Cyclotron And Radioisotope Center Research Articles

Monte Carlo modelling of cyclotron and radioisotope center (CYRIC) at Tohoku University: a radiation protection study

Protection against ionizing radiations is important in laboratories with radioactive materials and high energy cyclotron beams. The Cyclotron and Radioisotope Center (CYRIC) located in Tohoku University in Miyagi prefecture, Japan and is a well-known nuclear science laboratory with cyclotron beams and substantial number of high activity radioactive materials. Considering this, it is important to perform complete radiation transport computations to ensure the safety of non-occupational and occupational workers. In the present work, we have developed a complete 3-dimensional model of the main cyclotron building and radiation labs using Monte Carlo method. We have found that the dispersed photons and neutrons inside and in the surrounding of the CYRIC building pose no significant risk to occupational and non-occupational workers. The present work and the developed models would be useful in the field of radiation protection.

An accelerator experiment for junior and senior high school students to improve students’ involvement in fundamental physics

In Japan, research activities by junior and senior high school students show an upward trend. However, there are limited examples of research activities in the field of elementary particles and atoms. This is due to the difficulty associated with procuring research tools such as accelerators or particle detectors. Therefore, we hosted the ‘Accel Kitchen’ in 2018 and 2019 at the Cyclotron and Radioisotope Center (CYRIC) in Tohoku University where junior and senior high school students could participate in ongoing research of particle and atomic physics. At each workshop, 12 junior and senior high school students participated in the beam experiment, including the production of francium atoms (Fr) by the fusion reaction of oxygen and gold, optimizing the transport of the ion beam and identifying the alpha decay nuclei, and laser trapping of Fr for two days. Each group that was involved in the experiment was supported by researchers and university students who acted as mentors. This was the first opportunity for junior and senior high school students to know about the particle beam experiment in Japan.

Two-dimensional beam profile monitor for the detection of alpha-emitting radioactive isotope beam

Ions with similar charge-to-mass ratios cannot be separated from existing beam profile monitors (BPMs) in nuclear facilities in which low-energy radioactive ions are produced due to nuclear fusion reactions. In this study, we developed a BPM using a microchannel plate and a charge-coupled device to differentiate the beam profiles of alpha-decaying radioactive isotopes from other ions (reaction products) produced in a nuclear reaction. This BPM was employed to optimize the low-energy radioactive francium ion (Fr+) beam developed at the Cyclotron and Radioisotope Center (CYRIC), Tohoku University, for electron permanent electric dipole moment (e-EDM) search experiments using Fr atoms. We demonstrated the performance of the BPM by separating the Fr+ beam from other reaction products produced during the nuclear fusion reaction of an oxygen (18O) beam and gold (197Au) target. However, as the mass of Au is close to that of Fr, separating the ions of these elements using a mass filter is a challenge, and a dominant number of Au+ renders the Fr+ beam profile invisible when using a typical BPM. Therefore, by employing the new BPM, we could successfully observe the Fr+ beam and other ion beams distinctly by measuring the alpha decay of Fr isotopes. This novel technique to monitor the alpha-emitting radioactive beam covers a broad range of lifetimes, for example, from approximately 1 s to 10 min, and can be implemented for other alpha-emitter beams utilized for medical applications.

Radiation hardness of the low gain avalanche diodes developed by NDL and IHEP in China

This paper studies the radiation hardness of low gain avalanche detector (LGAD) developed by the Novel Device Laboratory (NDL) in Beijing and the Institute of High Energy Physics (IHEP) of Chinese Academy of Sciences, in the context of an upgrade project of the ATLAS detector for the high luminosity phase of LHC. NDL LGAD sensors with different layouts, epitaxial resistivity and doping profile were irradiated up to 1.02 × 1015 neq/cm2 by 70 MeV protons at Cyclotron and Radioisotope Center (CYRIC). The timing resolution of NDL LGAD sensors reached 50 ps and the collected charge reached 3 - 4 fC after irradiation.

