Limit Of Weak Interactions Research Articles

Interaction-Driven Instabilities in the Random-Field XXZ Chain.

Despite enormous efforts devoted to the study of the many-body localization (MBL) phenomenon, the nature of the high-energy behavior of the Heisenberg spin chain in a strong random magnetic field is lacking consensus. Here, we take a step back by exploring the weak interaction limit starting from the Anderson localized (AL) insulator. Through shift-invert diagonalization, we find that, below a certain disorder threshold h^{*}, weak interactions necessarily lead to an ergodic instability, whereas at strong disorder the AL insulator directly turns into MBL, in agreement with a simple interpretation of the avalanche theory for restoration of ergodicity. We further map the phase diagram for the generic XXZ model in the disorder h-interaction Δ plane. Taking advantage of the total magnetization conservation, our results unveil the remarkable behavior of the spin-spin correlation functions: in the regime indicated as MBL by standard observables, their exponential decay undergoes an inversion of orientation ξ_{z}>ξ_{x}. We find that the longitudinal length ξ_{z} is a key quantity for capturing ergodic instabilities, as it increases with system size near the thermal phase, in sharp contrast to its transverse counterpart.

Two atoms in a harmonic trap with spin-orbital-angular-momentum coupling

We study the problem of two harmonically trapped atoms in the presence of spin-orbital-angular-momentum (SOAM) coupling. The two-body energy spectrum is numerically calculated by utilizing the exact diagonalization method. We analyze how the degeneracy of energy levels is lifted under the interplay between the interatomic interaction and SOAM coupling. The exact numerical results show excellent agreement with that of perturbation theory in the weak-interaction limit as well as that in the absence of SOAM coupling. The properties of correlations between the two atoms are also discussed with respect to the interaction strength. The findings in this paper may provide valuable insights into few-body physics subjected to SOAM coupling and the possible experimental detection of spectrum functions in many-body systems, such as radiofrequency spectroscopy. Published by the American Physical Society 2024

Superconductivity in monolayer Janus titanium-sulfur hydride (TiSH) at ambient pressure

Janus two dimensional (2D) materials are new and novel materials. As they break out-of-plane symmetry, they possess several fascinating properties which can be applied in catalytic reactions and opto-electronics. Recent synthesis of MoSH and the prediction of phonon-mediated superconductivity have opened a new way to investigate the properties of hydrogenated Janus materials (Novoselov et al 2004 Science 306 666–9; Mehta et al 2023 Solid State Commun. 375 115347; Naik et al 2023 Comput. Theor. Chem. 1228 114278). In this work, we performed the density functional theory calculations to demonstrate that titanium sulfur hydride (TiSH) is dynamically stable and becomes phonon-mediated superconductor with the superconducting critical temperature, Tc = 9.24 K with the corresponding value of electron–phonon coupling constant, λ = 0.71, in the weak interaction limits, under ambient conditions. Eliashberg spectral function α2F(ω) was well converged for dense grid of q1 × q2 × q3 = 12 × 12 × 1 and nk1 × nk2 × nk3 = 140 × 140 × 1. The effect of smearing broadening was also considered for determining well converged value of Tc and λ. Figure (b) shows that after smearing broadening of 0.02 Ry, λ shows convergent values, and subsequent changes are as low as less that 5% of the peak value. Overall, our findings predicted a new member in the 2D Janus hydride family with possible applications in 2D nanomaterials and superconducting devices applications.

Trapped vortex dynamics implemented in composite Bessel beams

The divergence-free nature of Bessel beams can be harnessed to effectively trap optical vortices in free space laser propagation. We show how to generate arbitrary vortex configurations in Bessel traps to investigate few-body vortex interactions within a dynamically evolving fluid of light, which is a formal analog to a non-interacting Bose gas. We implement—theoretically and experimentally—initial conditions of vortex configurations first predicted in harmonically trapped quantum fluids, in the limit of weak atomic interactions, and model and measure the resultant dynamics. These hard trap dynamics are distinct from the harmonic trap predictions due to the non-local interactions that occur among the hard-wall boundary and steep phase gradients that nucleate other vortices. By simultaneously presenting experimental demonstrations with the theoretical proposal, we validate the potential application of using Bessel hard-wall traps as testing grounds for engineering few-body vortex interactions within trapped, two-dimensional compressible fluids.

Adiabatic connection interaction strength interpolation method made accurate for the uniform electron gas.

