Low Magnetic Damping Research Articles

High spin mixing conductance and spin interface transparency at the interface of a Co2Fe0.4Mn0.6Si Heusler alloy and Pt

Ferromagnetic materials exhibiting low magnetic damping (α) and moderately high-saturation magnetization are required from the viewpoints of generation, transmission, and detection of spin waves. Since spin-to-charge conversion efficiency is another important parameter, high spin mixing conductance ({g_{r}^{uparrow downarrow}}) is the key for efficient spin-to-charge conversion. Full Heusler alloys, e.g., Co2Fe0.4Mn0.6Si (CFMS), which are predicted to be 100% spin-polarized, exhibit low α. However, g_r^{ uparrow downarrow } at the interface between CFMS and a paramagnet is not fully understood. Here, we report investigations of spin pumping and the inverse spin Hall effect in CFMS/Pt bilayers. Damping analysis indicates the presence of significant spin pumping at the interface of CFMS and Pt, which is also confirmed by the detection of an inverse spin Hall voltage. We show that in CFMS/Pt, g_r^{ uparrow downarrow } (1.70 × 1020 m−2) and the interface transparency (83%) are higher than the values reported for other ferromagnetic/heavy metal systems. We observed a spin Hall angle of ~0.026 for the CFMS/Pt bilayer system.

Long-distance spin-transport across the Morin phase transition up to room temperature in ultra-low damping single crystals of the antiferromagnet \u03b1-Fe2O3

Antiferromagnetic materials can host spin-waves with polarizations ranging from circular to linear depending on their magnetic anisotropies. Until now, only easy-axis anisotropy antiferromagnets with circularly polarized spin-waves were reported to carry spin-information over long distances of micrometers. In this article, we report long-distance spin-transport in the easy-plane canted antiferromagnetic phase of hematite and at room temperature, where the linearly polarized magnons are not intuitively expected to carry spin. We demonstrate that the spin-transport signal decreases continuously through the easy-axis to easy-plane Morin transition, and persists in the easy-plane phase through current induced pairs of linearly polarized magnons with dephasing lengths in the micrometer range. We explain the long transport distance as a result of the low magnetic damping, which we measure to be ≤ 10−5 as in the best ferromagnets. All of this together demonstrates that long-distance transport can be achieved across a range of anisotropies and temperatures, up to room temperature, highlighting the promising potential of this insulating antiferromagnet for magnon-based devices.

Ultra-low magnetic damping in epitaxial Li0.5Fe2.5O4 thin films

The realization of more energy efficient nanomagnetic information devices relies on the existence of magnetic insulators capable of supporting pure spin currents in the absence of a dissipative charge current. Currently, there is a limited number of thin-film magnetic insulators with low magnetic damping. Li0.5Fe2.5O4 (LFO) is well known to possess the lowest damping among the bulk spinel structure oxides, but, thus far, LFO thin films have not lived up to these expectations. Here, we demonstrate low magnetic damping (even lower than typical bulk values) and bulk magnetization in 3 nm thick epitaxial LFO thin films. At room temperature, SQUID magnetometry shows a high saturation magnetization of 320 kA/m, and broadband ferromagnetic resonance measurements yield an effective Gilbert damping parameter of 1.3×10−3, which is among the lowest reported for ferro-/ferrimagnetic films of comparable thickness. Our results show the promise of LFO as a candidate material for spin current-based spintronics.

Spin Wave Excitation, Detection, and Utilization in the Organic-Based Magnet, V(TCNE)x (TCNE = Tetracyanoethylene).

Spin waves, quantized as magnons, have low energy loss and magnetic damping, which are critical for devices based on spin-wave propagation needed for information processing devices. The organic-based magnet [V(TCNE)x ; TCNE = tetracyanoethylene; x ≈ 2] has shown an extremely low magnetic damping comparable to, for example, yttrium iron garnet (YIG). The excitation, detection, and utilization of coherent and non-coherent spin waves on various modes in V(TCNE)x is demonstrated and show that the angular momentum carried by microwave-excited coherent spin waves in a V(TCNE)x film can be transferred into an adjacent Pt layer via spin pumping and detected using the inverse spin Hall effect. The spin pumping efficiency can be tuned by choosing different excited spin wave modes in the V(TCNE)x film. In addition, it is shown that non-coherent spin waves in a V(TCNE)x film, excited thermally via the spin Seebeck effect, can also be used as spin pumping source that generates an electrical signal in Pt with a sign change in accordance with the magnetization switching of the V(TCNE)x . Combining coherent and non-coherent spin wave detection, the spin pumping efficiency can be thermally controlled, and new insight is gained for the spintronic applications of spin wave modes in organic-based magnets.

