Light In Microcavities Research Articles

Ultra-low intensity light pulses for large cargo delivery into hard-to-transfect cells using an rGO mixed PDMS microtip device.

Nanoparticle-mediated photoporation has arisen as a universal intracellular delivery tool; however, the direct interaction of nanoparticles and cells hampers its clinical translation. Here, we report a uniform contactless intracellular delivery that transfects a large number of cells within a minute and avoids direct contact of nanoparticles and cells, thereby improving the cell viability. Our platform consists of an array of polydimethylsiloxane (PDMS) mixed reduced graphene oxide (rGO) nanoflakes on pyramidal microtips, uniformly distributed at the apex of the tip. The extraordinary optoelectronic properties of rGO were combined with micro-pyramidal cavities to entrap light in micro-cavities and efficiently convert it into heat through multiple reflections and absorptions. As a result, ultralow infra-red laser pulse irradiation could create cavitation bubbles followed by cell membrane deformation and biomolecular delivery. Using this delivery platform, we have achieved the delivery of small to large cargo (668 Da to 465 kDa) in various mammalian cells, including hard-to-transfect H9C2 cardiomyocytes. The best results were achieved for enzyme (465 kDa) delivery with a transfection efficiency and cell viability of 95% and 98%, respectively, in SiHa cells. The highly efficient cargo delivery tool demonstrated a safe and effective approach for cell therapy and diagnostics.

Directional planar antennae in polariton condensates

We report on the realization of all-optical planar microlensing for exciton–polariton condensates in semiconductor microcavities. We utilize spatial light modulators to structure a nonresonant pumping beam into a plano–concave lens-shape focused onto the microcavity plane. When pumped above condensation threshold, the system effectively becomes a directional polariton antenna, generating an intense focused beam of coherent polaritons away from the pump region. The effects of pump intensity, which regulates the interplay between gain and blueshift of polaritons, as well as the geometry of the lens-shaped pump are studied, and a strategy to optimize the focusing of the condensate is proposed. Our work underpins the feasibility to guide nonlinear light in microcavities using nonresonant excitation schemes, offering perspectives on optically reprogramable on-chip polariton circuitry.

Magneto-optical induced supermode switching in quantum fluids of light

The insensitivity of photons towards external magnetic fields forms one of the hardest barriers against efficient magneto-optical control, aiming at modulating the polarization state of light. However, there is even scarcer evidence of magneto-optical effects that can spatially modulate light. Here, we demonstrate the latter by exploiting strongly coupled states of semimagnetic matter and light in planar semiconductor microcavities. We nonresonantly excite two spatially adjacent exciton-polariton condensates which, through inherent ballistic near field coupling mechanism, spontaneously synchronise into a dissipative quantum fluidic supermode of definite parity. Applying a magnetic field along the optical axis, we continuously adjust the light-matter composition of the condensate exciton-polaritons, inducing a supermode switch into a higher order mode of opposite parity. Our findings set the ground towards magnetic spatial modulation of nonlinear light.

Magnetic strong coupling between rectangular hole metamaterials and Fabry–Pérot microcavity in THz region

Various studies have so far been conducted on the strong coupling interaction between light and matter in microcavities. Although most of them report on the coupling between the electric field and the electric dipole, the coupling between the magnetic field and the magnetic dipole is rarely reported. In this study, we investigated the strong coupling interaction between a magnetic field and a magnetic dipole using a Fabry–Pérot microcavity structure in the THz region consisting of wire grid (WG) mirrors and rectangular hole (RH) metamaterials. Here, the RH is well known as a magnetic current type slot antenna, which can be regarded as a magnetic dipole. To verify this concept, we analyzed the transmission properties of WG, RH, and a microcavity consisting of WG and RH (WGRH) using the transmission line theory. Consequently, we found that in this WGRH, normal mode splitting occurs, and anti-crossing behavior is observed in the dispersion relation. The samples were designed using the finite difference time-domain method and were fabricated via photolithography. We measured the transmission spectrum of the fabricated samples using THz time-domain spectroscopy. Finally, we observed a splitting of the transmission peak owing to mode coupling between the magnetic field and the magnetic dipole in WGRH.

