Laser-target Interaction Research Articles

A hybrid simulation integrating molecular dynamics and particle-in-cell methods for improved laser-target interaction

Ultra-thin targets (less than 10 nm), such as graphene, can be irradiated with relativistic intensity lasers to generate energetic ions. However, the laser prepulse can prematurely destroy these targets and significantly influence the final ion energies. Due to the limitations of the conventional hydrodynamic model, simulating the interaction between ultra-thin targets and a prepulse is infeasible. To overcome this issue, we propose a hybrid simulation technique in this study. This technique involves simulating the target-prepulse interaction using molecular dynamics (MD) simulation, which is then combined with the particle-in-cell simulation for the target-main pulse interaction, in order to accurately model the entire laser-target interaction dynamics. A realistic, experimentally measured laser intensity profile for the prepulse is used for the MD simulation, and the particle energies from this hybrid simulation are found to be in good agreement with the experiment.

Toward machine-learning-assisted PW-class high-repetition-rate experiments with solid targets

We present progress in utilizing a machine learning (ML) assisted optimization framework to study the trends in a parameter space defined by spectrally shaped, high-intensity, petawatt-class (8 J, 45 fs) laser pulses interacting with solid targets and give the first simulation-based overview of predicted trends. A neural network (NN) incorporating uncertainty quantification is trained to predict the number of hot electrons generated by the laser–target interaction as a function of pulse shaping parameters. The predictions of this NN serve as the basis function for a Bayesian optimization framework to navigate this space. For post-experimental evaluation, we compare two separate neural network (NN) models. One is based solely on data from experiments, and the other is trained only on ensemble particle-in-cell simulations. Reviewing the predicted and observed trends across the experiment-capable laser parameter search space, we find that both ML models predict a maximal increase in hot electron generation at a level of approximately 12%–18%; however, no statistically significant enhancement was observed in experiments. On direct comparison of the NN models, the average discrepancy is 8.5%, with a maximum of 30%. Since shot-to-shot fluctuations in experiments affect the observations, we evaluate the behavior of our optimization framework by performing virtual experiments that vary the number of repeated observations and the noise levels. Here, we discuss the implications of such a framework for future autonomous exploration platforms in high-repetition-rate experiments.

Proton spectroscopy for 11B(p,α)2α fusion reaction with RCF films: calibration and unfolding procedure

The reaction occurring between protons and 11B isotope (p+11B → 3α+8.7 MeV) has recently attracted attention as a possible candidate to overcome the generation of high-energy neutrons via the more studied Deuterium-Tritium fusion reaction. Since the early 2000s, several experiments have been carried out to investigate the viability of triggering this aneutronic reaction in laser-target interaction schemes. During these experiments, the total number of escaping α particles is measured to infer fusion reaction efficiency. However, the accurate detection of α particles in such experiments poses a real challenge.In this scenario, RadioChromic Films(RCFs) arranged in a stack configuration can be used for the fluence and energy spectra reconstruction of generated protons, being this mandatory information in both “pitcher-catcher” and “in plasma” p-11B irradiation schemes. Nevertheless, RCF response exhibits a dependence on Linear Energy Transfer (LET), which leads to an underestimation of the response in high-LET conditions. This can result in dosimetric errors if not properly taken into account.In this work, an analytical procedure able to reconstruct the incident energy spectra in an RCF stack was developed and validated thanks to a calibration procedure that was established for high and low proton energy (4–60 MeV) beams to properly reconstruct the incident spectra in the “pitcher-catcher” irradiation scheme.

Enhanced positron acceleration driven by femto-second laser pulses irradiating structured targets

We have proposed a compact scheme for generating high-density and high-energy positrons by irradiating different shaped targets with an ultra-intense laser pulse, using 2D particle-in-cell simulations and numerical analysis. Our simulations show that the Breit–Wheeler process dominates positron production during laser-target interaction when a laser with an intensity of 4×1023 Wcm−2 is used. We obtain a positron beam with an energy of 2.5 GeV and a total number exceeding 109, which is an improvement by two orders of magnitude compared to previous work with the same laser intensity. By using different shaped targets, we are able to generate a high-energy positron beam with low divergence. The yield of positron pairs depends on both the target and the laser parameters, and we have investigated how the shape of the target can enhance pair production and reduce divergence. Both of our analytical and simulation results demonstrate that this high-flux and low-divergence positron beam has direct applications in the field of medical and astro-physics that can be explored in the upcoming high intensity laser facilities.