Influence of structure and cation distribution on magnetic anisotropy and damping in Zn/Al doped nickel ferrites

An in-depth analysis of Zn/Al doped nickel ferrites grown by reactive magnetron sputtering is relevant due to their promising characteristics for applications in spintronics. The material is insulating and ferromagnetic at room temperature with an additional low magnetic damping. By studying the complex interplay between strain and cation distribution their impact on the magnetic properties, i.e. anisotropy, damping and g-factor is unravelled. In particular, a strong influence of the lattice site occupation of Ni$^{2+}_{\text{Td}}$ and cation coordination of Fe$^{2+}_{\text{Oh}}$ on the intrinsic damping is found. Furthermore, the critical role of the incorporation of Zn$^{2+}$ and Al$^{3+}$ is evidenced by comparison with a sample of altered composition. Especially, the dopant Zn$^{2+}$ is evidenced as a tuning factor for Ni$^{2+}_{\text{Td}}$ and therefore unquenched orbital moments directly controlling the g-factor. A strain-independent reduction of the magnetic anisotropy and damping by adapting the cation distribution is demonstrated.

Nonlinear losses in magnon transport due to four-magnon scattering

We report on the impact of nonlinear four-magnon scattering on magnon transport in microstructured Co25Fe75 waveguides with low magnetic damping. We determine the magnon propagation length with microfocused Brillouin light scattering over a broad range of excitation powers and detect a decrease of the attenuation length at high powers. This is consistent with the onset of nonlinear four-magnon scattering. Hence, it is critical to stay in the linear regime, when deriving damping parameters from the magnon propagation length. Otherwise, the intrinsic nonlinearity of magnetization dynamics may lead to a misinterpretation of magnon propagation lengths and, thus, to incorrect values of the magnetic damping of the system.

Nanometer-Thick Yttrium Iron Garnet Films with Perpendicular Anisotropy and Low Damping

${\mathrm{Y}}_{3}{\mathrm{Fe}}_{5}{\mathrm{O}}_{12}$ ($\mathrm{YIG}$) thin films having a thickness of several nanometers and showing both strong perpendicular magnetic anisotropy (PMA) and low magnetic damping are reported. The films are deposited by magnetron sputtering at room temperature first and then annealed in ${\mathrm{O}}_{2}$ at high temperature. The substrates are ${\mathrm{Gd}}_{3}({\mathrm{Sc}}_{2}{\mathrm{Ga}}_{3}){\mathrm{O}}_{12}$, which share the same crystalline structure as $\mathrm{YIG}$, but have a lattice constant slightly larger than that of $\mathrm{YIG}$; the lattice mismatching gives rise to an out-of-plane compressive strain and PMA in the $\mathrm{YIG}$ films. The PMA is confirmed by vibrating sample magnetometer, magneto-optical Kerr effect, anomalous Hall effect, and angle-dependent ferromagnetic resonance (FMR) measurements. The damping of the films is analyzed through frequency-dependent FMR measurements. As an example, an 8-nm-thick $\mathrm{YIG}$ film shows an effective PMA field of about 2800 Oe, a nearly square hysteresis loop, and a damping constant of only $4.2\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}4}$. As an illustration of possible applications of such films in spintronic devices, current-induced switching of the magnetization of the PMA $\mathrm{YIG}$ films is demonstrated by the use of $\mathrm{YIG}$/$\mathrm{Pt}$ bilayered Hall bar devices.