The adiabatic connection interaction strength interpolation (ISI)-like method provides a high-level expression for the correlation energy, being, in principle, exact not only in the weak-interaction limit, where it recovers the second-order Görling-Levy perturbation term, but also in the strong-interaction limit that is described by the strictly correlated electron approach. In this work, we construct a genISI functional made accurate for the uniform electron gas, a solid-state physics paradigm that is a very difficult test for ISI-like correlation functionals. We assess the genISI functional for various jellium spheres with the number of electrons Z ≤ 912 and for the non-relativistic noble atoms with Z ≤ 290. For the jellium clusters, the genISI is remarkably accurate, while for the noble atoms, it shows a good performance, similar to other ISI-like methods. Then, the genISI functional can open the path using the ISI-like method in solid-state calculations.

Exact Quantum Virial Expansion for the Optical Response of Doped Two-Dimensional Semiconductors.

We introduce a quantum virial expansion for the optical response of a doped two-dimensional semiconductor. As we show, this constitutes a perturbatively exact theory in the high-temperature or low-doping regime, where the electrons' thermal wavelength is smaller than their interparticle spacing. We obtain exact analytic expressions for the photoluminescence and we predict new features such as a nontrivial shape of the attractive branch peak related to universal resonant exciton-electron scattering and an associated energy shift from the trion energy. Our theory furthermore allows us to formally unify the two distinct theoretical pictures that have been applied to this system, where we reveal that the predictions of the conventional trion picture correspond to a high-temperature and weak-interaction limit of Fermi-polaron theory. Our results are in excellent agreement with recent experiments on doped monolayer MoSe_{2} and they provide the foundation for modeling a range of emerging optically active materials such as van der Waals heterostructures.

Quantum Otto cycle under strong coupling.

Quantum heat engines are often discussed under the weak-coupling assumption that the interaction between the system and the reservoirs is negligible. Although this setup is easier to analyze, this assumption cannot be justified on the quantum scale. In this study, a quantum Otto cycle model that can be generally applied without the weak-coupling assumption is proposed. We replace the thermalization process in the weak-coupling model with a process comprising thermalization and decoupling. The efficiency of the proposed model is analytically calculated and indicates that, when the contribution of the interaction terms is neglected in the weak-interaction limit, it reduces to that of the earlier model. The sufficient condition for the efficiency of the proposed model not to surpass that of the weak-coupling model is that the decoupling processes of our model have a positive cost. Moreover, the relation between the interaction strength and the efficiency of the proposed model is numerically examined by using a simple two-level system. Furthermore, we show that our model's efficiency can surpass that of the weak-coupling model under particular cases. From analyzing the majorization relation, we also find a design method of the optimal interaction Hamiltonians, which are expected to provide the maximum efficiency of the proposed model. Under these interaction Hamiltonians, the numerical experiment shows that the proposed model achieves higher efficiency than that of its weak-coupling counterpart.

Dissipation Mechanisms in Fermionic Josephson Junction.

We characterize numerically the dominant dynamical regimes in a superfluid ultracold fermionic Josephson junction. Beyond the coherent Josephson plasma regime, we discuss the onset and physical mechanism of dissipation due to the superflow exceeding a characteristic speed, and provide clear evidence distinguishing its physical mechanism across the weakly and strongly interacting limits, despite qualitative dynamics of global characteristics being only weakly sensitive to the operating dissipative mechanism. Specifically, dissipation in the strongly interacting regime occurs through the phase-slippage process, caused by the emission and propagation of quantum vortices, and sound waves-similar to the Bose-Einstein condensation limit. Instead, in the weak interaction limit, the main dissipative channel arises through the pair-breaking mechanism.

The grazing collisions limit from the linearized Boltzmann equation to the Landau equation for short-range potentials

The Landau equation and the Boltzmann equation are connected through the limit of grazing collisions. This has been proved rigorously for certain families of Boltzmann operators concentrating on grazing collisions. In this contribution, we study the collision kernels associated to the two-particle scattering via a finite range potential $ \Phi(x) $ in three dimensions. We then consider the limit of weak interaction given by $ \Phi_ \epsilon(x) = \epsilon \Phi(x) $. Here $ \epsilon\rightarrow 0 $ is the grazing parameter, and the rate of collisions is rescaled to obtain a non-trivial limit. The grazing collisions limit is of particular interest for potentials with a singularity of order $ s\geq 0 $ at the origin, i.e. $ \phi(x) \sim |x|^{-s} $ as $ |x|\rightarrow 0 $. For $ s\in [0,1] $, we prove the convergence to the Landau equation with diffusion coefficient given by the Born approximation, as predicted in the works of Landau and Balescu. On the other hand, for potentials with $ s>1 $ we obtain the non-cutoff Boltzmann equation in the limit. The Coulomb singularity $ s = 1 $ appears as a threshold value with a logarithmic correction to the diffusive timescale, the so-called Coulomb logarithm.

