower water vapor values in the upper troposphere. Copyright © 2011 Royal Meteorological Society

Airborne and Ground-Based Measurements Using a High-Performance Raman Lidar

Abstract A high-performance Raman lidar operating in the UV portion of the spectrum has been used to acquire, for the first time using a single lidar, simultaneous airborne profiles of the water vapor mixing ratio, aerosol backscatter, aerosol extinction, aerosol depolarization and research mode measurements of cloud liquid water, cloud droplet radius, and number density. The Raman Airborne Spectroscopic Lidar (RASL) system was installed in a Beechcraft King Air B200 aircraft and was flown over the mid-Atlantic United States during July–August 2007 at altitudes ranging between 5 and 8 km. During these flights, despite suboptimal laser performance and subaperture use of the telescope, all RASL measurement expectations were met, except that of aerosol extinction. Following the Water Vapor Validation Experiment—Satellite/Sondes (WAVES_2007) field campaign in the summer of 2007, RASL was installed in a mobile trailer for ground-based use during the Measurements of Humidity and Validation Experiment (MOHAVE-II) field campaign held during October 2007 at the Jet Propulsion Laboratory’s Table Mountain Facility in southern California. This ground-based configuration of the lidar hardware is called Atmospheric Lidar for Validation, Interagency Collaboration and Education (ALVICE). During the MOHAVE-II field campaign, during which only nighttime measurements were made, ALVICE demonstrated significant sensitivity to lower-stratospheric water vapor. Numerical simulation and comparisons with a cryogenic frost-point hygrometer are used to demonstrate that a system with the performance characteristics of RASL–ALVICE should indeed be able to quantify water vapor well into the lower stratosphere with extended averaging from an elevated location like Table Mountain. The same design considerations that optimize Raman lidar for airborne use on a small research aircraft are, therefore, shown to yield significant dividends in the quantification of lower-stratospheric water vapor. The MOHAVE-II measurements, along with numerical simulation, were used to determine that the likely reason for the suboptimal airborne aerosol extinction performance during the WAVES_2007 campaign was a misaligned interference filter. With full laser power and a properly tuned interference filter, RASL is shown to be capable of measuring the main water vapor and aerosol parameters with temporal resolutions of between 2 and 45 s and spatial resolutions ranging from 30 to 330 m from a flight altitude of 8 km with precision of generally less than 10%, providing performance that is competitive with some airborne Differential Absorption Lidar (DIAL) water vapor and High Spectral Resolution Lidar (HSRL) aerosol instruments. The use of diode-pumped laser technology would improve the performance of an airborne Raman lidar and permit additional instrumentation to be carried on board a small research aircraft. The combined airborne and ground-based measurements presented here demonstrate a level of versatility in Raman lidar that may be impossible to duplicate with any other single lidar technique.

Seasonal to decadal variations of water vapor in the tropical lower stratosphere observed with balloon‐borne cryogenic frost point hygrometers

We investigated water vapor variations in the tropical lower stratosphere on seasonal, quasi‐biennial oscillation (QBO), and decadal time scales using balloon‐borne cryogenic frost point hygrometer data taken between 1993 and 2009 during various campaigns including the Central Equatorial Pacific Experiment (March 1993), campaigns once or twice annually during the Soundings of Ozone and Water in the Equatorial Region (SOWER) project in the eastern Pacific (1998–2003) and in the western Pacific and Southeast Asia (2001–2009), and the Ticosonde campaigns and regular sounding at Costa Rica (2005–2009). Quasi‐regular sounding data taken at Costa Rica clearly show the tape recorder signal. The observed ascent rates agree well with the ones from the Halogen Occultation Experiment (HALOE) satellite sensor. Average profiles from the recent five SOWER campaigns in the equatorial western Pacific in northern winter and from the three Ticosonde campaigns at Costa Rica (10°N) in northern summer clearly show two effects of the QBO. One is the vertical displacement of water vapor profiles associated with the QBO meridional circulation anomalies, and the other is the concentration variations associated with the QBO tropopause temperature variations. Time series of cryogenic frost point hygrometer data averaged in a lower stratospheric layer together with HALOE and Aura Microwave Limb Sounder data show the existence of decadal variations: The mixing ratios were higher and increasing in the 1990s, lower in the early 2000s, and probably slightly higher again or recovering after 2004. Thus linear trend analysis is not appropriate to investigate the behavior of the tropical lower stratospheric water vapor.