Probing the peripheral self-generated magnetic field distribution in laser-plasma magnetic reconnection with Martin–Puplett interferometer polarimeter

Magnetic reconnection of the self-generated magnetic fields in laser-plasma interaction is an important laboratory method for modeling high-energy density astronomical and astrophysical phenomena. We use the Martin–Puplett interferometer (MPI) polarimeter to probe the peripheral magnetic fields generated in the common magnetic reconnection configuration, two separated coplanar plane targets, in laser-target interaction. We introduce a new method that can obtain polarization information from the interference pattern instead of the sinusoidal function fitting of the intensity. A bidirectional magnetic field is observed from the side view, which is consistent with the magneto-hydro-dynamical (MHD) simulation results of self-generated magnetic field reconnection. We find that the cancellation of reverse magnetic fields after averaging and integration along the observing direction could reduce the magnetic field strength by one to two orders of magnitude. It indicates that imaging resolution can significantly affect the accuracy of measured magnetic field strength.

Spatial and temporal evolution of electromagnetic pulses from solid target irradiated with multi-hundred-terawatt laser pulse inside target chamber

Giant electromagnetic pulses (EMPs) induced by high-power laser irradiating solid targets interfere with various experimental diagnoses and even damage equipment, so unveiling the evolution of EMPs inside the laser chamber is crucial for designing effective EMP shielding. In this work, the transmission characteristics of EMPs as a function of distances from the target chamber center (TCC) are studied using B-dot probes. The mean EMP amplitude generated by picosecond laser-target interaction reaches 561 kV m−1, 357 kV m−1, 395 kV m−1, and 341 kV m−1 at 0.32 m, 0.53 m, 0.76 m, and 1 m from TCC, which decreases dramatically from 0.32 m to 0.53 m. However, it shows a fluctuation from 0.53 m to 1 m. The temporal features of EMPs indicate that time-domain EMP signals near the target chamber wall have a wider full width at half maximum compared to that close to TCC, mainly due to the echo oscillation of electromagnetic waves inside the target chamber based on simulation and experimentation. The conclusions of this study will provide a new approach to mitigate strong electromagnetic pulses by decreasing the echo oscillation of electromagnetic waves inside the target chamber during laser coupling with targets.

Ultrahigh-energy density state in nanowire arrays irradiated with picosecond kilojoule-class ultra-intense laser

Ultrahigh-energy density (UHED) states greater than 1 Gbar pressure are typically observed under extreme conditions, such as in the core of an inertial confinement fusion implosion. A novel alternative approach for generating volumetric UHED states is to use nanowire arrays irradiated with a femtosecond ultrahigh-intensity laser. In this paper, we present an experimental investigation on laser absorption and energy transport in nanowire arrays irradiated with a picosecond kilojoule petawatt laser. The laser–target interactions were studied by measuring the x-ray emission and escaping hot electrons from a bare Cu foil and a foil with a nanowire array grown on its surface. The measured Cu-Kα and He-α emissions from the nanowire array were higher than those from the flat foil. In addition, hot electrons observed from the front surface of the nanowire array were enhanced. On the other hand, despite the stronger Kα emission from the nanowire array and the enhancement of hot electrons escaping from the front surface of the nanowire array, the number of hot electrons observed from the rear side of the flat foil target was slightly lower than that of the flat foil. A comparison of the experimental results with the results of a two-dimensional particle-in-cell simulation code suggested that the magnetic fields generated around the periodic nanowire array trap hot electrons, improving the electron-to-target energy coupling and efficiently producing UHED states.

Modeling of electron refluxing and TNSA fields in laser–target interactions based on analysis of K α emission

We analyze and model fast-electron-induced Kα emission from an experiment in which a high-intensity ultra-short laser irradiated foil and bulk titanium targets. The motion of electrons inside the targets is calculated allowing for multiple scattering and collisional energy loss, while outside the target, electric fields of arbitrary configurations are assumed. It is shown that both the radial Kα-intensity distributions and the somewhat non-intuitive dependence of the absolute Kα emission on the target thickness can be reproduced by taking into account the fast-electron refluxing with an electric field configuration based on the target normal sheath acceleration model. We infer the presence of a sheath electric field on the order of TV/m, extending to about 100μm in the radial direction. In addition, we obtain a temporal profile of the Kα radiation.