Novel multi-layer plastic-scintillator-based solid active proton target for inverse-kinematics experiments

We have constructed and tested a novel plastic-scintillator-based solid-state active proton target for use in nuclear spectroscopic studies with nuclear reactions induced by an ion beam in inverse kinematics. The active target system, named Stack Structure Solid organic Scintillator Active Target (S4AT), consists of five layers of plastic scintillators, each with a 1-mm thickness. To determine the reaction point in the thickness direction, we exploit the difference in the energy losses due to the beam particle and the charged reaction product(s) in the scintillator material. S4AT offers the prospect of a relatively thick target while maintaining a good energy resolution. By considering the relative energy loss between different layers, the energy loss contributed by coincident unreacted beam particles can be eliminated. Such a procedure, made possible by the multi-layer structure, is essential to eliminate the contribution from coincident unreacted beam particles, thus enabling its operation at a moderate beam intensity of up to a few Mcps. We evaluated the performance of S4AT by measuring the elastic proton–proton scattering using a 70-MeV proton beam at Cyclotron and Radioisotope Center (CYRIC), Tohoku University.

Development of a neutron detector with a high position resolution at intermediate energies

A high position resolution neutron detector for time-of-flight measurements is being developed to measure the (p,pn) reaction in inverse kinematics with an excitation energy resolution of 1 MeV at the RIKEN RI Beam Factory. In this study, a new method based on the segmentation of the neutron detector part is employed to achieve a position resolution on the order of mm with a prototype neutron detector. The prototype detector consists of 8 × 8 scintillating fibers, two multi-anode photomultiplier tubes (PMTs) and two light guides. The scintillating fibers have a cross sectional area of 3.75×3.75mm2. The prototype’s performance is studied using the neutron and proton beams provided at the Cyclotron and Radioisotope Center (CYRIC), Tohoku University and the Research Center for Nuclear Physics (RCNP), Osaka University. It is confirmed that the hit pattern analysis correctly recognizes the neutron detection position within the fiber size of 3.75 mm. The obtained TOF resolution of 350 ps (FWHM), lateral position resolution of 2.5 mm (FWHM), and longitudinal position resolution of 50–60 mm (FWHM) satisfy the requirements to achieve an excitation energy resolution of 1 MeV. The typical detection efficiency is ∼2.0% for a neutron with a kinetic energy of 50–200 MeV. The detailed investigation of the detection efficiency in conjunction with the neutron hit position reveals the existence of the non-uniformity of the efficiency. It is shown that the non-uniformity can be mitigated by reducing the threshold level, and by increasing the detector size. For a larger neutron detector, based on the design of the prototype detector, the non-uniformity will thus be negligible.

Test beam evaluation of newly developed n-in-p planar pixel sensors for use in a high radiation environment

Radiation-tolerant n-in-p planar pixel sensors have been under development in cooperation with Hamamatsu Photonics K.K. (HPK). This is geared towards applications in high-radiation environments, such as for the future Inner Tracker (ITk) placed in the innermost part of the ATLAS detector in the high luminosity LHC (HL-LHC) experiment. Prototypes of those sensors have been produced, irradiated, and evaluated over the last few years. In the previous studies, it was reported that significant drops in the detection efficiency were observed after irradiation, especially under bias structures. The bias structures are made up of poly-Si or Al bias rails and poly-Si bias resistors. The structure is implemented on the sensors to allow quality checks to be performed before the bump-bonding process, and to ensure that charge generated in floating pixels due to non-contacting or missing bump-bonds is dumped in a controlled way in order to avoid noise. To minimize the efficiency drop, several new pixel structures have been designed with bias rails and bias resistors relocated. Several test beams have been carried out to evaluate the drops in the detection efficiency of the new sensor structures after irradiation. Newly developed sensor modules were irradiated with proton-beams at the Cyclotron and Radio-Isotope Center (CYRIC) in Tohoku University to see the effect of sensor-bulk damage and surface charge-up. An irradiation with γ-rays was also carried out at Takasaki Advanced Radiation Research Center, with the goal of decoupling the effect of surface charge-up from that of bulk damage. Those irradiated sensors have been evaluated with particle beams at DESY and CERN. Comparison between different sensor structures confirmed significant improvements in minimizing efficiency loss under the bias structures after irradiation. The results from γ-irradiation also enabled cross-checking the results of a semiconductor technology simulation program (TCAD).

