Efficient Spin-photon Interface Research Articles

Alignment-free coupling to arrays of diamond microdisk cavities with fabrication tolerant spin-photon interfaces.

We propose a design for an efficient spin-photon interface to a color center in a diamond microdisk. The design consists of a silicon oxynitride triangular lattice overlaid on a diamond microdisk without any aligmnent between the layers. This enables vertical emission from the microdisk into low-numerical aperture modes, with quantum efficiencies as high as 46% for a tin vacancy (SnV) center. Our design is robust to manufacturing errors, potentially enabling large scale fabrication of quantum emitters coupled to optical collection modes. We also introduce a novel approach for optimizing the free space performance of our device using a dipole model, achieving comparable results to full-wave finite difference time domain simulations with 7 · 106 reduction in computational time.

Spin–photon interface for a solid-state spin system via single trapped ion

An efficient spin–photon interface plays a significant role in building quantum network and distributed quantum computing with solid-state spin system, e.g., nitrogen-vacancy (NV) center in diamond. Solid-state spin system has the advantages of excellent portability and long coherence time, however, it suffers from a critical drawback of low efficiency of spontaneously emitted photons in the zero phonon line. This poses a severe challenge for the generation of an efficient interface between solid-state spin and photon. Here, we propose a method to establish a coherent interface between photon and solid-state spin system which is coupled to a trapped ion via a quantum transducer. Our method provides a new route to establish an efficient spin–photon interface allowing the generation of entanglement between distant spins.

Purcell enhancement of single-photon emitters in silicon

Individual spins that are coupled to telecommunication photons offer unique promise for distributed quantum information processing once a coherent and efficient spin–photon interface can be fabricated at scale. We implement such an interface by integrating erbium dopants into a nanophotonic silicon resonator. We achieve spin-resolved excitation of individual emitters with <0.1GHz spectral diffusion linewidth. Upon resonant driving, we observe optical Rabi oscillations and single-photon emission with a 78-fold Purcell enhancement. Our results establish a promising platform for quantum networks.

Near-deterministic hybrid generation of arbitrary photonic graph states using a single quantum emitter and linear optics

Since linear-optical two-photon gates are inherently probabilistic, measurement-based implementations are particularly well suited for photonic platforms: a large highly-entangled photonic resource state, called a graph state, is consumed through measurements to perform a computation. The challenge is thus to produce these graph states. Several generation procedures, which use either interacting quantum emitters or efficient spin-photon interface, have been proposed to create these photonic graph states deterministically. Yet, these solutions are still out of reach experimentally since the state-of-the-art is the generation of a linear graph state. Here, we introduce near-deterministic solutions for the generation of graph states using the current quantum emitter capabilities. We propose hybridizing quantum-emitter-based graph state generation with all-photonic fusion gates to produce graph states of complex topology near-deterministically. Our results should pave the way towards the practical implementation of resource-efficient quantum information processing, including measurement-based quantum communication and quantum computing.

Structure‐Induced Tunable Multipolar Moments and the Associated Purcell Enhancement in Silicon‐Like Metasurfaces

The recent breakthrough in integrating single quantum emitters to dielectric metasurfaces opens up avenues in quantum technologies with the possibility to obtain on‐demand single photon sources and efficient spin–photon interface. All‐dielectric metasurfaces with unprecedented possibilities of generating directional light scattering instigated a novel concept of the Kerker effect that led to applications in nanophotonics. Here, an all‐dielectric metasurface consisting of silicon‐like nanodisks with square lattice symmetry that exhibits Kerker condition governed by constructive interference of multipoles optimized for the zero‐phonon line (ZPL) of negatively charged nitrogen‐vacancy (NV‐) center at a wavelength of 640 nm is discussed. The phase and amplitude of excited multipolar moments are manipulated by varying the geometrical parameters of the metasurfaces. The constructive interference between multipolar moments generates a Kerker condition, which is tunable by varying the diameter, thickness, refractive index of nanodisks, and substrate refractive index. The Kerker condition is further used to control the emission from a single NV‐ center and a Purcell enhancement of 300 times is achieved at 640 nm. The study profoundly explores new insights into quantum metasurfaces and paves a new way to utilize dielectric resonators with emitters as on‐chip quantum light sources at Kerker condition.