On self-energy contributions near Berezinskii–Kosterlitz–Thouless transition in interacting homogeneous 2D Bose system

ABSTRACT We explore the consequences of including quantum corrections in an interacting 2D Bose system near Berezinskii–Kosterlitz–Thouless (BKT) transition. To go beyond mean-field theory and treat correlations, we use Matsubara Green's function method, and, following a previous novel approach, study features of the interacting Green's function just above the transition. We numerically obtain self-consistent solutions of boson self-energy to second order as well as higher order (re-summation of ladder and bubble diagrams) in the interaction strength, for the entire range of momentum, k, and compare our findings with analytic results in the limits of low- and high-k. Thereby, in the weak interaction limit, we retrieve the universal transition condition and calculate the universal scaling parameter (independent of interaction strength). The renormalised single-particle Green's function is found to decay algebraically at large distance r.

Interpolating between small- and large- g expansions using Bayesian model mixing

Bayesian model mixing (BMM) is a statistical technique that can be used to combine models that are predictive in different input domains into a composite distribution that has improved predictive power over the entire input space. We explore the application of BMM to the mixing of two expansions of a function of a coupling constant $g$ that are valid at small and large values of $g$ respectively. This type of problem is quite common in nuclear physics, where physical properties are straightforwardly calculable in strong and weak interaction limits or at low and high densities or momentum transfers, but difficult to calculate in between. Interpolation between these limits is often accomplished by a suitable interpolating function, e.g., Pad\'e approximants, but it is then unclear how to quantify the uncertainty of the interpolant. We address this problem in the simple context of the partition function of zero-dimensional ${\ensuremath{\phi}}^{4}$ theory, for which the (asymptotic) expansion at small $g$ and the (convergent) expansion at large $g$ are both known. We consider three mixing methods: linear mixture BMM, localized bivariate BMM, and localized multivariate BMM with Gaussian processes. We find that employing a Gaussian process in the intermediate region between the two predictive models leads to the best results of the three methods. The methods and validation strategies we present here should be generalizable to other nuclear physics settings.

Tunneling density of states in a Luttinger liquid in proximity to a superconductor: Effect of nonlocal interaction

A recent study have shown that it is possible to have enhancement, in contrast to an expected suppression, in tunneling density of states (TDOS) in a Luttinger liquid (LL) which is solely driven by the non-local density-density interactions. Also, it is well known that a LL in proximity to a superconductor (SC) shows enhancement in TDOS in the vicinity of the junction in the zero energy limit. In this paper, we study the interplay of nonlocal density-density interaction and superconducting correlations in the TDOS in the vicinity of the SC-LL junction, where the LL maybe realized on the edge of an integer or a fractional quantum Hall state. We show that the TDOS enhancement in a LL quantum wire (QW) due to superconducting correlation at the junction can be farther amplified in presence of appropriate choice of non-local interaction parameters, which is demonstrated through a neat algebraic expression in the weak interaction limit. We also show that, in the full parameter regime comprising both the local and the non-local interaction, the region of enhanced TDOS for LL junction with "superconducting" boundary condition and that of "non-superconducting charge conserving" boundary condition (discussed in Phys. Rev. B 104, 045402 (2021)) are mutually exclusive. We show that this fact can be understood in terms of symmetry relation established between the superconducting and non-superconducting sectors of the theory. We compare the dependence of the proximity induced pair potential and TDOS as a function of distance $x$ from the junction. We demonstrate that the dependence of the spatial power law exponent for the `TDOS(x)/TDOS(x -> 0)' and the `pair-potential(x)/pair-potential(x -> 0)' are distinct function of the various local and non-local interaction parameters, which implies that the TDOS enhancement can not be directly attributed to the proximity induced pair potential in the LL.

Formation and structural characterization of two-dimensional wetting water layer on graphite (0001).

