Electric Field Region Research Articles

Numerical model of restrikes in gliding arc discharges

Abstract Direct current (DC) electric arcs are of particular interest because they can produce large volumes of thermal plasmas with controlled energy deposition. When such discharges are applied in a gas flow, convection displaces the top of the arc downstream while the arc roots remain attached to the electrodes, thus increasing the length of the arc over time. However, this growth is limited by a restrike phenomenon, which starts from streamers appearing in high electric field regions and shortcutting the long, stretched electric arc. From a numerical point of view, DC arcs can be efficiently simulated with a resistive magneto-hydrodynamics (MHD) model, with numerical requirements in terms of spatial and temporal discretization that are compatible with classic fluid dynamics and combustion simulations. However, arc restrikes rely on the propagation of streamer discharges that are highly non-neutral phenomena, whereas classical MHD assumes neutrality. To tackle this problem, we propose in this paper a model of restrike that can be used in an MHD approach. After describing the ideas of the model, we perform a parametric study of the input parameters to examine its influence on the discharge dynamics.

Mg content regulating built-in electric field for self-powered ZnO/MgxZn1-xO Schottky UV photodetector

In recent years, self-powered Schottky ultraviolet (UV) photodetectors (PDs) have attracted great attention due to their low manufacturing cost and zero-bias response. However, the development of high-performance self-powered Schottky devices is limited by the weak light response due to the internal weak electric field. Here, we introduce a MgxZn1-xO capping layer on ZnO and fabricate a ZnO/MgxZn1-xO heterojunction Schottky UV PD by using the sol-gel method. The improved device exhibits excellent self-powered characteristics and stability, specifically, an increase of 909% in photocurrent, an improvement of more than one order of magnitude in responsivity, and an improved linear dynamic region (LDR: 33.7 dB). The introduction of the MgxZn1-xO capping layer is responsible for the improved device performance, resulting in enhanced built-in electric field and depletion region width due to the increase of the Schottky barrier, thereby facilitating the separation and transport of photogenerated carriers. This work provides an effective way to fabricate high-performance self-powered ZnO Schottky UV PDs.

Effects of Annealing and Domain Structure on the Photovoltaic Response in Pb[(Mg1/3Nb2/3)0.70Ti0.30]O3 Single Crystal

Crystalline acentricity leading to the photovoltaic (PV) effect in ferroelectrics (FEs) emerges these materials as important candidates for the PV cells potentially overcoming the Shockley–Queisser limit of semiconductors. However, this research direction still requires more investigations to develop reliable pathways for PV efficiency optimization. Herein, it is reported that due to the sample annealing above the Curie point the PV effect asymmetry with respect to the poling sign can be compensated and intrinsic PV response of the FE crystal can be increased by more than 20% in comparison with the pristine sample. It is also reported how the orientation of domain walls can be used to engineer the PV effect in the subcoercive electric field region. The reported results contribute to better understanding of PV effect tuning in the FEs paving the way for more efficient and sustainable solar energy utilization.

Meta-Aerogel Electric Trap Enables Instant and Continuable Pathogen Killing in Face Masks.

The tremendous menace of the COVID-19 pandemic has underscored the urgency for antipathogen masks to stop the transmission of airborne infectious diseases. Most prevailing antipathogen masks manifest a slower sterilization rate that lags behind the pathogen momentum traversing the masks, thereby engendering an elevated susceptibility to infection. Here we tailor nanofibrous meta-aerogel electric traps, 3D-assembled from self-knotted carbon nanotube networks in an all rigid nanofibrous skeleton. This superior configuration revolves around the creation of numerous "dielectrophoretic-aerodynamic grippers", which are capable of directional manipulation of microbes toward the region of the lethal intensive electric field. Based on this, we present a disinfection unit comprising a pair of aerogel electrodes that demonstrate a rapid killing rate (>99.99% biocidal efficacy within 0.016 s) and long-term durability (12 h of continuous operation). Additionally, a microbutton lithium cell is employed as a power supply to fabricate an antipathogen face mask with this disinfection unit, which exhibits superior pathogen inactivation efficacy compared to commercial masks. This scalable biocidal protective equipment holds great potential for use in emergency medical services.