(Invited) Spin and Optical Properties of the Silicon Vacancy in 4H-SiC for Quantum Science and Technology

Silicon vacancies in SiC are of significant interest for quantum information and sensing due to their unusual combination of long spin coherence time, optical addressability, and room-temperature operation in an industrially-relevant semiconductor. We characterize the spin and optical properties of the V2 silicon vacancy in 4H-SiC for both single defects and ensembles. We also show that they can be deterministically placed with sub-micron precision using focused Li ion implantation. Low-temperature photoluminescence excitation spectroscopy of the spin-dependent optical transitions of single silicon vacancies reveals two sharp lines with linewidths near the radiative lifetime limit. These lines correspond to the ms=±1/2 and ms=±3/2 states of an S=3/2 spin system that can be optically initialized, coherently manipulated with RF pulses, and read out via spin-dependent photoluminescence. We measure the different properties of spins in the two bases, and compare them to theoretical models. To suppress the limiting effects of the nuclear spin bath, we grow isotopically purified SiC with a very low abundance of 29Si and 13C. Our room temperature spin coherence measurements show orders-of-magnitude improvement of the coherence times in these materials. In particular, the inhomogeneous dephasing time T2 * in the ms=±1/2 basis shows a ~100x improvement, reaching 20 μs. We consider the prospects of this system for quantum sensing and as an efficient spin-photon interface for use in quantum networks.This work was supported by the U.S. Office of Naval Research, the OSD Quantum Sciences and Engineering Program, the Defense Threat Reduction Agency, and the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. Sandia National Laboratories is a multi-mission laboratory managed and operated by National Technology and Engineering Solutions of Sandia, LLC., a wholly owned subsidiary of Honeywell International, Inc., for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-NA-0003525.

Multidimensional cluster states using a single spin-photon interface coupled strongly to an intrinsic nuclear register

Photonic cluster states are a powerful resource for measurement-based quantum computing and loss-tolerant quantum communication. Proposals to generate multi-dimensional lattice cluster states have identified coupled spin-photon interfaces, spin-ancilla systems, and optical feedback mechanisms as potential schemes. Following these, we propose the generation of multi-dimensional lattice cluster states using a single, efficient spin-photon interface coupled strongly to a nuclear register. Our scheme makes use of the contact hyperfine interaction to enable universal quantum gates between the interface spin and a local nuclear register and funnels the resulting entanglement to photons via the spin-photon interface. Among several quantum emitters, we identify the silicon-29 vacancy centre in diamond, coupled to a nanophotonic structure, as possessing the right combination of optical quality and spin coherence for this scheme. We show numerically that using this system a 2×5-sized cluster state with a lower-bound fidelity of 0.5 and repetition rate of 65 kHz is achievable under currently realised experimental performances and with feasible technical overhead. Realistic gate improvements put 100-photon cluster states within experimental reach.

Field-based design of a resonant dielectric antenna for coherent spin-photon interfaces.

We propose a field-based design for dielectric antennas to interface diamond color centers in dielectric membranes with a Gaussian propagating far field. This antenna design enables an efficient spin-photon interface with a Purcell factor exceeding 400 and a 93% mode overlap to a 0.4 numerical aperture far-field Gaussian mode. The antenna design with the back reflector is robust to fabrication imperfections, such as variations in the dimensions of the dielectric perturbations and the emitter dipole location. The field-based dielectric antenna design provides an efficient free-space interface for closely packed arrays of quantum memories for multiplexed quantum repeaters, arrayed quantum sensors, and modular quantum computers.

Fabrication and Characterization of Single-Crystal Diamond Membranes for Quantum Photonics with Tunable Microcavities.

The development of quantum technologies is one of the big challenges in modern research. A crucial component for many applications is an efficient, coherent spin–photon interface, and coupling single-color centers in thin diamond membranes to a microcavity is a promising approach. To structure such micrometer thin single-crystal diamond (SCD) membranes with a good quality, it is important to minimize defects originating from polishing or etching procedures. Here, we report on the fabrication of SCD membranes, with various diameters, exhibiting a low surface roughness down to 0.4 nm on a small area scale, by etching through a diamond bulk mask with angled holes. A significant reduction in pits induced by micromasking and polishing damages was accomplished by the application of alternating Ar/Cl2 + O2 dry etching steps. By a variation of etching parameters regarding the Ar/Cl2 step, an enhanced planarization of the surface was obtained, in particular, for surfaces with a higher initial surface roughness of several nanometers. Furthermore, we present the successful bonding of an SCD membrane via van der Waals forces on a cavity mirror and perform finesse measurements which yielded values between 500 and 5000, depending on the position and hence on the membrane thickness. Our results are promising for, e.g., an efficient spin–photon interface.

Initialization and Readout of Nuclear Spins via a Negatively Charged Silicon-Vacancy Center in Diamond.

In this Letter, we demonstrate initialization and readout of nuclear spins via a negatively charged silicon-vacancy (SiV) electron spin qubit. Under Hartmann-Hahn conditions the electron spin polarization is coherently transferred to the nuclear spin. The readout of the nuclear polarization is observed via the fluorescence of the SiV. We also show that the coherence time of the nuclear spin (6ms) is limited by the electron spin-lattice relaxation due to the hyperfine coupling to the electron spin. This Letter paves the way toward realization of building blocks of quantum hardware with an efficient spin-photon interface based on the SiV color center coupled to a long lasting nuclear memory.