Combined Spectroscopy System Utilizing Gas Electron Multiplier and Timepix3 Technology for Laser Plasma Experiments

We present an innovative X-ray spectroscopy system to address the complex study of the X-ray emissions arising from laser–target interactions, where the emissions occur within extremely brief intervals from femtoseconds to nanoseconds. Our system combines a Gas Electron Multiplier (GEM) detector with a silicon-based Timepix3 (TPX3) detector. These detectors work in tandem, allowing for a spectroscopic radiation analysis along the same line of sight. With an active area of 10 × 10 cm2, the GEM detector allows for 1D measurements for X-ray energies (2–50 keV) by utilizing the full 10 cm gas depth. The high-energy part of the radiation beam exits through a downstream side window of the GEM without being absorbed in the gas volume. Positioned side-on at the GEM detector’s exit, the TPX3 detector, equipped with a pixelated sensor (55 µm × 55 µm; active area 14 mm × 14 mm), uses its full 14 mm silicon sensor to detect hard X-rays (50–500 keV) and gamma rays (0.5–10 MeV). We demonstrate the correct operation of the entire detection system and provide a detailed description of the Timepix3 detector’s calibration procedure, highlighting the suitability of the combined system to work in laser plasma facilities.

Proof-of-Principle of Absolute Dosimetry Using an Absorbed Dose Portable Calorimeter with Laser-Driven Proton Beams

Charged particle beams driven to ultra-high dose rates (UHDRs) have been shown to offer potential benefits for future clinical applications, particularly in the reduction of normal-tissue toxicity. Studies of the so-called FLASH effect have shown promise, generating huge interest in high dose rate radiation studies. With laser-driven proton beams, where the duration of the proton burst delivered to a sample can be as short as hundreds of picoseconds, the instantaneous dose rates are several orders of magnitude higher than those used for conventional radiotherapy. The dosimetry of these beam modalities is not trivial, with conventional active detectors, such as ionisation chambers, experiencing saturation effects making them unusable at the extremely high dose rates. Calorimeters, measuring the radiation-induced temperature rise in an absorber, offer an ideal candidate for the dosimetry of UHDR beams. However, their application in the measurement of laser-driven UHDR beams has so far not been trialled, and their effective suitability to work with the quasi-instantaneous and inhomogeneous dose deposition patterns and the harsh environment of a laser-plasma experiment has not been tested. The measurement of the absorbed dose of laser-driven proton beams was conducted in a first-of-its-kind investigation, employing the VULCAN-PW laser system of the Central Laser Facility (CLF) at the Rutherford Appleton Laboratory (RAL), using a small-body portable graphite calorimeter (SPGC) developed at the National Physical Laboratory (NPL) and radiochromic films. A small number of shots were recorded, with the corresponding absorbed dose measurements resulting from the induced temperature rise. The effect of the electromagnetic pulse (EMP) generated during laser–target interaction was assessed on the system, showing no significant effects on the derived signal-to-noise ratio. These proof-of-principle tests highlight the ability of calorimetry techniques to measure the absorbed dose for laser-driven proton beams.

Influence of ambient pressure and laser energy on the plasma dynamics and parameters of laser-irradiated polyvinyl chloride

The dependence of propulsion performance generated by laser ablation of polyvinyl chloride on laser energy and pressure is investigated using Q-switched Nd: YAG laser with the wavelength of 1064 nm. When the pressure is decreased, the impulse and coupling coefficient rise first and then decline. Such a trend is also reflected in the variation of coupling coefficient with laser energy in the whole pressure range. However, the change in impulse with laser energy at atmospheric pressure is not completely consistent with that at low pressure levels. The dynamic behavior and duration of plasma plume are considered to be the factors for the difference in propulsion performance. By capturing the fast exposure images of plume, the separation at atmospheric pressure and severe expansion accompanied by rapid quenching in near vacuum are observed. Moreover, the plasma plume lasts longer time at high pressures. It is ascribed to the higher electron temperature, which promotes background gas to excite and ionize. Since the electron density increases with the improvement of laser energy and pressure, the absorption of electrons to laser energy becomes stronger through the inverse bremsstrahlung mechanism. Accordingly, the shielding effect of plasma is enhanced, causing the weak laser-target interaction. The result is that the crater depth and ablative mass increase with decreasing pressure. This work is important for understanding the energy conversion mechanism and optimizing the laser propulsion performance.