Enhanced spin-dependent parity-nonconservation effect in the7sS1/22→6dD5/22transition in Fr: A possibility for unambiguous detection of the nuclear anapole moment

Employing the relativistic coupled-cluster method, comparative studies of the parity non-conserving electric dipole amplitudes for the $7s \ ^2S_{1/2} \rightarrow 6d \ ^2D_{5/2}$ transitions in $^{210}$Fr and $^{211}$Fr isotopes have been carried out. It is found that these transition amplitudes, sensitive only to the nuclear spin dependent effects, are enhanced by more than 3 orders compared to the low-lying $S-D_{5/2}$ transitions in Ba$^+$ and Ra$^+$ owing to the very large contributions from the electron core-polarization effects in Fr. This translates to a relatively large and, in principle, measurable induced light shift, which would be a signature of nuclear spin dependent parity nonconservation that is dominated by the nuclear anapole moment in a heavy atom like Fr. A plausible scheme to measure this quantity using the Cyclotron and Radioisotope Center (CYRIC) facility at Tohoku University has been outlined.

Restoration of accelerator facilities damaged by Great East Japan Earthquake at Cyclotron and Radioisotope Center, Tohoku University.

The Cyclotron and Radioisotope Center (CYRIC) of Tohoku University is a joint-use institution for education and research in a wide variety of fields ranging from physics to medicine. Accelerator facilities at the CYRIC provide opportunities for implementing a broad research program, including medical research using positron emission tomography (PET), with accelerated ions and radioisotopes. At the Great East Japan Earthquake on March 11, 2011, no human injuries occurred and a smooth evacuation was made in the CYRIC, thanks to the anti-earthquake measures such as the renovation of the cyclotron building in 2009 mainly to provide seismic strengthening, fixation of shelves to prevent the falling of objects, and securement of the width of the evacuation route. The preparation of an emergency response manual was also helpful. However, the accelerator facilities were damaged because of strong shaking that continued for a few minutes. For example, two columns on which a 930 cyclotron was placed were damaged, and thereby the 930 cyclotron was inclined. All the elements of beam transport lines were deviated from the beam axis. Some peripheral devices in a HM12 cyclotron were broken. Two shielding doors fell from the carriage onto the floor and blocked the entrances to the rooms. The repair work on the accelerator facilities was started at the end of July 2011. During the repair work, the joint use of the accelerator facilities was suspended. After the repair work was completed, the joint use was re-started at October 2012, one and a half years after the earthquake.

Search for a permanent EDM using laser cooled radioactive atom

An Electric Dipole Moment (EDM) of the elementary particle is a good prove to observe the phenomena beyond the Standard Model. A non-zero EDM shows the violation of the time reversal symmetry, and under the CPT invariance it means the CP violation. In paramagnetic atoms, an electron EDM results in an atomic EDM enhanced by the factor of the 3rd power of the charge of the nucleus due the relativistic effects. A heaviest alkali element francium (Fr), which is the radioactive atom, has the largest enhancement factor K ∼ 895. Then, we are developing a high intensity laser cooled Fr factory at Cyclotron and Radioisotope Center (CYRIC), Tohoku University to perform the search for the EDM of Fr with the accuracy of 10−29 e · cm. The important points to overcome the current accuracy limit of the EDM are to realize the high intensity Fr source and to reduce the systematic error due to the motional magnetic field and inhomogeneous applied field. To reduce the dominant component of the systematic errors mentioned above, we will confine the Fr atoms in the small region with the Magneto-Optical Trap and optical lattice using the laser cooling and trapping techniques. The construction of the experimental apparatus is making progress, and the new thermal ionizer already produces the Fr of ∼106 ions/s with the primary beam intensity 200 nA. The developments of the laser system and optical equipments are in progress, and the present status and future plan of the experimental project is reported.

CHIRALITY IN THE MASS 80 REGION: 79Kr

The high spin states of 79 Kr were studied via the 70 Zn (13 C , 4 n ) reaction to search for chiral doublet bands based on the three-quasi-particle configuration, πg9/22 ⊗ νg9/2-1. The 13 C beam of 65 MeV was provided by the 930 AVF Cyclotron at CYclotron and RadioIsotope Center (CYRIC) facility at Tohoku University. The triple coincidence γ rays were detected by the Hyperball2 array. The side band structure to the πg9/22 ⊗ νg9/2-1 yrast band has been identified in 79 Kr . Spin and parity assignments are made based on the DCO ratio and linear polarization analysis.

Installation and application of an intense 7Li(p,n) Neutron source for 20-90 MeV region

An intense (7)Li(p,n) neutron source was installed with the K = 110-MeV azimuthally varying field (AVF) cyclotron at the Cyclotron and Radioisotope Center (CYRIC), Tohoku University, by employing a special arrangement to allow a short target-sample distance down to 1 m. The source can deliver a neutron flux around 1.5 x 10(6) n cm(-2) s(-1) with a lithium target of thickness equivalent to 2-MeV energy loss and 3-microA proton beam, which is the highest intensity in the world. The source is successfully used for (1) measurement of neutron cross sections relevant to radiation safety and radiation effect and (2) semiconductor irradiation test for single-event effect and (3) characterisation of neutron detectors and dosemeters.

