Femtosecond Laser Pulses In Air Research Articles

Energy interchange between large-scale free propagating filaments and its background reservoir

Multiple filaments surrounded by a large area of energy reservoir have been generated by a free propagating intense femtosecond laser pulse in air. The effects of the energy reservoir on the filament core have been investigated by inserting a diaphragm in a selected single filament path to block the energy of the reservoir. The evolution of filamentation has been studied experimentally and numerically as a function of diaphragm size. Both experimental and numerical results show that for millimeter size filaments with hundreds of meters distance, the energy reservoir can be extended to about 10 mm from the filament core.

Peculiarities of the spatial focusing of a high-power femtosecond laser pulse in air

The propagation of focused high-power femtosecond laser pulses in air is numerically simulated. The dependences of the effective average size of a focal spot and the maximum achievable radiation intensity in the focal beam waist on the peak power of incident radiation are studied. It is shown that in the regime of nonstationary self-action of radiation, due to photoionisation of the medium and formation of plasma, it becomes impossible to focus radiation into a spot of diffraction-limited size predicted by a linear theory.

Filamentation of interacting femtosecond laser pulses in air

The filamentation of two co-propagated femtosecond (fs) laser pulses in air is studied by numerical simulation. Depending on the different initial separation distances, relative phase shift and crossing angles, simulations show attraction, fusion, repulsion and collision of the two pulses. A long plasma channel can be formed by two in-phase pulses with small separation distance and cross angle. The coupling of two laser beam becomes weaker when the separation distance or cross angle between two beams is larger. In this case, the filamentation of each pulse develops independently. Our simulation results will be helpful for understanding the effect of the initial amplitude and phase modulation of laser pulse on the filamentation characteristics.

Experimental study and numerical simulation of the propulsion of microbeads by femtosecond laser filament

The light filament formed by intense femtosecond laser pulses in air can be used to generate the effective impulse to propel a micro glass bead. In this report, through both experimental studies and the corresponding numerical simulations that involve the dynamics of the nonlinear propagation of light and the laser ablation mechanism, we confirm that this propulsion scheme is based on the laser ablation of the target material. The fundamental characteristics of laser propulsion using a single ultrafast laser filament is also revealed.

Ultra-broadband enhanced absorption of metal surfaces structured by femtosecond laser pulses

We investigate the enhanced absorption properties in a wavelength range of 0.2-25 microm for NiTi alloy targets structured by femtosecond laser pulses in air. Three different types of surface structures are produced with varying laser fluences. Measured reflectances through integrating sphere technique show that their couplings of incident electromagnetic irradiations are improved greatly over the broadband wavelength range. In particular, for coral-like micro-structures on the metal surfaces, approximate 90% absorption can be achieved from ultraviolet to mid-infrared region. Cut-off wavelengths of the enhanced absorption for the varied dimensional surface structures are determined experimentally. Chemical analysis by X-ray photoelectron spectroscopy indicates that blackness of metal surfaces is not attributed to the change in elemental composition. The physics of such remarkable absorption for the structured metal surfaces are discussed as well.

Observation of filamentation-induced continuous self-frequency down shift in air

We observed a new filamentation nonlinear process: continuous self-frequency down shift inside the filament zone during the propagation of a femtosecond laser pulse in air. The frequency shift depends strongly on the length of the self-guided column (filament).

Evolution and termination of a femtosecond laser filament in air

The evolution of the filamentation of a femtosecond laser pulse in air is measured. The divergence of the filament core is almost constant over a long distance, encompassing a zone with efficient ionization followed by another where ionization is much weaker. At the end, the core diverges out linearly with a low divergence due to self-spatial filtering.

Spectroscopic analysis of femtosecond laser plasma filament in air

We report a spectroscopic analysis of a filament generated by a femtosecond laser pulse in air. In the filament spectra, the characteristic Stark broadened atomic oxygen triplet centered at 777.4nm has been observed. The measured electron impact Stark broadening parameter of the triplet is larger than the theoretical value by Griem [H.R. Griem, Plasma Spectroscopy, McGraw Hill, New York, 1964] by a factor 6.7. Using the experimental value 0.0166nm, the plasma densities derived from Stark broadening agree well with those most recently obtained from Théberge et al.’s measurement of the nitrogen fluorescence calibrated by longitudinal diffraction [F. Théberge, W. Liu, P.T. Simard, A. Becker, S. L. Chin, Phys. Rev. E 74 (2006) 036406]. However, the Stark broadening approach is much simpler and can be used to non-invasively measure the filament plasma density distribution in air under different propagation conditions.

Simultaneous detection and identification of multigas pollutants using filament-induced nonlinear spectroscopy

The authors report on an approach for simultaneous monitoring of multigas pollutants based on fluorescence emission of trace gases, induced by the filamentation of intense femtosecond laser pulses in air. The high intensity inside a filament can dissociate the gas molecules into small fragments which emit characteristic fluorescence. This method is illustrated for simultaneously sensing atmospheric trace gases, methane and acetylene. The spectra of an “unknown” mixture were analyzed by using a genetic algorithm, showing good concentration agreement with the experimental results within an error of 25%.

Oval-like hollow intensity distribution of tightly focused femtosecond laser pulses in air

The propagation of a tightly focused femtosecond laser pulse in air has been investigated. Unlike long-distance self-guided propagation of short laser pulses, a novel oval-like hollow distribution of the laser intensity is observed in the experiments and reproduced by the numerical simulations. The formation of the hollow structures can be explained by the interplay between ionization-induced refraction and Kerr self-focusing.

