Superposition Of Coherent States Research Articles

A unified theory of tunneling times promoted by Ramsey clocks.

What time does a clock tell after quantum tunneling? Predictions and indirect measurements range from superluminal or instantaneous tunneling to finite durations, depending on the specific experiment and the precise definition of the elapsed time. Proposals and implementations use the atomic motion to define this delay, although the inherent quantum nature of atoms implies a delocalization and is in sharp contrast to classical trajectories. Here, we rely on an operational approach: We prepare atoms in a coherent superposition of internal states and study the time read-off via a Ramsey sequence after the tunneling process without the notion of classical trajectories or velocities. Our operational framework (i) unifies definitions of tunneling delay within one approach, (ii) connects the time to a frequency standard given by a conventional atomic clock that can be boosted by differential light shifts, and (iii) highlights that there exists no superluminal or instantaneous tunneling.

Coherent x-ray spontaneous emission spectroscopy of conical intersections.

Conical intersections are known to play a vital role in many photochemical processes. The breakdown of the Born-Oppenheimer approximation in the vicinity of a conical intersection causes exciting phenomena, such as the ultrafast radiationless decay of excited states. The passage of a molecule through a conical intersection creates a coherent superposition of electronic states via nonadiabatic couplings. Detecting this coherent superposition may serve as a direct probe of the conical intersection. In this paper, we theoretically demonstrate the use of coherent spontaneous emission in samples with long-range order for probing the occurrence of a conical intersection in a molecule. Our simulations show that the spectrum contains clear signatures of the created coherent superposition of electronic states. We investigate the bandwidth requirements for the x-ray probes, which influence the observation of coherent superposition generated by the conical intersection.

Elastic bit and Berry phase: Investigating topological phenomena in a classical granular network

This study investigates the Berry phase, a key concept in classical and quantum physics, and its manifestation in a classical system. We achieve controlled accumulation of the Berry phase by manipulating the elastic bit (a classical analogue to a quantum bit) in an externally driven, homogeneous, spherical, nonlinear granular network. This is achieved through the classical counterpart of quantum coherent superposition of states. The elastic bit's state vectors are navigated on the Bloch sphere using external drivers' amplitude, phase, and frequency, yielding specific Berry phases. These phases distinguish between trivial and nontrivial topologies of the elastic bit, with the zero Berry phase indicating pure states of the linearized granular system and the nontrivial π phase representing equal superposed states. Other superposed states acquire different Berry phases. Crucially, these phases correlate with the structure's eigenmode vibrations: trivial phases align with distinct, in-phase, or out-of-phase eigenmodes, while nontrivial phases correspond to coupled vibrations where energy is shared among granules, alternating between oscillation and rest. Additionally, we explore Berry's phase generalizations for non-cyclic evolutions. This research paves the way for advanced quantum-inspired sensing and computation applications by utilizing and controlling the Berry phase.

Nonadiabatic dynamics with classical trajectories: The problem of an initial coherent superposition of electronic states.

Advances in coherent light sources and development of pump-probe techniques in recent decades have opened the way to study electronic motion in its natural time scale. When an ultrashort laser pulse interacts with a molecular target, a coherent superposition of electronic states is created and the triggered electron dynamics is coupled to the nuclear motion. A natural and computationally efficient choice to simulate this correlated dynamics is a trajectory-based method where the quantum-mechanical electronic evolution is coupled to a classical-like nuclear dynamics. These methods must approximate the initial correlated electron-nuclear state by associating an initial electronic wavefunction to each classical trajectory in the ensemble. Different possibilities exist that reproduce the initial populations of the exact molecular wavefunction when represented in a basis. We show that different choices yield different dynamics and explore the effect of this choice in Ehrenfest, surface hopping, and exact-factorization-based coupled-trajectory schemes in a one-dimensional two-electronic-state model system that can be solved numerically exactly. This work aims to clarify the problems that standard trajectory-based techniques might have when a coherent superposition of electronic states is created to initialize the dynamics, to discuss what properties and observables are affected by different choices of electronic initial conditions and to point out the importance of quantum-momentum-induced electronic transitions in coupled-trajectory schemes.

Second-scale rotational coherence and dipolar interactions in a gas of ultracold polar molecules

Ultracold polar molecules combine a rich structure of long-lived internal states with access to controllable long-range anisotropic dipole–dipole interactions. In particular, the rotational states of polar molecules confined in optical tweezers or optical lattices may be used to encode interacting qubits for quantum computation or pseudo-spins for simulating quantum magnetism. As with all quantum platforms, the engineering of robust coherent superpositions of states is vital. However, for optically trapped molecules, the coherence time between rotational states is typically limited by inhomogeneous differential light shifts. Here we demonstrate a rotationally magic optical trap for 87Rb133Cs molecules that supports a Ramsey coherence time of 0.78(4) s in the absence of dipole–dipole interactions. This is estimated to extend to >1.4 s at the 95% confidence level using a single spin-echo pulse. In our trap, dipolar interactions become the dominant mechanism by which Ramsey contrast is lost for superpositions that generate oscillating dipoles. By changing the states forming the superposition, we tune the effective dipole moment and show that the coherence time is inversely proportional to the strength of the dipolar interaction. Our work unlocks the full potential of the rotational degree of freedom in molecules for quantum computation and quantum simulation.