A perpendicular graphene/ferromagnet electrode for spintronics

We report on the large-scale integration of graphene layers over a FePd perpendicular magnetic anisotropy (PMA) platform, targeting further downscaling of spin circuits. An L10 FePd ordered alloy showing both high magneto-crystalline anisotropy and a low magnetic damping constant, is deposited by magnetron sputtering. The graphene layer is then grown on top of it by large-scale chemical vapor deposition. A step-by-step study, including structural and magnetic analyses by x-ray diffraction and Kerr microscopy, shows that the measured FePd properties are preserved after the graphene deposition process. This scheme provides a graphene protected perpendicular spin electrode showing resistance to oxidation, atomic flatness, stable crystallinity, and perpendicular magnetic properties. This, in turn, opens the way to the generalization of hybrid 2D-materials on optimized PMA platforms, sustaining the development of spintronics circuits based on perpendicular spin-sources as required, for instance, for perpendicular-magnetic random-access memory schemes.

The role of iron in magnetic damping of Mg(Al,Fe)2O4 spinel ferrite thin films

We have investigated magnesium aluminum ferrite thin films with a range of iron concentrations and identified the optimal iron content to obtain high crystalline quality thin films with the low magnetic damping required for spin current-based applications. Epitaxial MgAl2−x FexO4 films with 0.8 < x < 2.0 were grown by pulsed laser deposition on single crystal MgAl2O4 substrates and were characterized structurally and magnetically. We find that the x = 1.5 composition minimizes the room-temperature magnetic damping with a typical Gilbert damping parameter of αeff=1.8×10−3. This minimized damping is governed by a competition between the more robust magnetic ordering with increased iron content, x, and the more defective structure due to larger film-substrate lattice mismatch with increased iron content. The temperature-dependent magnetization curves indicate that Tc is suppressed below room temperature for iron content x≤1.2 and eventually suppressed entirely for x = 0.8. X-ray magnetic circular dichroism results indicate that for all x the magnetic moment is dominated by Fe3+ cations distributed in a 60:40 ratio on the octahedral and tetrahedral sites, with minimal contribution from Fe2+ cations. Films with x=1.4−1.6 exhibit very strong ferromagnetic resonance and low Gilbert damping with αeff=(1.8−6)×10−3, making them ideal candidates for microwave and spintronic applications.

Polycrystalline Co2Mn-based Heusler thin films with high spin polarization and low magnetic damping

Spin-polarization and magnetic damping are measured for several polycrystalline films with each of them being made of a different single Co2Mn-based Heusler compound. As several epitaxial Co2Mn-based Heusler compounds are shown to be half-metal magnetic materials with full spin-polarization and ultralow magnetic damping, we explore here these properties but in polycrystalline films. Co2MnSi, Co2MnGe, and Co2MnGa thin films were grown on glass substrates and analyzed in situ by electron diffraction and spin-resolved photoemission and ex situ by transmission electron microscopy and ferromagnetic resonance. Despite the polycrystalline state of the films, they still exhibit high spin polarizations and very low magnetic damping coefficients. The latter are at least of the same order as the best epitaxial films using regular ferromagnetic materials. The key point to achieve such properties is to control the Heusler stoichiometry as best as possible.

Low Magnetic Damping of Ferrimagnetic GdFeCo Alloys.

We investigate the Gilbert damping parameter α for rare earth (RE)-transition metal (TM) ferrimagnets over a wide temperature range. Extracted from the field-driven magnetic domain-wall mobility, α was as low as the order of 10^{-3} and was almost constant across the angular momentum compensation temperature T_{A}, starkly contrasting previous predictions that α should diverge at T_{A} due to a vanishing total angular momentum. Thus, magnetic damping of RE-TM ferrimagnets is not related to the total angular momentum but is dominated by electron scattering at the Fermi level where the TM has a dominant damping role. This low value of the Gilbert damping parameter suggests that ferrimagnets can serve as versatile platforms for low-dissipation high-speed magnetic devices.