Nonlocality-induced surface localization in Bose-Einstein condensates of light

The ability to create and manipulate strongly correlated quantum many-body states is of central importance to the study of collective phenomena in several condensed-matter systems. In the last decades, a great amount of work has been focused on ultracold atoms in optical lattices, which provide a flexible platform to simulate peculiar phases of matter both for fermionic and bosonic particles. The recent experimental demonstration of Bose-Einstein condensation (BEC) of light in dye-filled microcavities has opened the intriguing possibility to build photonic simulators of solid-state systems, with potential advantages over their atomic counterpart. A distinctive feature of photon BEC is the thermo-optical nature of the effective photon-photon interaction, which is intrinsically nonlocal and can thus induce interactions of arbitrary range. This offers the opportunity to systematically study the collective behaviour of many-body systems with tunable interaction range. In this paper, we theoretically study the effect of nonlocal interactions in photon BEC. We first present numerical results of BEC in a double-well potential, and then extend our analysis to a short one-dimensional lattice with open boundaries. By resorting to a numerical procedure inspired by the Newton-Raphson method, we simulate the time-independent Gross-Pitaevskii equation and provide evidence of surface localization induced by nonlocality, where the condensate density is localized at the boundaries of the potential. Our work paves the way towards the realization of synthetic matter with photons, where the interplay between long-range interactions and low dimensionality can lead to the emergence of unexplored nontrivial collective phenomena.

Realization of Exciton‐Mediated Optical Spin‐Orbit Interaction in Organic Microcrystalline Resonators

AbstractThe ability to control the spin‐orbit interaction (SOI) of light in optical microresonators is of fundamental importance for future photonics. Organic microcrystals, due to their giant optical anisotropy, play a crucial role in spin‐optics and topological photonics. Here, the controllable and wavelength‐dependent Rashba–Dresselhaus (RD) SOI is realized that is attributed to the anisotropic excitonic response in an optical microcavity filled with an organic microcrystalline. This work investigates the transition of the spin‐splitting from twice winding caused by the splitting of the transverse‐electric and transverse‐magnetic modes to once winding caused by the RD effect. The interplay of the two allows engineer the SOI of light in organic microcavities, which besides its fundamental interest promises applications in spin‐controlled on‐chip integrated nanophotonic elements, toward exploiting nonmagnetic and low‐cost spin‐photonic devices.

Bespoke mirror fabrication for quantum simulation with light in open-access microcavities.

In this work, we use focused ion beam (FIB) milling to generate custom mirror shapes for quantum simulation in optical microcavities. In the paraxial limit, light in multimode optical microcavities follows an equation of motion which is equivalent to Schrödinger's equation, with the surface topography of the mirrors playing the role of the potential energy landscape. FIB milling allows us to engineer a wide variety of trapping potentials for microcavity light, through exquisite control over the mirror topography, including 2D box, 1D waveguide, and Mexican hat potentials. The 2D box potentials are sufficiently flat over tens of microns, that the optical modes of the cavity, found by solving Schrödinger's equation on the measured cavity topography, are standing-wave modes of the box, rather than localised to deviations. The predicted scattering loss due to surface roughness measured using atomic force microscopy is found to be 177 parts per million, which corresponds to a cavity finesse of 2.2 × 104 once other losses have been taken into account. Spectra from dye-filled microcavities formed using these features show thermalised light in flat 2D potentials close to dye resonance, and spectrally-resolved cavity modes at the predicted frequencies for elliptical potentials. These results also represent a first step towards realising superfluid light and quantum simulation in arbitrary-shaped optical microcavities using FIB milling.

Spin-orbit interaction of light in three-dimensional microcavities

We investigate the spin-orbit coupling of light in three-dimensional cylindrical and tube-like whispering gallery mode resonators. We show that its origin is the transverse confinement of light in the resonator walls, even in the absence of inhomogeneities or anisotropies. The spin-orbit interaction results in elliptical far-field polarization (spin) states and causes spatial separation of polarization handedness in the far field. The ellipticity and spatial separation are enhanced for whispering gallery modes with higher excitation numbers along the resonator height. We analyze the asymmetry of the ellipticity and the tilt of the polarization orientation in the far field of cone-like microcavities. Furthermore, we find a direct relationship between the tilt of the polarization orientation in the far field and the local inclination of the resonator wall. Our findings are based on FDTD-simulations and are supported by three-dimensional diffraction theory.

Regular-Orbit-Engineered Chaotic Photon Transport in Mixed Phase Space.

The dynamical evolution of light in asymmetric microcavities is of primary interest for broadband optical coupling and enhanced light-matter interaction. Here, we propose and demonstrate that the chaos-assisted photon transport can be engineered by regular periodic orbits in the momentum-position phase space of an asymmetric microcavity. Remarkably, light at different initial states experiences different evolution pathways, following either regular-chaotic channels or pure chaotic channels. Experimentally, we develop a nanofiber technique to accurately control the excitation position of light in the phase space. We find that the coupling to high-Q whispering gallery modes depends strongly on excitation in islands or chaotic sea, showing a good agreement with the theoretical prediction. The engineered chaotic photon transport has potential in light manipulation, broadband photonic devices, and phase-space reconstruction.