Local Electron Density Depletions in the Martian Upper Ionosphere Obtained From MARSIS: Comparison With ASPERA‐3, and MAVEN, and the Connection With Crustal Magnetic Fields

AbstractSteep electron density depletions in the Martian ionosphere are important, especially because they could be regions of significant plasma escape. Local electron density profiles of the Martian ionosphere obtained from the radar sounder onboard the Mars Express spacecraft often show large fluctuations. In some cases, these fluctuations are observed as deep depletions in the electron density. Investigation over the past 12 years of Mars Advanced Radar for Subsurface and Ionospheric Sounding data have revealed over 200 cases of density depletions where the lowest density is less than one fifth of the density in the surrounding regions. These density dips occur both on the dayside and the nightside, with an abundance between solar zenith angles of 50–70° and 100–120°. They occur at all altitudes in the ionosphere. Many of the depletions occur in the southern hemisphere where the crustal magnetic field is stronger and there are more regions where the crustal magnetic field is mostly vertical. In more than half of the cases, the depletion in the local electron density corresponds to a decrease in the electron flux measured with the Analyzer of Space Plasmas and Energetic Atoms electron spectrometer. Several different mechanisms could be responsible for the formation of the depletions, including regions of localized electric fields or magnetic fields creating areas of increased field pressure, escape of the plasma along magnetic field lines depleting density locally, and the density decrease around the photoelectron boundary followed by an increase in the plasma density due to plasma clouds.

Dynamics of dielectric micropore discharge in atmospheric pulsed dielectric barrier discharge

In this paper, a two-dimensional self-consistent fluid model was developed in atmospheric helium for dielectric barrier discharge excited by microsecond voltage pulses, in which a dielectric sheet with micropore is inserted in the interelectrode gap. It demonstrates that the discharge generated in dielectric micropore is in the form of propagating ionization wave, which reaches the plasma density of 1.32 × 1020 m−3 and the mean electron energy of 17.70 eV. The transverse electric field perpendicular to the applied longitudinal electric field in dielectric micropore is found to play an important role on the electron acceleration and generation, which is induced by the space charges in the micropore. The migration fluxes of electron and ions driven by electric field and diffusion explains the formation of transverse electric field and sheath regions above the dielectric surfaces.

Piezoelectric Relaxation in Piezoceramics in the Region of Weak Permanent Electric Fields

Piezoelectric Relaxation in Piezoceramics in the Region of Weak Permanent Electric Fields

Nonlinear and Relaxation Processes in Piezoceramics in the Region of Weak Electric Fields

Nonlinear and Relaxation Processes in Piezoceramics in the Region of Weak Electric Fields

Influence of low electric field parts of electric field–current density curves of superconductors on their ac loss characteristics

We performed numerical electromagnetic field analyses to investigate the influence of the low electric field parts of the electric field (E)–current density (J) curves of superconductors on their ac loss characteristics. A simple one-dimensional model across the width of a coated conductor was used for the analyses. Whereas we fixed the n value of the high E part of E–J curves of superconductors, we varied the n values of low E parts. J distributions as well as E distributions were calculated in coated conductors carrying ac currents and/or exposed to ac magnetic fields. We examined the influence of the n values at low E part of E–J curves on ac loss characteristics and discussed the electric field regions that are relevant to ac loss generation. We also discussed the applicability of the results to copper-plated multifilament coated conductors.