Current-Induced Nucleation and Dynamics of Skyrmions in a Co -based Heusler Alloy

We demonstrate room-temperature stabilization of dipolar magnetic skyrmions with diameters in the range of $100$ nm in a single ultrathin layer of the Heusler alloy Co$_2$FeAl (CFA) under moderate magnetic fields. Current-induced skyrmion dynamics in microwires is studied with a scanning Nitrogen-Vacancy magnetometer operating in the photoluminescence quenching mode. We first demonstrate skyrmion nucleation by spin-orbit torque and show that its efficiency can be significantly improved using tilted magnetic fields, an effect which is not specific to Heusler alloys and could be advantageous for future skyrmion-based devices. We then show that current-induced skyrmion motion remains limited by strong pinning effects, even though CFA is a magnetic material with a low magnetic damping parameter.

Investigation of spin Seebeck effect and magnetic damping in nanometer thick Ce0.5Y2.5Fe5O12 films

The ferromagnetic insulators (FMI) involving the phonon-magnon interaction in generation of spin currents are providing new opportunities to explore the thermal to electrical conversion efficiency in comparison to electron based themoelectrics. Here, we have investigated the magnetic damping behavior and spin Seebeck effect in crystalline, highly smooth surfaced, nano-meter thick FMI Ce0.5Y2.5Fe5O12 (CeYIG) films, synthesized via pulsed laser deposition technique, for their application in spin caloritronics. The CeYIG films reveal an increase of saturation magnetization, strong magnetic anisotropy and a very low magnetic damping, optimum for investigation of pure spin currents generated via inverse spin Hall Effect. The room temperature longitudinal spin Seebeck effect (LSSE) was observed on sputtering of 8 nm thick Hall bar patterned rhodium (Rh) on CeYIG films. The magnitude of LSSE voltage obtained showed a characteristic increase and saturation of signal with the increase of film thickness, indicating the origin of spin current generation from the bulk of CeYIG film. The pure spin Hall magnetoresistance (SMR) was observed in temperature range of 5–300 K implying the LSSE observed in Rh layer is purely from the spin current generated within the FMI and free from parasitic magnetic proximity effect (MPE). The use of Rh as a normal metal for the detection of spin current can open a new window in the exploration of pure spin current related phenomena.

The observation of inherent spin Seebeck effect in Rh/YIG hybrid structure

Rhodium (Rh) is a 4d metal possessing a large spin orbit coupling strength and spin-Hall conductivity with a very small magnetic susceptibility, implying an insignificant magnetic proximity effect (MPE). We report here the observation of longitudinal spin Seebeck effect (LSSE) using Rh as a normal metal. A Rh film was sputtered on nanometer thick YIG films of highly crystalline nature and extremely low magnetic damping to obtain Rh/YIG hybrid structure. A clear thermal voltage Vth (SSE voltage) was obtained when a temperature gradient was applied on the Rh/YIG hybrid. The Rh film showed a very weak anomalous Hall resistance and the magneto-resistive testing clearly ruled out the magnetization of the Rh films via MPE. The anisotropic magnetoresistance (AMR) revealed a clear spin hall magnetoresistance (SMR) signal in Rh film implying a purely intrinsic spin current generation, free from any parasitic magnetic effects. The work can open a new window in the study of pure and uncontaminated spin current, generated in ferromagnetic insulators, using Rh as spin current detector.

Spin–Orbit Torque Switching in a Nearly Compensated Heusler Ferrimagnet

Ferrimagnetic materials combine the advantages of the low magnetic moment of an antiferromagnet and the ease of realizing magnetic reading of a ferromagnet. Recently, it was demonstrated that compensated ferrimagnetic half metals can be realized in Heusler alloys, where high spin polarization, zero magnetic moment, and low magnetic damping can be achieved at the same time. In this work, by studying the spin-orbit torque induced switching in the Heusler alloy Mn2 Ru1- x Ga, it is found that efficient current-induced magnetic switching can be realized in a nearly compensated sample with strong perpendicular anisotropy and large film thickness. This work demonstrates the possibility of employing compensated Heusler alloys for fast, energy-efficient spintronic devices.