Measurement of neutron activation cross sections for major elements of water, air and soil between 30 and 70 MeV

Neutron activation cross sections between 30 and 70 MeV were measured by the activation method using a semi-monoenergetic neutron field settled at the AVF cyclotron of the Cyclotron and Radioisotope Center(CYRIC), Tohoku University. Natural samples of N, O, Si, Na, Ca and Mg which are the major elements of water, air and soil were irradiated in this neutron field generated through the 7Li(p,n)7Be reaction by 30, 35,40, 50,60 and 70 MeV protons on thin Li target. Neutron yields were measured with the time-of-flight method using a calibrated NE213 organic liquid scintillator. From the induced activities measured with the HPGe detectors, we estimated the excitation functions of 15 cross sections.

Overview of recent experimental works on high energy neutron shielding

Several experiments on high energy neutron shielding have recently been performed using medium to high energy accelerators of energies above 20 MeV. Below 100 MeV, the benchmark experiments have been done using 25 and 35 MeV p-Li quasi-monoenergetic neutrons at the Cyclotron and Radioisotope Center (CYRIC), Tohoku University, Japan, 43 and 68 MeV p-Li quasi-monoenergetic neutrons at the Azimuthally Varying Field (AVF) cyclotron facility, TIARA of Japan Atomic Energy Research Institute (JAERI). Above 100 MeV, the neutron shielding experiments have been done using 800 MeV protons at ISIS, Rutherford Appleton laboratory (RAL), England, 400 MeV/nucleon carbon ions at the heavy ion medical accelerator facility, HIMAC of National Institute of Radiological Sciences (NIBS), Japan, 500 MeV protons at the spallation neutron source facility, KEK spallation neutron source facility (KENS) of High Energy Accelerator Research Organization (KEK), Japan, 500 MeV protons at the accelerator facility, TRIUMF, Canada, 1.6 to 24 GeV protons at the Alternating Gradient Synchrotron (AGS), Brookhaven National Laboratory (BNL), U.S.A., 28.7 GeV electrons at the Stanford Linear Accelerator Center (SLAG), U.S.A., 800 MeV protons at the Los Alamos Neutron Science Center (LANSCE), Los Alamos National Laboratory (LANL), U.S.A., 120, 205 GeV/c protons and 160 GeV/nucleon lead ions at the European Organization for Nuclear Research (CERN), Switzerland, 230 MeV protons at the Loma Linda University Medical Center, U.S.A., 200 MeV protons at the Orsay Proton Therapy Center, France. In this review paper, the outlines of these deep penetration experiments are summarized together with the neutron detection techniques.

Measurement of Residual Radioactivity of Machine Elements and Concrete on the Cyclotron Decommissioning

The AVF cyclotron was decommissioned at the CYRIC (Cyclotron and Radioisotope Center) of Tohoku University for installing a new cyclotron. With this decommissioning, we sampled the main part of machine elements such as accelerator box, acceleration electrodes, magnet yoke, and the concrete of the cyclotron vault which had been strongly activated for about 20 years operation. We measured the residual radioactivities of these samples with a high pure Ge detector and identified the nuclides of 22Na, 46Sc, 51Cr, 54Mn,59Fe, 56Co, 58Co, 60Co, 65Zn, 134Cs, 152Eu from the gamma-ray spectra and half-lives. The peak counts per unit time (cps) were converted into radioactivities per unit mass (Bq/g) with the Ge peak efficiency In addition, we measured the spatial dose distribution in the cyclotron room and the surface dose of electromagnet with a Nal (Tl) survey meter. These results will be useful for the future accelerator decommissioning.

FACILITY OF PIXE ANALYSIS AT TOHOKU UNIVERSITY

PIXE research at the 4.5-MV Dynamitron laboratory of the Faculty of Engineering, Tohoku University started as a joint project between Cyclotron and Radioisotope Center(CYRIC), Tohoku University, and the Dynamitron laboratory. The PIXE equipments including vertical beam in air PIXE system called ViaPIXE was installed at a vacant beam course of the Dynamitron laboratory. Some PIXE experiments conducted at this facility as well future PIXE research in this laboratory are briefly described.