A composite material with a nominal composition of Ni0.6Fe2.4O4 was prepared by the solid-phase reaction method. X-ray diffraction analysis shows that the product is composed of α-Fe2O3 and a solid solution of Fe3O4 and NiFe2O4. Although α-Fe2O3 non-magnetic phase reduces the saturation magnetization, it greatly improves the temperature and frequency stability of magnetic permeability. Based on the measurement results of the amplitude permeability in the range of −60 °C to 100 °C, the temperature coefficient αμ and specific temperature coefficient β were calculated. αμ and β of the composite material are 7.15 ×10-5/°C and 8.6 ×10-6/°C, respectively, which are much smaller than αμ (1.26×10-3/°C) and β (9.5×10-5/°C) of NiFe2O4. At the same time, the magnetic spectrum curves show that the real part of the complex permeability μ' basically remains unchanged within the measurement frequency range (f < 106 Hz). This improvement in temperature and frequency stability is attributed to the effect of the α-Fe2O3 phase.
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