Three-dimensional trapping of light with light in semiconductor planar microcavities

When light is confined in all three directions and in dimensions of the order of the light wavelength, full discretization of the photon spectra and distinctive phenomena occur, the Purcell effect and the inhibition of emission of atoms being two paradigmatic examples. Diverse solid-state devices that confine light in all three dimensions have been developed and applied. Typically the confinement volume, operating wavelength, and quality factor of these resonators are set by construction, and small variations of these characteristics with external perturbations are targeted for applications including light modulation and control. Here we describe full 3D light trapping, that is set and tuned by laser excitation in an all-optical scheme. The proposed device is based on a planar distributed Bragg reflector GaAs semiconductor microcavity operated at room temperature. Lateral confinement is generated with an attractive effective photonic potential tailored by the increase in the cavity spacer refractive index, induced by carriers photoexcited by a focused laser. Strong three dimensional trapping of light is evidenced by the laser-induced changes on the spectral, spatial, and k-space distribution of the emission. The dynamics of the laser induced photonic potential is studied using modulated optical excitation, highlighting the central role of thermal effects at the origin of the observed phenomena.

Theory for Bose-Einstein condensation of light in nanofabricated semiconductor microcavities

We construct a theory for Bose-Einstein condensation of light in nano-fabricated semiconductor microcavities. We model the semiconductor by one conduction and one valence band which consist of electrons and holes that interact via a Coulomb interaction. Moreover, we incorporate screening effects by using a contact interaction with the scattering length for a Yukawa potential and describe in this manner the crossover from exciton gas to electron-hole plasma as we increase the excitation level of the semiconductor. We then show that the dynamics of the light in the microcavities is damped due to the coupling to the semiconductor. Furthermore, we demonstrate that on the electron-hole plasma side of the crossover, which is relevant for the Bose-Einstein condensation of light, this damping can be described by a single dimensionless damping parameter that depends on the external pumping. Hereafter, we propose to probe the superfluidity of light in these nano-fabricated semiconductor microcavities by making use of the differences in the response in the normal or superfluid phase to a sudden rotation of the trap. In particular, we determine frequencies and damping of the scissors modes that are excited in this manner. Moreover, we show that a distinct signature of the dynamical Casimir effect can be observed in the density-density correlations of the excited light fluid.

Localized Surface Plasmons Selectively Coupled to Resonant Light in Tubular Microcavities.

Vertical gold nanogaps are created on microtubular cavities to explore the coupling between resonant light supported by the microcavities and surface plasmons localized at the nanogaps. Selective coupling of optical axial modes and localized surface plasmons critically depends on the exact location of the gold nanogap on the microcavities, which is conveniently achieved by rolling up specially designed thin dielectric films into three-dimensional microtube cavities. The coupling phenomenon is explained by a modified quasipotential model based on perturbation theory. Our work reveals the coupling of surface plasmon resonances localized at the nanoscale to optical resonances confined in microtubular cavities at the microscale, implying a promising strategy for the investigation of light-matter interactions.

Spin-orbit coupling of light in asymmetric microcavities.

When spinning particles, such as electrons and photons, undergo spin–orbit coupling, they can acquire an extra phase in addition to the well-known dynamical phase. This extra phase is called the geometric phase (also known as the Berry phase), which plays an important role in a startling variety of physical contexts such as in photonics, condensed matter, high-energy and space physics. The geometric phase was originally discussed for a cyclically evolving physical system with an Abelian evolution, and was later generalized to non-cyclic and non-Abelian cases, which are the most interesting fundamental subjects in this area and indicate promising applications in various fields. Here, we enable optical spin–orbit coupling in asymmetric microcavities and experimentally observe a non-cyclic optical geometric phase acquired in a non-Abelian evolution. Our work is relevant to fundamental studies and implies promising applications by manipulating photons in on-chip quantum devices.

Entangled light from driven dissipative microcavities

We study the generation of entangled light in planar semiconductor microcavities. The focus is on a particular pump configuration where the dissipative internal polariton dynamics leads to the emission of entangled light in a W-state. Our study is based on the nonlinear equations of motion for the polariton operators derived within the dynamics-controlled truncation formalism. They include the losses through the cavity mirrors, the interaction with lattice vibrations, and the external laser driving in a Langevin approach. We find that the generated entanglement is robust against decoherence under realistic experimental conditions. The results show that pair correlations in solid-state devices can be used to stabilize the nonlocal properties of the emitted radiation.

Polariton-generated intensity squeezing in semiconductor micropillars

The generation of squeezed and entangled light fields is a crucial ingredient for the implementation of quantum information protocols. In this context, semiconductor materials offer a strong potential for the implementation of on-chip devices operating at the quantum level. Here we demonstrate a novel source of continuous variable squeezed light in pillar-shaped semiconductor microcavities in the strong coupling regime. Degenerate polariton four-wave mixing is obtained by exciting the pillar at normal incidence. We observe a bistable behaviour and we demonstrate the generation of squeezing near the turning point of the bistability curve. The confined pillar geometry allows for a larger amount of squeezing than planar microcavities due to the discrete energy levels protected from excess noise. By analysing the noise of the emitted light, we obtain a measured intensity squeezing of 20.3%, inferred to be 35.8% after corrections.