Understanding the structure and wettability of monolayer water is essential for revealing the mechanisms of nucleation, growth, and chemical reactivity at interfaces. We have investigated the wetting layer formation of water (ice) on the graphite (0001) surface using a combination of low-energy electron diffraction (LEED) and scanning tunneling microscopy (STM). At around monolayer coverages, the LEED pattern showed a (2 × 2) periodicity and STM revealed a hydrogen-bonded hexagonal network. The lattice constant was about 9% larger than that for ice Ih/Ic crystals, and the packing density was 0.096 Å-2. These results indicate that an extended ice network is formed on graphite, different from that on metal surfaces. Graphite is hydrophobic under ambient conditions due to the airborne contaminant but is considered inherently hydrophilic for a clean surface. In this study, the hydrophilic nature of the clean surface has been investigated from a molecular viewpoint. The formation of a well-ordered commensurate monolayer supports that the interaction of water with graphite is not negligible so that a commensurate wetting layer is formed at the weak substrate-molecule interaction limit.

The superconductivity of Sr2RuO4 under c-axis uniaxial stress

Applying in-plane uniaxial pressure to strongly correlated low-dimensional systems has been shown to tune the electronic structure dramatically. For example, the unconventional superconductor Sr2RuO4 can be tuned through a single Van Hove point, resulting in strong enhancement of both Tc and Hc2. Out-of-plane (c axis) uniaxial pressure is expected to tune the quasi-two-dimensional structure even more strongly, by pushing it towards two Van Hove points simultaneously. Here, we achieve a record uniaxial stress of 3.2 GPa along the c axis of Sr2RuO4. Hc2 increases, as expected for increasing density of states, but unexpectedly Tc falls. As a first attempt to explain this result, we present three-dimensional calculations in the weak interaction limit. We find that within the weak-coupling framework there is no single order parameter that can account for the contrasting effects of in-plane versus c-axis uniaxial stress, which makes this new result a strong constraint on theories of the superconductivity of Sr2RuO4.

Tunable transport in the mass-imbalanced Fermi-Hubbard model

The late-time dynamics of quantum many-body systems is organized in distinct dynamical universality classes, characterized by their conservation laws and thus by their emergent hydrodynamic transport. Here, we study transport in the one-dimensional Hubbard model with different masses of the two fermionic species. To this end, we develop a quantum Boltzmann approach valid in the limit of weak interactions. We explore the crossover from ballistic to diffusive transport, whose timescale strongly depends on the mass ratio of the two species. For timescales accessible with matrix product operators, we find excellent agreement between these numerically exact results and the quantum Boltzmann equation, even for intermediate interactions. We investigate two scenarios which have been recently studied with ultracold atom experiments. First, in the presence of a tilt, the quantum Boltzmann equation predicts that transport is significantly slowed down and becomes subdiffusive, consistent with previous studies. Second, we study transport probed by displacing a harmonic confinement potential and find good quantitative agreement with recent experimental data [N. Darkwah Oppong et al., arXiv:2011.12411]. Our results demonstrate that the quantum Boltzmann equation is a useful tool to study complex non-equilibrium states in inhomogeneous potentials, as often probed with synthetic quantum systems.

Cuts through the manifold of molecular H2O potential energy surfaces in liquid water at ambient conditions

The fluctuating hydrogen bridge bonded network of liquid water at ambient conditions entails a varied ensemble of the underlying constituting H2O molecular moieties. This is mirrored in a manifold of the H2O molecular potentials. Subnatural line width resonant inelastic X-ray scattering allowed us to quantify the manifold of molecular potential energy surfaces along the H2O symmetric normal mode and the local asymmetric O-H bond coordinate up to 1 and 1.5 Å, respectively. The comparison of the single H2O molecular potentials and spectroscopic signatures with the ambient conditions liquid phase H2O molecular potentials is done on various levels. In the gas phase, first principles, Morse potentials, and stepwise harmonic potential reconstruction have been employed and benchmarked. In the liquid phase the determination of the potential energy manifold along the local asymmetric O-H bond coordinate from resonant inelastic X-ray scattering via the bound state oxygen 1s to [Formula: see text] resonance is treated within these frameworks. The potential energy surface manifold along the symmetric stretch from resonant inelastic X-ray scattering via the oxygen 1s to [Formula: see text] resonance is based on stepwise harmonic reconstruction. We find in liquid water at ambient conditions H2O molecular potentials ranging from the weak interaction limit to strongly distorted potentials which are put into perspective to established parameters, i.e., intermolecular O-H, H-H, and O-O correlation lengths from neutron scattering.