Optimization of multiple filamentation of femtosecond laser pulses in air using a pinhole

The robustness and prolongation of multiple filamentation (MF) for femtosecond laser propagation in air are investigated experimentally and numerically. It is shown that the number, pattern, propagation distance, and spatial stability of MF can be controlled by a variable-aperture on-axis pinhole. The random MF pattern can be optimized to a deterministic pattern. In our numerical simulations, we configured double filaments to principlly simulate the experimental MF interactions. It is experimentally and numerically demonstrated that the pinhole can reduce the modulational instability of MF and is favorable for a more stable MF evolution.

Remote detection of similar biological materials using femtosecond filament-induced breakdown spectroscopy

We demonstrated the feasibility of remote detection and differentiation of some very similar agricultural-activity related bioaerosols, namely barley, corn, and wheat grain dusts, through nonlinear fluorescence of fragments induced by the high-intensity inside filaments of femtosecond laser pulses in air. The signals were detected in Lidar configuration with targets located at 4.7 m away from the detection system. All the species showed identical spectra, namely those from molecular C2 and CN bands, as well as atomic Si, C, Mg, Al, Na, Ca, Mn, Fe, Sr and K lines. These identical spectral bands and lines reveal similar chemical compositions; however, the relative intensities of the spectra are different showing different element abundances from these three bio-targets. The intensity ratios of different elemental lines were used to distinguish these three samples. Good reproducibility was obtained. We expect that this technique could be used at long distance and thus played as a sensor of similar biological hazards for public and defense security.

Characteristics of multiple filaments generated by femtosecond laser pulses in air: Prefocused versus free propagation

The characteristics of the multiple filaments formed by prefocused and freely propagating femtosecond laser pulses are investigated and compared. It is shown in our experiments that the diameter, length, stability, and interaction for the two cases can be quite different. The filaments formed by prefocused beam indicate dynamic spatial evolution with higher laser intensity and electron density. They have a typical diameter of 100 microm are of shorter length. In the free propagation case, the filaments exhibit interesting properties such as hundred-meter propagation distance and mm-size diameter. Moreover, only the interaction of the filaments with the energy background affects the evolution of the filaments. Filament-filament interactions such as the filament splitting and merging were not observed in this case.

Generation of third harmonic emission in propagation of femtosecond laser pulses in air

The main characteristics of the third harmonic emission generated by femtosecond laser pulses propagating in air are investigated by numerically solving the coupled nonlinear Schrodinger equations. Strong third harmonic emission is observed with a maximum conversion efficiency as high as 0.43%. The on-axis phase difference between fundamental beam and third harmonic is investigated. The result is in good agreement with the phase-locking mechanism. Dependence of the conversion of third harmonic emission on focusing conditions is also studied. The results are also compared with those of experiments.

Self-focusing arrest of femtosecond laser pulses in air at different pressures

We study analytically and numerically the self-focusing arrest of femtosecond laser pulses in air at different pressures in the presence of an external focus lens. Analytical estimations as well as results of simulations show that the intensity at which the self-focusing arrest occurs is almost independent of the gas pressure. However, a dependence on the temperature is found. The Raman effect is taken into account, and an estimation of the intensity inside of filaments at high altitudes is given.

Interaction of Light Filaments Generated by Femtosecond Laser Pulses in Air

The interaction of two light filaments propagating in air is simulated. Simulations show that the interaction of the two light filaments displays interesting features such as attraction, fusion, repulsion, and spiral propagation, depending on the relative phase shift and the crossing angle between them. A long and stable channel can be formed by fusing two in-phase light filaments. The channel becomes unstable with the increase of the crossing angle and phase shift. The interaction of two light filaments in different planes is studied and the spiral propagation is observed.

UV–Supercontinuum generated by femtosecond pulse filamentation in air: Meter-range experiments versus numerical simulations

We report new experimental and numerical results on supercontinuum generation at ultraviolet/visible wavelengths produced by the propagation of infrared femtosecond laser pulses in air. Spectral broadening is shown to similarly affect single filaments over laboratory distance scales, as well as broad beams over long-range propagation distances. Numerical simulations display evidence of the crucial role of third harmonic generation in the build-up of UV–visible wavelengths, by comparison with current single-envelope models including chromatic dispersion and self-steepening.

Collapse dynamics of super-Gaussian Beams

We investigate the self-focusing dynamics of super-Gaussian optical beams in a Kerr medium. We find that up to several times the critical power for self-focusing, super-Gaussian beams evolve towards a Townes profile. At higher powers the super-Gaussian beams form rings which break into filaments as a result of noise. Our results are consistent with the observed self-focusing dynamics of femtosecond laser pulses in air [1] in which filaments are formed along a ring about the axis of the initial beam where the initial beam did not form a ring.

Long lifetime plasma channel in air generated by multiple femtosecond laser pulses and an external electrical field

The lifetime of a plasma channel produced by self-guiding intense femtosecond laser pulses in air is largely prolonged by adding a high voltage electrical field in the plasma and by introducing a series of femtosecond laser pulses. An optimal lifetime value is realized through adjusting the delay among these laser pulses. The lifetime of a plasma channel is greatly enhanced to 350 ns by using four sequential intense 100fs(FWHM) laser pulses with an external electrical field of about 350kV/m, which proves the feasibility of prolonging the lifetime of plasma by adding an external electrical field and employing multiple laser pulses.

Femtosecond filamentation in air at low pressures. Part II: Laboratory experiments

We present experimental studies of filamentation of a femtosecond laser pulse in air at low pressures. The evolution of the filament has been studied by measuring along the propagation axis the conductivity and the sub-THz emission from the plasma channel. We show experimentally that the filamentation process occurs at pressures as low as 0.2atm in agreement with numerical simulations. Experimental and numerical results [A. Couairon, M. Franco, G. Méchain, T. Olivier, B. Prade, A. Mysyrowicz, Opt. Commun., submitted for publication] are compared and the possible sources of discrepancy are discussed.