Intense Laser Beam Research Articles

Control of Coherent Light through Microperiodic Director Modulation in Nematic Films under Low-Voltage DC Electric Field.

This work addresses the achievement of efficient control of laser light transmission through stationary microperiodic parallel stripe textures formed in films of nematic liquid crystals (NLCs) in planar-oriented cells upon a direct-current (DC) electric field. By varying the field intensity and, thereby, the field-induced periodic modulation of the nematic director and hence the complex transmittance function corresponding to the longitudinal domain texture induced in NLC films with initial planar alignment, the intensity of a linearly polarized laser beam passed through the films can be well controlled. In 25 µm-thick films of room-temperature NLCs pentylcyanobiphenyl (5CB), this results in a low-voltage (~4 V) sharp and deep V-shaped behavior of their electro-optically controlled transmittance. Such a reversible electro-optical effect is interesting for active control of laser beam intensity and other applications. The relevant physical mechanism is analyzed and explained.

Probability of High Intensities of the Light Wave Propagating in a Turbulent Atmosphere

We examine statistics of fluctuations of the laser beam intensity at its propagating in turbulent atmosphere. We are interested in relatively large propagating distances and the remote tail of the probability density function. The tail is determined by the stretched exponent, we find its index.

Design and Construction of a Variable-Angle Three-Beam Stimulated Resonant Photon Collider toward eV-Scale ALP Search

We aim to search for axion-like particles in the eV mass range using a variable-angle stimulated resonance photon collider (SRPC) with three intense laser beams. By changing angle of incidence of the three beams, the center-of-mass-system collision energy can be varied and the eV mass range can be continuously searched for. In this paper, we present the design and construction of such a variable-angle three-beam SRPC (tSRPC), the verification of the variable-angle mechanism using a calibration laser, and realistic sensitivity projections for searches in the near future.

Nonlinear optical effects in natural topaz

We investigate the nonlinear optical properties of natural topaz. For the first time, the observation of nonlinear phenomena related to multiphoton absorption effects, such as the up-conversion luminescence of the material defects, is reported in natural gems. In particular, we were able to detect the presence of the AlO4-related defects which are responsible for the change of the color of topaz as a consequence of irradiation with γ-rays as well as electrons and neutrons beams. Besides, the nonlinear spectral broadening of intense laser beams permits to spot of the presence of rare earth elements, such as Ytterbium and Neodymium, which are not found by means of standard characterization techniques of natural gems, e.g., those based on X-ray fluorescence, electron paramagnetic resonance, and linear optical fluorescence and absorbance measurements. In this sense, our results demonstrate that nonlinear optical effects induced luminescence measurements are a complementary, and previously unforeseen, technique for the characterization of the optical and physicochemical properties of natural gems. Finally, using intense infrared laser pulses allowed us to trigger extreme nonlinear effects, such as multiphoton ionization and conical emission. Our results will be of interest for the investigation of novel nonlinear optical effects in materials that are transparent in the whole visible spectral range and may give insights into the development of materials for nonlinear photonics.

Direct Femtosecond Laser Processing for Generating High Spatial Frequency LIPSS (HSFL) on Borosilicate Glasses with Large-Area Coverage

Large-area nanostructuring of glasses using intense laser beams is a challenging task due to the material’s extreme non-linear absorption of laser energy. Precise optimization of the process parameters is essential for fabricating nanostructures with large-area coverage. In this study, we report the findings on creating high-spatial-frequency LIPSS (HSFL) on borosilicate glass through direct laser writing, using a femtosecond laser with a wavelength λ = 800 nm, pulse duration τ = 35 fs, and repetition frequency frep = 1 kHz. We measured the single-pulse ablation threshold and incubation factor of Borosilicate glasses to achieve high-precision control of the large-area surface structuring. Single-spot experiments indicated that, when there was higher fluence and a larger number of irradiated laser pulses, a melt formation inside the irradiated area limited the uniformity of LIPSS formation. Additionally, the orientation of the scan axis with the laser beam polarization was found to significantly influence the uniformity of LIPSS generated along the scan line, with more redeposition and melt formation when the scan axis was perpendicular to the laser beam polarization. For large-area processing, the borosilicate glass surface was scanned line-by-line by the laser beam, with a scan orientation parallel to the polarization of the laser. The optical characterization revealed that the transmittance and reflectance of the borosilicate glass decreased significantly after processing. Additionally, the surface’s wettability changed from hydrophilic to super-hydrophilic after processing. These chemical contamination-free and uniformly distributed structures have potential applications in optics, microfluidics, photovoltaics, and biomaterials.