On the Practical Limitations for the Generation of Gunn Oscillations in Highly Doped GaN Diodes

Planar Gunn diodes based on doped GaN active layers with different geometries have been fabricated and characterized. Gunn oscillations have not been observed due to the catastrophic breakdown of the diodes for applied voltages around 20–25 V, much below the bias theoretically needed for the onset of Gunn oscillations. The breakdown of the diodes has been analyzed by pulsed <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"> <tex-math notation="LaTeX">$\textit{I}$</tex-math> </inline-formula> – <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"> <tex-math notation="LaTeX">$\textit{V}$</tex-math> </inline-formula> measurements at low temperatures, and it has been observed to be almost independent of the geometry of the channels, thus allowing to discard self-heating effects as the origin of the device burning. The other possible mechanism for the device failure is an impact-ionization avalanche due to the high electric fields present at the anode corner of the isolating trenches. However, Monte Carlo simulations using the typical value of the intervalley energy separation of GaN, <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"> <tex-math notation="LaTeX">$\varepsilon_{\text{1}-\text{2}}$</tex-math> </inline-formula> <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"> <tex-math notation="LaTeX">$=$</tex-math> </inline-formula> 2.2 eV, show that impact ionization mechanisms are not significant for the voltages for which the experimental failure is observed. But recent experiments showed that <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"> <tex-math notation="LaTeX">$\varepsilon_{\text{1}-\text{2}}$</tex-math> </inline-formula> is lower, around 0.9 eV. This lower intervalley separation leads to a much lower threshold voltage for the Gunn oscillations, not far from the experimental breakdown. Therefore, we attribute the device’s failure to an avalanche process just when Gunn domains start to form, since they increase the population of electrons at the high electric field region, thus strongly enhancing impact ionization mechanisms that lead to the diode failure.

High electric field characteristics of GaAsSb photodiodes on InP substrates

Low noise avalanche photodiodes (APDs) detecting 1550 nm wavelength play a crucial role in optical communication and LiDAR systems. These APDs utilize a separate absorption, charge, and multiplication (SACM) architecture with an absorber for 1400–1650 nm detection and a low noise, high gain multiplier that can be independently optimized for a high signal-to-noise ratio. Recently, GaAs0.5Sb0.5/Al0.85Ga0.15As0.56Sb0.44 SACM APDs have demonstrated ultra-high gain and extremely low noise, possibly improving sensitivity over Si and InGaAs/InP commercial APDs. This accomplishment was achieved using a GaAsSb absorber instead of a conventional InGaAs absorber, mitigating band discontinuities between the absorber and the multiplier. However, further optimization is required to reduce noise due to tunneling and impact ionization from the GaAsSb absorber, which occurs at a high electric field region. This paper focuses on the study of the high-field characteristics of GaAsSb photodiodes (PDs). The tunneling phenomenon is analyzed through current density-voltage measurements, and the impact ionization behavior is evaluated by measuring the multiplication of p-i-n GaAsSb PDs. The result suggests that when designing a SACM APD with a GaAsSb absorber, the electric field in the absorber can be increased to 175 kV/cm without the detrimental effects of ionization occurring in the absorber. The findings from this investigation will assist in optimizing GaAsSb-based SACM APDs and promoting further advancements in the 1550 nm APD technology.

Ambient Conditions of Winter Thunderstorms in Japan to Reproduce Observed Gamma‐Ray Glow Energy Spectra

AbstractElectric field of thunderclouds modifies components and energy spectra of the cosmic‐ray air shower. In particular, thunderstorms accelerate charged particles, resulting in an enhancement of gamma‐ray fluxes on the ground, known as a gamma‐ray glow. This phenomenon has been observed in recent years by the Gamma‐Ray Observation of Winter THunderclouds collaboration from winter thunderstorms in the Hokuriku area of Japan. The present work examines the ambient conditions required to produce spectral features of the previously detected gamma‐ray glows, by using Monte Carlo simulations of particle interactions in the atmosphere. We focus on three parameters, the strength and length of the electric field, and the length of a null‐field attenuation region below the electrified region. The average spectrum of observed gamma‐ray glows in winter thunderstorms of Japan requires an electric field intensity close to 0.31 MV/m, slightly exceeding the Relativistic Runaway Electron Avalanche threshold of 0.284 MV/m. The vertical size of the electric field region should be comparable to 1 km. The estimated attenuation region size is 300–500 m, necessary to reduce the low‐energy photon flux of the average gamma‐ray glows. There is still a wide range of acceptable parameter sets with degeneracy to make a similar spectrum.