Absolute calibration up to 20 MeV of an online readout CMOS system suitable to detect high-power lasers accelerated protons

We present the design and absolute calibration of a charged particle online readout CMOS system tailored for high-power laser experiments. This system equips a Thomson parabola spectrometer, which is used at the Apollon petawatt scale laser facility to measure the spectra of protons produced by high-intensity laser–target interactions. The RadEye1 CMOS matrices array detectors are paired with a custom triggering system for image grabbing. This allows us to register the proton and ion signals remotely. The repetition rate is presently 1 shot/min, but the frame grabbing enables the system to be compatible with modern high-power lasers running, e.g., at 1 Hz. We detail here the implementation, in the harsh electromagnetic environment of such interactions, of the system, and its absolute calibration, which was performed for proton energies from 4 to 20 MeV.

Plasma polymers as targets for laser-driven proton-boron fusion

Laser-driven proton-boron (pB) fusion has been gaining significant interest for energetic alpha particles production because of its neutron-less nature. This approach requires the use of B- and H-rich materials as targets, and common practice is the use of BN and conventional polymers. In this work, we chose plasma-assisted vapour phase deposition to prepare films of oligoethylenes (plasma polymers) on Boron Nitride BN substrates as an advanced alternative. The r.f. power delivered to the plasma was varied between 0 and 50 W to produce coatings with different crosslink density and hydrogen content, while maintaining the constant thickness of 1 μm. The chemical composition, including the hydrogen concentration, was investigated using XPS and RBS/ERDA, whereas the surface topography was analyzed using SEM and AFM. We triggered the pB nuclear fusion reaction focusing laser pulses from two different systems (i.e., the TARANIS multi-TW laser at the Queen’s University Belfast (United Kingdom) and the PERLA B 10-GW laser system at the HiLASE center in Prague (Czech Republic)) directly onto these targets. We achieved a yield up to 108 and 104 alpha particles/sr using the TARANIS and PERLA B lasers, respectively. Radiative-hydrodynamic and particle-in-cell PIC simulations were performed to understand the laser-target interaction and retrieve the energy spectra of the protons. The nuclear collisional algorithm implemented in the WarpX PIC code was used to identify the region where pB fusion occurs. Taken together, the results suggest a complex relationship between the hydrogen content, target morphology, and structure of the plasma polymer, which play a crucial role in laser absorption, target expansion, proton acceleration and ultimately nuclear fusion reactions in the plasma.

Observation of proton modulations in laser–solid interaction

We report on an experimental investigation into proton acceleration from the interaction of an intense laser pulse, with an intensity of about 1020 W cm−2, with a thin foil of aluminum, titanium and gold of thickness 2 µm. Protons are accelerated via the TNSA mechanism from the rear surface of the target and, in addition, protons accelerated from the front surface are also detected on the radio chromic films. Hollow proton rings could be seen on the radio chromic films, corresponding to 1–3 MeV protons. The protons from the front surface are driven into the target and directed towards the rear side of the target by the Kilotesla magnetic fields generated from the laser plasma. 2D particle-in-cell simulations predict an increase in the flux of lower energy protons similar to experimental observations and also show strong magnetic field structures in the laser–target interaction region.

Numerical simulation and investigation of ultra-short pulse laser ablation on Ti6Al4V and stainless steel

In ultra-short pulse laser machining and micro/surface processing, accurate simulation of laser ablation is important for understanding laser-target interaction and improving ablation performance, but it remains challenging. This work aims to develop a numerical model to improve the accuracy of the ablation depth calculation. A grid deformation scheme is proposed based on energy conservation and considering contributions to instant material removal from both the electron and lattice subsystems. By incorporating this scheme with the two-temperature model (TTM), a reasonable prediction of the instant target surface profile during laser ablation has been achieved. In the case of single-pulse femtosecond laser ablation of Ti6Al4V, the calculated ablation depth ranges from 0.06 to 0.56 μm for laser energy from 1.0 to 10.0 μJ. For single-pulse picosecond laser ablation of stainless steel, as laser energy increases from 6.0 to 18.5 μJ, the predicted ablation crater deepens accordingly from 40 to 87 nm. In addition, for multi-pulse picosecond laser ablation of stainless steel, a linear dependence of the ablation depth on the pulse number is observed up to a depth of about 803 nm at 6.0 μJ and 20 pulses. In all the above-mentioned cases, the calculation results are in better agreement with experimental measurements than conventional TTM or other material removal schemes, validating the accuracy of the proposed model.

Design and optimization of a high-energy optical parametric amplifier for broadband, spectrally incoherent pulses.