Fabrication of Surface Acoustic wave resonator as Acousto-optic Modulator

Acousto-optic modulation techniques are gaining edge in diverse applications in the area of agriculture, entertainment and defense. Present work focuses on indigenously developed pump probe technique to study the acousto-optic modulation using surface acoustic wave (SAW) device. For this study, SAW device has been fabricated on ST-cut quartz that is an optically nonlinear piezoelectric material. Coupling of acoustic wave with optical wave has been monitored and a visible modulation in the intensity of probe laser beam has been obtained. A clear shift in the value of probe intensity (∼12 μW) is observed when surface acoustic waves are excited. Angular rotation of the fabricated SAW device under pump probe microscopy shows the periodicity of the nonlinearity in substrate while acoustic wave is propagating in it. The effect of variation in the intensity of pump laser beam on the acousto-optic modulation is also studied. The acousto-optic modulation behavior observed in surface acoustic devices in the present study demonstrates the possible application in telecommunication for signal modulation and in spectroscopy for frequency control.

Dynamics of Nanosecond Laser Pulse Propagation and of Associated Instabilities in a Magnetized Underdense Plasma.

The propagation and energy coupling of intense laser beams in plasmas are critical issues in inertial confinement fusion. Applying magnetic fields to such a setup has been shown to enhance fuel confinement and heating. Here we report on experimental measurements demonstrating improved transmission and increased smoothing of a high-power laser beam propagating in a magnetized underdense plasma. We also measure enhanced backscattering, which our kinetic simulations show is due to magnetic confinement of hot electrons, thus leading to reduced target preheating.

Laser intensity and surface distribution identification at weld interface during laser transmission welding of thermoplastic polymers: A combined numerical inverse method and experimental temperature measurement approach

AbstractThe determination of the laser intensity profile necessary to weld two thermoplastic parts is crucial for understanding and optimizing the laser welding process in polymers and composite materials. Traditional methods of measuring the laser beam intensity profile, such as laser beam profiling techniques, can be difficult to implement and expensive. In this paper, we present the development of a technique that combines a numerical inverse method with experimental temperature measurements to determinate the laser intensity distribution at the weld interface. This technique does not require specialized or expensive equipment and accounts for variations in laser beam intensity caused by different components and interfaces. The technique uses thermocouple sensors to measure interface temperatures during welding, and an analytical gaussian model to estimate the laser intensity distribution at the weld interface. The model is then used as input data in a numerical heat transfer model. The technique is validated through experimental investigations on transparent and absorbent Polylactic acid polymers.

Four-dimensional dynamics of multirotational transition stimulated rotational Raman scattering in air

Stimulated rotational Raman scattering in air is a powerful parasitic process that degrades high intensity laser beams and pulses propagated over significant distances. Conversely, it is used beneficially in the context of Raman lasers. Through this inelastic scattering process, laser photons are converted to higher (anti-Stokes) or lower (Stokes) energies, according to rotational mode transitions in nitrogen and oxygen diatomic molecules. The full wave-mixing problem involves numerous frequencies, and it is consistently assumed that only one rotational mode contributes to the conversion process. We instead present a dynamic 4D multirotational model that is implemented in a parallelized manner within the Virtual Beamline++ optical modeling package allowing high-resolution 4D studies. We highlight the effect that spontaneous emission plays in large and small beam-width setups, even in the highly saturating regime. The weaker transition modes play a large role in the persistent dynamics and can lead to complex spatiotemporal coupling through nonlinear competition of the modes. We highlight how and why these weaker modes persist, how the size and shape of speckle patterns depends highly on the initial beam profile, and how weaker modes can transiently become stronger as a result of such competition.

Excitation gratings in cross-beam filament wake channels in a dense argon gas: Formation, control, and Rabi sideband manifestation.

When two intense laser beams cross at a small angle, the interference in the crossing area results in a finite intensity grating. We consider femtosecond laser filamentation in such a grating, in a situation when the process is largely confined to the grating maxima and leads to formation of a structured filament wake channel. In a dense gas, electron impact processes during the laser pulse cause a copious excitation of neutral atoms, resulting in formation of a finite grating of the density of excited atoms. Numerically solving the equations of laser-driven kinetics, we obtain the properties of this grating, as depending on the characteristics of the interfering beams and especially on the interbeam phase delay. The excitation gratings thus formed give rise to a hallmark effect of Rabi sideband emission when probed by a picosecond 800 nm laser pulse, which couples with transitions in the excited states manifold. Spectral and spatial interference of the emitted radiation forms four-dimensional spatial-spectral fringe patterns accessible for observation on a remote screen. The patterns are indicative of the excitation grating structure; their sensitivity to the phase delay between the crossing pump pulses warrants experimental verification.