Inferring electrospray emission characteristics from molecular dynamics and simulated retarding potential analysis

In this work, we present coordinated molecular dynamics, ion cluster acceleration, and retarding potential analysis simulations to determine cluster fragmentation behavior in a realistic emitter geometry for electrosprays operating in the pure ionic regime. Molecular dynamics simulations are used to determine the fragmentation rates of ionic liquid clusters as a function of internal energy, electric field strength, and cluster size. A simplified model of electrospray cluster acceleration is developed from previous electrohydrodynamic emission models and used to simulate retarding potential analysis curves. Fragmentation rates and beam composition are inferred for experimental data based on the molecular dynamics and cluster acceleration simulations. We find that for these experimental data, temperatures of EMI-BF4 dimers likely range between 590 and 687 K while trimer temperatures are larger between 989 and 1092 K. The percentage of monomers, dimers, and trimers in the beam is approximately 45%, 30%–43%, and 13%–25%, respectively. Both ionic liquid cluster temperatures and beam composition agree with previous analysis of this experimental work, supporting the use of coordinated molecular dynamics and retarding potential analysis as a method of inferring electrospray beam parameters. Insights gained from this simulation process are discussed in the context of currently unexplained electrospray emitter behavior and experimental results including the presence of tetramers and trimers in the beam and fragmentation rates in high electric field regions.

Procedure to generate a selection chart for microwave sol-gel synthesis of nanoparticles

Numerical simulation is used to compare the temperature distribution existing during microwave or conventional heating by hot oil bath of a reaction volume. The simulation is applied to the sol-gel synthesis of TiO2 nanopowders, considering temperature dependent materials parameters. A WR340-based single mode applicator operating at 2.45 GHz is considered, with a cylindrical load positioned in regions of predominant electric field. A temperature homogeneity index, defined as the ratio between the average temperature and its standard deviation at a certain time, is used to compare homogeneity of conventional and microwave heating at different power densities, from 370 to 7400 W/L. Based on that comparison, a selection chart of the more homogenous heating process as a function of power density and average temperature of the reaction volume is defined and can be used to select the experimental conditions expected to lead to a more or less homogeneous particle size of the products.A dedicated instrumented model, including three optical fibres, is developed as well, for validation purposes. Experimental validation showed a very good predictive capability of the model, with errors on estimated temperature lower than 3 °C at temperatures lower than 80 °C.

Modeling the Neuruppin ball lightning incident

In 1994, a 370-kA positive cloud-to-ground (CG) discharge 5 km east of Neuruppin, Germany was immediately followed by the production of at least ten ball lightning objects seen by numerous eyewitnesses. We propose a sequence of events based on observations of upward lightning triggered by CG flashes which can explain how a large ground-level electric field (∼1 MV m−1) could be produced by negative leaders extending into a region of positive charge above Neuruppin, resulting in transfer of a large amount of charge horizontally between the CG discharge and the region of high electric field. This model provides a causal link between the large CG discharge east of Neuruppin and the large ground-level fields which were associated with the production of ball lightning. Recommendations follow for producing ball lightning in a large laboratory experiment.

Orbital Polarization-Dependent Fragment Twist-Induced Intramolecular Electric-Field-Driven Charge Transfer

Defects, such as twisting, in fused aromatic hydrocarbons disrupt the plane of the π orbital. The twisted structure induces an electric field in the system and affects the spectra. In this work, theoretical studies show that the intramolecular electric field within a distinctly twisted structure is larger than that of other molecules. In addition, the spectral study shows that the degree of charge transfer and the magnetic transition dipole in the electrostatic potential extremum region of the molecular electric field were significantly improved, which affected the optical absorption and chiral optical behavior of the molecule. The discovery of this theoretical regulation law will provide a solid foundation for the electric-field-induced regulation of optical properties and will promote the precise design and synthesis of optoelectronic molecules with inner electric fields.

Dielectric polarization-based separations in an ionic solution.