Spectrally incoherent laser pulses with sufficiently large fractional bandwidth are in demand for the mitigation of laser-plasma instabilities occurring in high-energy laser-target interactions. Here, we modeled, implemented, and optimized a dual-stage high-energy optical parametric amplifier for broadband, spectrally incoherent pulses in the near-infrared. The amplifier delivers close to 400 mJ of signal energy through noncollinear parametric interaction of 100-nJ-scale broadband, spectrally incoherent seed pulses near 1053 nm with a narrowband high-energy pump operating at 526.5 nm. Mitigation strategies for high-frequency spatial modulations in the amplified signal caused by index inhomogeneities in the Nd:YLF rods of the pump laser are explored and discussed in detail.

Radiation Protection at Petawatt Laser-Driven Accelerator Facilities: The ELI Beamlines Case

ELI Beamlines is a newly constructed petawatt (PW) laser-based accelerator facility. Its flagship laser has a nominal peak power of 10 PW with a pulse duration of 150 fs. The radiation fields emerging from the laser-target interactions will be pulsed and made of mixed particles of high intensity and energy, thus posing new and daunting challenges compared to conventional radiation protection. The civil engineering constraints of a laser facility bring localized weaknesses to the shielding structures. The ultrashort pulses in conjunction with ultrahigh dose rates strain the capabilities of the commercially available radiation detectors. The complexity of modeling laser-target interactions and the resulting ionizing radiation complicates the radiation protection calculations. This paper is a review of the radiation protection challenges at ELI Beamlines, the adopted solutions, and the practices to minimize the harmful effects of ionizing radiation linked to its activities. Some of the presented solutions may have universal validity, while others are specific to this site and can only serve as an inspiration.

Strongly magnetized plasma produced by interaction of nanosecond kJ-class laser with snail targets

Magnetized plasma studies are necessary for many applied studies, including laser-driven inertial fusion, modeling astrophysically relevant phenomena, and innovative industrial and medical applications. An interesting method of generating highly magnetized plasma can be based on the interaction of a laser with spiral-shaped cavity (snail-like) targets. A target shaped in this way can represent the central area of a spherical pellet that is not irradiated radially, but rather through an entrance hole allowing the laser beam to almost impact its inner surface tangentially (Pisarczyk et al 2018 Sci. Rep. 8 17 895). In the reported experiment, snail targets of various diameters were irradiated by linearly or circularly polarized radiation of a Prague asterix laser system (PALS) iodine laser delivering ∼500 J, 350 ps and 1.315 μm pulses on targets. Three-frame complex interferometry demonstrated that plasma is generated on the entire inside and outside surfaces of the snail target, starting from the very beginning of the laser–target interaction. The time-resolved records of the magnetic field and the electron density distribution inside and outside the snail target characterize the changes in the structure of the magnetized plasma. Inside the target, the magnetic field survives long after the termination of the laser–matter interaction, namely longer than 10 ns. Compared to a circularly polarized laser pulse, the irradiation of targets with a p-polarized beam increases both the emission of hot electrons (HEs) and the intensity of the magnetic field. The emission of HEs is not isotropic, and their energy distribution cannot be characterized by a single temperature.

Dynamic simulation on laser-metal interaction in laser ablation propulsion considering moving interface, finite thermal wave transfer, and phase explosion

Despite extensive investigations on the mechanism of laser-irradiated solid propellants, formulating an accurate model that characterizes more details of laser-target interactions remains a challenging task. In this paper, a thermal model for nanosecond pulsed laser ablation of aluminum was developed using the finite volume method which considers the instant recession on the propellant surface and the non-Fourier effect during heat conduction. The robust coupling iteration scheme adopted in the model tracks the dynamic boundary condition due to instant propellant removal. In particular, the pre-qualified threshold is used as discriminator for phase explosion and the thermal relaxation time is introduced to quantify the non-Fourier effect on heat conduction. In addition, the temperature-dependent physical and optical parameters of the propellant were also regarded in the proposed model. The numerical implementations for Gaussian laser ablation of aluminum were performed at different laser fluences and thermal relaxation times. The theoretical computation of the ablation depth coincides well with the experimental results to validate the feasibility of the model.

Spectral-temporal measurement capabilities of third-order correlators.

We present a method extending scanning third-order correlator temporal pulse evolution measurement capabilities of high power short pulse lasers to spectral sensitivity within the spectral range exploited by typical chirped pulse amplification systems. Modelling of the spectral response achieved by angle tuning of the third harmonic generating crystal is applied and experimentally validated. Exemplary measurements of spectrally resolved pulse contrast of a Petawatt laser frontend illustrate the importance of full bandwidth coverage for the interpretation of relativistic laser target interaction in particular for the case of solid targets.