Parametric instability of a vertically driven magnetic pendulum with eddy-current braking by a flat plate

The vertically driven pendulum is one of the classical systems where parametric instability occurs. We study its behavior with an additional electromagnetic interaction caused by eddy currents in a nearby thick conducting plate that are induced when the bob is a magnetic dipole. The known analytical expressions of the induced electromagnetic force and torque acting on the dipole are valid in the quasistatic limit, i.e., when magnetic diffusivity of the plate is sufficiently high to ensure an equilibrium between magnetic field advection and diffusion. The equation of motion of the vertically driven pendulum is derived assuming that its magnetic dipole moment is aligned with the axis of rotation and that the conducting plate is horizontal. The vertical position of the pendulum remains an equilibrium with the electromagnetic interaction. Conditions for instability of this equilibrium are derived analytically by the harmonic balance method for the subharmonic and harmonic resonances in the limit of weak electromagnetic interaction. The analytical stability boundaries agree with the results of numerical Floquet analysis for these conditions but differ substantially when the electromagnetic interaction is strong. The numerical analysis demonstrates that the area of harmonic instability can become doubly connected. Bifurcation diagrams obtained numerically show the co-existence of stable periodic orbits in such conditions. For moderately strong driving, chaotic motions can be maintained for the subharmonic instability.

Nonequilibrium master equationfor interacting Brownian particles in a deep-well periodic potential.

Employing a creation and annihilation operator formulation, we derive an approximate many-body master equationdescribing discrete hopping from the more general continuous description of Brownian motion on a deep-well nonequilibrium periodic potential. The many-body master equationdescribes interactions of arbitrary strength and range arising from a "top-hat" two-body interaction potential. We show that this master equationreduces to the well-known asymmetric simple exclusion process and the zero range process in certain regimes. We also use the creation and annihilation operator formalism to derive results for the steady-state drift and the number fluctuations in special cases, including the unexplored limit of weak interparticle interactions.

Tunable transport in the mass-imbalanced Fermi Hubbard model

The late-time dynamics of quantum many-body systems is organized in distinct dynamical universality classes, characterized by their conservation laws and thus by their emergent hydrodynamic transport. Here, we study transport in the one-dimensional Hubbard model with different masses of the two fermionic species. To this end, we develop a quantum Boltzmann approach valid in the limit of weak interactions. We explore the crossover from ballistic to diffusive transport, whose timescale strongly depends on the mass ratio of the two species. For timescales accessible with matrix product operators, we find excellent agreement between these numerically exact results and the quantum Boltzmann equation, even for intermediate interactions. We investigate two scenarios which have been recently studied with ultracold atom experiments. First, in the presence of a tilt, the quantum Boltzmann equation predicts that transport is significantly slowed down and becomes subdiffusive, consistent with previous studies. Second, we study transport probed by displacing a harmonic confinement potential and find good quantitative agreement with recent experimental data from [Oppong et al., arXiv:2011.12411]. Our results demonstrate that the quantum Boltzmann equation is a useful tool to study complex non-equilibrium states in inhomogeneous potentials, as often probed with synthetic quantum systems.

Nonadiabatic Exchange-Correlation Potential for Strongly Correlated Materials in the Weak and Strong Interaction Limits

In this work, nonadiabatic exchange-correlation (XC) potentials for time-dependent density-functional theory (TDDFT) for strongly correlated materials are derived in the limits of strong and weak correlations. After summarizing some essentials of the available dynamical mean-field theory (DMFT) XC potentials valid for these systems, we present details of the Sham–Schluter equation approach that we use to obtain, in principle, an exact XC potential from a many-body theory solution for the nonequilibrium electron self-energy. We derive the XC potentials for the one-band Hubbard model in the limits of weak and strong on-site Coulomb repulsion. To test the accuracy of the obtained potentials, we compare the TDDFT results obtained with these potentials with the corresponding nonequilibrium DMFT solution for the one-band Hubbard model and find that the agreement between the solutions is rather good. We also discuss possible directions to obtain a universal XC potential that would be appropriate for the case of intermediate interaction strengths, i.e., a nonadiabatic potential that can be used to perform TDDFT analysis of nonequilibrium phenomena, such as transport and other ultrafast properties of materials with any strength of electron correlation at any value in the applied perturbing field.