Diamond photonics platform based on silicon vacancy centers in a single-crystal diamond membrane and a fiber cavity

We realize a potential platform for an efficient spin-photon interface, namely negatively-charged silicon-vacancy centers in a diamond membrane coupled to the mode of a fully-tunable, fiber-based, optical resonator. We demonstrate that introducing the thin ($\sim 200 \, \text{nm}$), single crystal diamond membrane into the mode of the resonator does not change the cavity properties, which is one of the crucial points for an efficient spin-photon interface. In particular, we observe constantly high Finesse values of up to $3000$ and a linear dispersion in the presence of the membrane. We observe cavity-coupled fluorescence froman ensemble of SiV$^{-}$ centers with an enhancement factor of $\sim 1.9$. Furthermore from our investigations we extract the ensemble absorption and extrapolate an absorption cross section of $(2.9 \, \pm \, 2) \, \cdot \, 10^{-12} \, \text{cm}^{2}$ for a single SiV$^{-}$ center, much higher than previously reported.

Characterization of the Si : Se+ Spin-Photon Interface

Silicon is the most developed electronic and photonic technological platform and hosts some of the highest-performance spin and photonic qubits developed to date. A hybrid quantum technology harnessing an efficient spin-photon interface in silicon would unlock considerable potential by enabling ultra-long-lived photonic memories, distributed quantum networks, microwave to optical photon converters, and spin-based quantum processors, all linked using integrated silicon photonics. However, the indirect bandgap of silicon makes identification of efficient spin-photon interfaces nontrivial. Here we build upon the recent identification of chalcogen donors as a promising spin-photon interface in silicon. We determined that the spin-dependent optical degree of freedom has a transition dipole moment stronger than previously thought (here 1.96(8) Debye), and the T1 spin lifetime in low magnetic fields is longer than previously thought (> 4.6(1.5) hours). We furthermore determined the optical excited state lifetime (7.7(4) ns), and therefore the natural radiative efficiency (0.80(9) %), and by measuring the phonon sideband, determined the zero-phonon emission fraction (16(1) %). Taken together, these parameters indicate that an integrated quantum optoelectronic platform based upon chalcogen donor qubits in silicon is well within reach of current capabilities.

Deterministic entanglement between a propagating photon and a singlet-triplet qubit in an optically active quantum dot molecule

Two-electron charged self-assembled quantum dot molecules exhibit a decoherence-avoiding singlet-triplet qubit subspace and an efficient spin-photon interface. We demonstrate quantum entanglement between emitted photons and the spin-qubit after the emission event. We measure the overlap with a fully entangled state to be $69.5\pm2.7\,\%$, exceeding the threshold of $50\,\%$ required to prove the non-separability of the density matrix of the system. The photonic qubit is encoded in two photon states with an energy difference larger than the timing resolution of existing detectors. We devise a novel heterodyne detection method, enabling projective measurements of such photonic color qubits along any direction on the Bloch sphere.

Generation of heralded entanglement between distant hole spins

Quantum entanglement emerges naturally in interacting quantum systems and plays a central role in quantum information processing. Remarkably, it is possible to generate entanglement even in the absence of direct interactions: provided that which path information is erased, weak spin-state dependent light scattering can be used to project two distant spins onto a maximally entangled state upon detection of a single photon. Even though this approach is necessarily probabilistic, successful generation of entanglement is heralded by the photon detection event. Here, we demonstrate heralded quantum entanglement of two quantum dot heavy-hole spins separated by 5 meters using single-photon interference. Thanks to the long coherence time of hole spins and the efficient spin-photon interface provided by self-assembled quantum dots embedded in leaky microcavity structures, we generate 2300 entangled spin pairs per second, which represents an improvement approaching three orders of magnitude as compared to prior experiments. Delayed two-photon interference scheme we developed allows for efficient verification of quantum correlations. Our results lay the groundwork for the realization of quantum networks in semiconductor nanostructures. Combined with schemes for transferring quantum information to a long-lived memory qubit, fast entanglement generation we demonstrate could also impact quantum repeater architectures.

Coherent control of single spins in silicon carbide at room temperature.

Spins in solids are cornerstone elements of quantum spintronics. Leading contenders such as defects in diamond or individual phosphorus dopants in silicon have shown spectacular progress, but either lack established nanotechnology or an efficient spin/photon interface. Silicon carbide (SiC) combines the strength of both systems: it has a large bandgap with deep defects and benefits from mature fabrication techniques. Here, we report the characterization of photoluminescence and optical spin polarization from single silicon vacancies in SiC, and demonstrate that single spins can be addressed at room temperature. We show coherent control of a single defect spin and find long spin coherence times under ambient conditions. Our study provides evidence that SiC is a promising system for atomic-scale spintronics and quantum technology.