Magnetic and thermal properties of ferromagnetic insulator: Yttrium Iron Garnet

We present here the magneto thermal properties, damping behavior and effect of Cerium doping on ferromagnetic insulator Yttrium Iron Garnet (YIG), synthesized via solid state method and Spark Plasma Sintering. The thermal conductivity was measured using Laser Flash technique in the temperature range of 300–1000° K. A decrease in thermal conductivity was observed up to the Curie temperature of YIG, beyond which it showed a constant behavior. On Ce doping of YIG, 15% enhancement of thermal conductivity was achieved, besides leading to an increase of magnetic moment at all temperatures. This gain is attributed to the increase of grain size and replacement of diamagnetic Y3+ ions in YIG by paramagnetic Ce3+ ions in Ce doped YIG. The spark plasma sintered YIG showed a decrease in particle size and grain size resulting in decrease of both thermal conductivity and saturation magnetization. The damping parameters obtained from ferromagnetic resonance measurement revealed a very low magnetic damping even on Ce doping. The work provides effective information regarding the enhancement of spin dynamic properties of YIG suitable for spin-caloritronic applications.

Pseudomorphic spinel ferrite films with perpendicular anisotropy and low damping

We report on epitaxial thin films of spinel ferrite Ni0.65Zn0.35Fe1.2Al0.8O4 with strain-induced perpendicular magnetic anisotropy (PMA) and low magnetic damping. Static magnetometry and broadband ferromagnetic resonance experiments show a distinct change in the preferred direction of magnetization from in-plane to out-of-plane when the coherent strain in films changes from ∼2% compressive on (001) MgAl2O4 to ∼0.5% tensile on (001) MgGa2O4 substrates. Significant deviations from the spin-only value (2.0) of the g-factor suggest spin-orbit effects and further support our conclusion of strain-driven magnetic anisotropy in these films. The low Gilbert damping parameter of α = 5 × 10−3 in these ferrite films, combined with their PMA, makes them promising for spintronic and frequency-agile microwave device applications.

Low magnetic damping and large negative anisotropic magnetoresistance in half-metallic Co2−xMn1+xSi Heusler alloy films grown by molecular beam epitaxy

Co2−xMn1+xSi films with various composition x were epitaxially grown using molecular beam epitaxy (MBE). High crystallinity and atomic ordering in the prepared Co2−xMn1+xSi films were observed, and their magnetic damping and anisotropic magnetoresistance (AMR) effect were systematically investigated. An ultra-low magnetic damping constant of 0.0007 was obtained in the Co2−xMn1+xSi film with a valence electron number (NV) of about 29.0. Additionally, a relatively large negative AMR effect was observed in the Co2−xMn1+xSi films that had a NV of about 29.0. This low damping and the large negative AMR effect indicate that epitaxial Co2−xMn1+xSi films with high atomic ordering grown by MBE possess a high-spin polarization.

Strongly extended diffusion length for the nonequilibrium magnons in Y3Fe5O12 by photoexcitation

Deliberate control of magnon transportation will lead to an energy-efficient technology for information transmission and processing. Y3Fe5O12(YIG), exhibiting extremely large magnon diffusion length due to the low magnetic damping constant, has been intensively investigated for decades. While most of the previous works focused on the determination of magnon diffusion length by various techniques, herein we demonstrated how to tune magnon diffusion by light excitation. We found that the diffusion length of thermal magnons is strongly dependent on light wavelength when the magnon is generated by exposing YIG directly to laser beam. The diffusion length, determined by a nonlocal geometry at room temperature, is ~30 um for the magnons produced by visible light (400-650 nm), and ~136-156 um for the laser between 808 nm and 980 nm. The diffusion distance is much longer than the reported value. In addition to thermal gradient, we found that light illumination affected the electron configuration of the Fe3+ ion in YIG. Long wavelength laser triggers a high spin to low spin state transition of the Fe3+ ions in FeO6 octahedron. This in turn causes a substantial softening of the magnon thus a dramatic increase in diffusion distance. The present work paves the way towards an efficient tuning of magnon transport behavior which is crucially important for magnon spintronics.

Electronic, elastic and X-ray spectroscopic properties of direct and inverse full Heusler compounds Co2FeAl and Fe2CoAl, promising materials for spintronic applications: a DFT+Uapproach

Half-metallicity, low magnetic damping and high Curie temperatures (TC) are crucial for application in spintronics and full Heusler alloys are promising in this regard.