Shifting physics of vortex particles to higher energies via quantum entanglement

Physics of structured waves is currently limited to relatively small particle energies as the available generation techniques are only applicable to the soft X-ray twisted photons, to the beams of electron microscopes, to cold neutrons, or non-relativistic atoms. The highly energetic vortex particles with an orbital angular momentum would come in handy for a number of experiments in atomic physics, nuclear, hadronic, and accelerator physics, and to generate them one needs to develop alternative methods, applicable for ultrarelativistic energies and for composite particles. Here, we show that the vortex states of in principle arbitrary particles can be generated during photon emission in helical undulators, via Cherenkov radiation, in collisions of charged particles with intense laser beams, in such scattering or annihilation processes as emu rightarrow emu , ep rightarrow ep, e^-e^+ rightarrow pbar{p}, and so forth. The key element in obtaining them is the postselection protocol due to entanglement between a pair of final particles and it is largely not the process itself. The state of a final particle – be it a gamma -ray, a hadron, a nucleus, or an ion – becomes twisted if the azimuthal angle of the other particle momentum is measured with a large error or is not measured at all. As a result, requirements to the beam transverse coherence can be greatly relaxed, which enables the generation of highly energetic vortex beams at accelerators and synchrotron radiation facilities, thus making them a new tool for hadronic and spin studies.

Laguerre–Gaussian vortex beam for reduced thermal effects in nonlinear optical studies

Interaction of an intense laser beam with a material induces many thermal effects. In this work, thermo-optic effects induced by fundamental Gaussian and Laguerre–Gaussian vortex (LGV) laser beams in a sample in nonlinear optical (NLO) experiments are compared and their impact on the accuracy of determining the nonlinear susceptibility is examined. A solution of saturable absorber dye IR 26 in dichloroethane with the technique of z-scan to determine its third order nonlinear susceptibility was used as a model system. The LGV beams were generated by passing the Hermite–Gaussian beams from an Ar-ion laser through a cylindrical lens mode converter. Pump–probe setup was used to study the thermo-optic effects. Experiments and simulations suggest that the LGV beam is advantageous to reduce the thermal effects.

Effect of an external magnetic field on the self-focusing of a cosh-Gaussian laser beam in plasma under the relativistic-ponderomotive effect

This work presents an analytical and numerical study of the relativistic-ponderomotive effect on self-focusing of an intense cosh-Gaussian laser beam in a collisionless magnetized plasma by considering an external magnetic field in the direction of propagation of the laser beam. The nonlinear differential equation for the beam width parameter/intensity of a cosh-Gaussian laser beam in a magnetized plasma is obtained by Wentzel–Kramers–Brillouin (WKB) and paraxial-ray approximations. The self-focusing of the cosh-Gaussian beam at different values of the magnetic field parameter is investigated. The results have also been compared to relativistic nonlinearity. The results show that the self-focusing effect of cosh-Gaussian beam in magnetized plasma becomes stronger, when relativistic and ponderomotive nonlinearities acts together. In addition, the self-trapping of cosh-Gaussian beam in magnetized plasma has also been studied. Numerical results are presented for the well-established laser and plasma parameters.

Gamma Photons and electron-pairs Generation estimation for collision of PW-class Laser and electron beams

After the proposal of the concept of CPA techniques, the laser intensity has boosted dramatically since then. As the focusing intensity of the laser beam reaches the order above 1023 W/cm2 for multiple PW laser facilities, the laser material interaction enters the QED regime, where the gamma photons generation and electrons-positron pairs generation can be realized. This paper provides an overview of the current research in the field of electrodynamics about laser intensities and electron generation. Basic theories of the generation of e and e- pair and photons are introduced. The history of the development of major laser facilities with high-laser intensities is introduced, and the laser facilities are compared and discuss in terms of the electron generations. The results are further compared with the PIC simulation and typical generation scenarios are demonstrated. Potential limits are mentioned as the drawbacks of the models. Overall, these results shed light on guiding further exploration of laser-plasma interactions in the extremely strong intensity laser beam.

Energy-Conserving Theory of the Blowout Regime of Plasma Wakefield.

We present a self-consistent theory of strongly nonlinear plasma wakefield (bubble or blowout regime of the wakefield) based on the energy conservation approach. Such wakefields are excited in plasmas by intense laser or particle beam drivers and are characterized by the expulsion of plasma electrons from the propagation axis of the driver. As a result, a spherical cavity devoid of electrons (called a "bubble") and surrounded by a thin sheath made of expelled electrons is formed behind the driver. In contrast to the previous theoretical model [W. Lu etal., Phys. Rev. Lett. 96, 165002 (2006)PRLTAO0031-900710.1103/PhysRevLett.96.165002], the presented theory satisfies the energy conservation law, does not require any external fitting parameters, and describes the bubble structure and the electromagnetic field it contains with much higher accuracy in a wide range of parameters. The obtained results are verified by 3D particle-in-cell simulations.