Degenerate four-wave mixing in triply resonant Kerr cavities

We demonstrate theoretical conditions for highly-efficient degenerate four-wave mixing in triply-resonant nonlinear (Kerr) cavities. We employ a general and accurate temporal coupled-mode analysis in which the interaction of light in arbitrary microcavities is expressed in terms a set of coupling coefficients that we rigorously derive from the full Maxwell equations. Using the coupled-mode theory, we show that light consisting of an input signal of frequency $\omega_0-\Delta \omega$ can, in the presence of pump light at $\omega_0$, be converted with quantum-limited efficiency into an output shifted signal of frequency $\omega_0 + \Delta \omega$, and we derive expressions for the critical input powers at which this occurs. We find that critical powers in the order of 10mW assuming very conservative cavity parameters (modal volumes $\sim10$ cubic wavelengths and quality factors $\sim1000$. The standard Manley-Rowe efficiency limits are obtained from the solution of the classical coupled-mode equations, although we also derive them from simple photon-counting "quantum" arguments. Finally, using a linear stability analysis, we demonstrate that maximal conversion efficiency can be retained even in the presence of self- and cross-phase modulation effects that generally act to disrupt the resonance condition.

Photon properties of light in semiconductor microcavities

Properties of atom-like emitters in cavities are successfully described by cavity quantum electrodynamics (cavity-QED). In this work, we focus on the issue of the steady-state and spectral properties of the light emitted by a driven microcavity containing a quantum well (QW) with the excitonic interactions using simulation of fully quantum-mechanical treatment. The system is coherently pumped with laser, and it is found that depending on the relative values of pumping rate of stimulated emission, either one or two peaks close to the excitation energy of the QW or to the natural frequency of the cavity are shown in the emission spectrum. Furthermore, the nonclassical proprieties of the emitted photon have been investigated. This excitonic system presents several dynamical and statistical similarities to the atomic system, in particular for the bad-cavity and good-cavity limits. The results show that the photon emission can be significantly amplified due to the coupling strength between a single emitter and radiation field in the microcavity, and it is concluded that the present semiconductor microcavity system may serve as a QW laser with low threshold.

Low intensity directional switching of light in semiconductor microcavities

AbstractRecently it was demonstrated that in atomic vapors weak control beams can manipulate (or switch) the propagation direction of strong light beams [Dawes et al., Science 308, 672 (2005)]. As a semiconductor analog of such all‐optical switching, we present a proposal for similar manipulation and switching in planar semiconductor microcavities. Using a microscopic many‐particle theory, we investigate the spatio‐temporal dynamics of four‐wave mixing signals and related instabilities in these systems. Even though the underlying physical processes are different from atomic systems, we find that microcavities allow for reversible directional manipulation of light. (© 2009 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)

Harnessing optical forces in integrated photonic circuits

The force exerted by photons is of fundamental importance in light-matter interactions. For example, in free space, optical tweezers have been widely used to manipulate atoms and microscale dielectric particles. This optical force is expected to be greatly enhanced in integrated photonic circuits in which light is highly concentrated at the nanoscale. Harnessing the optical force on a semiconductor chip will allow solid state devices, such as electromechanical systems, to operate under new physical principles. Indeed, recent experiments have elucidated the radiation forces of light in high-finesse optical microcavities, but the large footprint of these devices ultimately prevents scaling down to nanoscale dimensions. Recent theoretical work has predicted that a transverse optical force can be generated and used directly for electromechanical actuation without the need for a high-finesse cavity. However, on-chip exploitation of this force has been a significant challenge, primarily owing to the lack of efficient nanoscale mechanical transducers in the photonics domain. Here we report the direct detection and exploitation of transverse optical forces in an integrated silicon photonic circuit through an embedded nanomechanical resonator. The nanomechanical device, a free-standing waveguide, is driven by the optical force and read out through evanescent coupling of the guided light to the dielectric substrate. This new optical force enables all-optical operation of nanomechanical systems on a CMOS (complementary metal-oxide-semiconductor)-compatible platform, with substantial bandwidth and design flexibility compared to conventional electrical-based schemes.

Photon statistics of light in semiconductor microcavities

We investigate the photon statistics in the light emitted by a microcavity containing a semiconductor quantum well. An analytical expression of the light-emitted autocorrelation function in the weak pumping regime is derived. We discuss photon statistical similarities with an atomic cavity.