A novel non-electrophoretic, electric field-based separation mechanism capable of transporting ions based on their dielectric properties is presented here for the first time. Though this polarization-based mechanism behaves similarly to dielectrophoresis, the separation mechanism is remarkably very efficient at small length scales compared to any dielectrophoretic separation mechanism for particles. For an applied electric field of strength as low as ∼0.75 MV m-1 across a 100 μm channel, the working solute - sodium fluorescein - is shown to decrease in its concentration by ≈20% in electric field region relative to the non electric field region. The existing macroscopic theoretical models like electrohydrodynamics and equilibrium thermodynamics are shown to underestimate the concentration change by two orders of magnitude for the same electric field strength. This surprisingly large difference between theory and experimental results suggests that the electric field-based equilibrium thermodynamic model lacks a key physics.

Cooperative multiple interactions of donor-π-acceptor dyes enhance the efficiency and stability of perovskite solar cells.

Surface passivation by organic dyes has been an effective strategy for simultaneous enhancement of the efficiency and stability of perovskite solar cells. However, lack of in-depth understanding of how subtle structural changes in dyes leads to distinctly different passivation effects is a challenge for screening effective passivation molecules (PMs). In an experiment done by Han et al. (Adv. Energy Mater., 2019, 9, 1803766), three donor-π-acceptor (D-π-A) dyes (SP1, SP2, and SP3) with distinct electron donors have been applied to passivate the perovskite surface, where the efficiency and stability of PSCs are quite different. Herein, we carried out first-principles calculations and ab initio molecular dynamics (AIMD) simulations on the structures and electronic properties of SP1, SP2, SP3, and their passivated perovskite surfaces. Our results showed that SP3 enhances the carrier transfer rate, electric field, and absorption region compared to SP1 and SP2. Moreover, AIMD simulations reveal that the cooperative multiple interactions of O-Pb, S-Pb, and H-I between SP3 and the perovskite surface result in a stronger passivation effect in a humid environment than that of SP1 and SP2. This work is expected to pave the way for screening dye passivation molecules to endow perovskite solar cells with high efficiency and stability.

Operando investigation of particle re-entrainment mechanism in electrostatic capture process on the lab-on-a-chip

Inhalable particle is a harmful air pollutant that causes a significant threat to people's health and ecological environments, which should be removed to purify air, but there exists limited removal efficiency due to particle re-entrainment. Here, Operando observation system based on microscopic visualization method is developed to make in situ test of particle migration, deposition and re-entrainment characteristics on a lab-on-a-chip to achieve the investigation in micro-level scale. The deposition evolution of charged particles is recorded in electric field region intuitively, which confirms the fracture of particle chain occurs during the growth process of deposited particles. It captures the instantaneous process that a larger particle with micron size due to the coagulation of submicron particles fractures from main body of the particle chain for the first time. The analysis of migration behavior of a single submicron particle near electrode surface demonstrates the direct influence of drag force on the fracture of particle chain. This work is the first-time visualization of dynamic process and mechanism elucidation of particle re-entrainment at the micron level, and the findings will provide the theory support for the particle re-entrainment mechanism and bring inspires of enhancing capture efficiency of inhalable particle.

Generation–recombination noise in uniformly doped semiconductors with contacts of finite surface recombination velocities

The formula for the voltage noise spectrum due to generation–recombination (G–R) rate fluctuations is derived for uniformly doped majority-carrier n-type semiconductor samples with contacts of finite surface recombination velocities. In the derivation of the formula, a new boundary condition with finite surface recombination velocities considered is used instead of the ohmic boundary condition. The G–R voltage noise spectra are calculated to become saturated and equal in the high electric field region irrespective of surface recombination velocities. However, the behaviors of slow surface recombination velocities in the low electric field region differ from those of fast ones. The profiles of the electron density fluctuations of slow ones differ significantly from those of fast ones in the low-field region. In the high field region, a steep rise in the magnitude of the electron density fluctuation occurs near the voltage contact toward which electrons drift. The various location dependencies of the contribution of noise sources to the voltage power spectral density are also derived for low and high field regions as well as low and high surface recombination velocities, and analytical expressions are developed for the voltage power spectral densities and electron density fluctuations.