Long-term repeatability improvement using beam intensity distribution for laser-induced breakdown spectroscopy

The relatively low measurement repeatability has long been considered as a major obstacle to the widespread use and commercialization of laser-induced breakdown spectroscopy (LIBS). Although many efforts have been made to improve the signal repeatability in the short term, how to improve the long-term signal repeatability is critical in practical applications and has rarely been studied. Moreover, the mechanisms behind the degradation of long-term repeatability are not fully revealed. This study proposes a new method to improve the long-term repeatability of LIBS measurement, which modifies the spectral intensity based on laser beam intensity distribution. It first pre-processes the beam intensity distribution profiles and spectral intensity. Then the relationship between the relative deviations of beam and spectral intensities is modelled using Partial Least Squares Regression (PLSR). The proposed method was tested on copper and silicon samples, and the spectra and laser beam intensity distribution were recorded for more than thirty days. Day-to-day variations in beam intensity distribution were observed. Such variations can lead to changes in spectral intensity, resulting in degraded signal repeatability. By modifying the spectral intensity, the long-term signal repeatability was improved. Specifically, in terms of day-mean spectral intensity, the valid correction rates were above 70% for both of copper silicon sample in most cases. Long-term RSD decreased from ∼13.5% to ∼4% for copper and decreased from ∼10.7% to 6.5% for silicon sample. These results indicate that the proposed method provides a viable method for improving the long-term repeatability of LIBS measurement.

Generation of High-Power Terahertz Waves in a Collisional and Magnetized Plasma by Two-Color Femtosecond Laser Beams

Terahertz (THz) radiation generation based on a nonlinear induced electron current density in the interaction of two-color femtosecond laser beams with collisional and magnetized plasma is investigated. The nonlinear electron current density that is responsible for THz radiation includes a share from nonlinear ponderomotive force and a part from relativistic term. In this work, relativistic effects along with the effects of variation of interacting plasma density, external magnetic field, and electron collision frequency on THz wave generation have been considered. The reduction of electron collision frequency along with rising in the magnitude of the external magnetic field generates more power without any deformation of radiation patterns. The angular distribution showing the radiation pattern of THz radiation in the forward direction is obtained and the effect of laser pulse second harmonic and variation of electric field on the directivity of generated waves is examined. The change in two-color laser beam intensities both in relativistic and nonrelativistic regimes leads to the generation of THz wave electric fields with different orders of magnitude. The numerical analysis indicated that the utilization of laser pulse second harmonic in a two-color scheme enhances the THz electric field leading to more intense radiation compared to single-color mechanism. The model also shows the effect of external magnetic field and electron collision frequency on the radiation efficiency of THz generation for linear and circular polarizations of two-color laser pulses.

Dynamics of Hermite–Gaussian laser beam in plasma and terahertz generation

In the present work, the dynamical study of a Hermite–Gaussian (HG) laser beam propagating through plasma with relativistic nonlinearity has been carried out. Furthermore, the dependency of THz generation on the HG laser dynamics has also been investigated. Self-focusing of laser beam inside plasma is achieved due to the modification in electron’s rest mass due to their motion at relativistic velocities. The coupled differential equations obtained using the method of moment determines the variation in spot size of laser beam and have been solved numerically. The laser beam propagating through plasma excites the plasma wave and the nonlinear coupling of HG beam and plasma wave generates THz radiation. It has been observed that THz generation strongly depends upon the variation of spot size, TEM modes, plasma density and intensity of laser beam. Furthermore, the self-trapping of HG laser beam has also been studied.

Direct time-resolved plasma characterization with broadband terahertz light pulses.

We report here the results of comprehensive plasma characterization and diagnostics by analyzing time-resolved absorption spectra of short ultrabroadband (0.1-50 THz) pulses propagated through the test plasma. Spectral analysis of plasma-induced absorption of such THz pulses provides very direct, in situ, high dynamical range, potentially single-shot access to the plasma density, plasma decay time, electron temperature, and ballistic dynamics of the plasma expansion. We have demonstrated a proof-of-principle measurement of plasma created by an intense laser beam. In particular, we showed a reliable measurement of plasma densities from around 10^{16} to 10^{20}cm^{-3}. Apart from the plasma parameters, this method allowed us to reconstruct peak intensity inside the plasma spot and to observe a very early stage of plasma evolution after its excitation.

Beam-by-beam Kerr clean-up in multimode optical fibres – INVITED

We propose and demonstrate the concept of beam-by-beam cleaning in multimode optical fibres, i.e., the increase of the spatial quality of an intense laser beam, induced by a relatively weak, quasi singlemode seed beam. This effect, which relies on the Kerr nonlinearity of the fibre, is quite efficient: a seed beam is capable of providing a bell-shape to a ten times more powerful beam. Our results pave the way for the development of a new class of all-optical switching devices for intense laser beams.