Coherent superposition of states in degenerate systems using zero-area pulses

The coherent superposition of states in degenerate quantum systems is investigated using detuned laser pulses in which the Rabi frequencies are time-dependent, and the pulse area is zero. In this study, a quantum system with an arbitrary number of degenerate states in the ground set as well as an arbitrary number of degenerate states in the exciting set is considered. We assume that all states in the ground set are coupled to the excited states using laser pulses such that the pulse area of Rabi frequency is zero, and all of them have the same time dependence. It is also assumed that all laser pulses are in a non-resonant condition with Bohr transitions, and all detunings are the same. We will show that by applying the appropriate temporal dependence for the pulses and the appropriate rate for the detunings, the population can be transferred from an arbitrary superposition from the ground states to a desired superposition from the excited states.

Semiclassical gravity beyond coherent states

We show that it is possible to still use semiclassical gravity together with quantum field theory beyond the regimes where the field state is coherent. In particular, we identify families of cat states (superposition of almost-distinguishable coherent states that have very non-classical features) for which the gravitational backreaction can be modeled by semiclassical gravity.

Conditional creation of superpositions of coherent states with an ineffective photon

The article shows that a single photon source and straightforward, purely optical processes can be used to produce a linear superposition of two macroscopically identifiable optical coherent states. A superposition of coherent states in a freely propagating optical field with high coherence amplitude can be generated via weak squeezing on a single photon, beam mixing with an auxiliary coherent state, and photon detection with imperfect threshold detectors. (α>2) and F=0.99, which is extremely precise. Our technique does not require a precise photon count, resolving measurements, or nonlinear Kerr-type interactions, in contrast to all existing schemes for obtaining such a state. It also exhibits some tolerance to inefficiencies in photon generation and is robust against detection of inefficiencies.

Coherence requirements for quantum communication from hybrid circuit dynamics

The coherent superposition of quantum states is an important resource for quantum information processing which distinguishes quantum dynamics and information from their classical counterparts. In this article we determine the coherence requirements to communicate quantum information in a broad setting encompassing monitored quantum dynamics and quantum error correction codes. We determine these requirements by considering hybrid circuits that are generated by a quantum information game played between two opponents, Alice and Eve, who compete by applying unitaries and measurements on a fixed number of qubits. Alice applies unitaries in an attempt to maintain quantum channel capacity, while Eve applies measurements in an attempt to destroy it. By limiting the coherence generating or destroying operations available to each opponent, we determine Alice’s coherence requirements. When Alice plays a random strategy aimed at mimicking generic monitored quantum dynamics, we discover a coherence-tuned phase transitions in entanglement and quantum channel capacity. We then derive a theorem giving the minimum coherence required by Alice in any successful strategy, and conclude by proving that coherence sets an upper bound on the code distance in any stabelizer quantum error correction code. Such bounds provide a rigorous quantification of the coherence resource requirements for quantum communication and error correction.

Probing the electron motion in molecules using forward-scattering photoelectron holography.

Charge migration initiated by the coherent superposition of several electronic states is a basic process in intense laser-matter interactions. Observing this process on its intrinsic timescale is one of the central goals of attosecond science. Here, using forward-scattering photoelectron holography we theoretically demonstrate a scheme to probe the charge migration in molecules. In our scheme, by solving the time-dependent Schrödinger equation, the photoelectron momentum distributions (PEMDs) for strong-field tunneling ionization of the molecule are obtained. For a superposition state, it is shown that an intriguing shift of the holographic interference appears in the PEMDs, when the molecule is aligned perpendicularly to the linearly polarized laser field. With the quantum-orbit analysis, we demonstrate that this shift of the interference fringes is caused by the time evolution of the non-stationary superposition state. By analyzing the dependence of the shift on the final parallel momentum of the electrons, the relative phase and the expansion coefficient ratio of the two electronic states involved in the superposition state are determined accurately. Our study provides an efficient method for probing the charge migration in molecules. It will facilitate the application of the forward-scattering photoelectron holography to survey the electronic dynamics in more complex molecules.

Simulation of quantum optics by coherent state decomposition

We introduce a framework for simulating quantum optics by decomposing the system into a finite rank (number of terms) superposition of coherent states. This allows us to define a resource theory, where linear optical operations are “free” (i.e., do not increase the rank), and the simulation complexity for an m-mode system scales quadratically in m, in stark contrast to the Hilbert space dimension. We outline this approach explicitly in the Fock basis, relevant in particular for Boson sampling, where the simulation time (space) complexity for computing output amplitudes, to arbitrary accuracy, scales as O(m2 2 n ) [O(m2 n )] for n photons distributed among m modes. We additionally demonstrate that linear optical simulations with the n photons initially in the same mode scales efficiently, as O(m2 n). This paradigm provides a practical notion of “non-classicality,” i.e., the classical resources required for simulation. Moreover, by making connections to the stellar rank formalism, we show this comes from two independent contributions, the number of single-photon additions and the amount of squeezing.

Bosonic Representation of Matrices and Angular Momentum Probabilistic Representation of Cyclic States.

The Jordan-Schwinger map allows us to go from a matrix representation of any arbitrary Lie algebra to an oscillator (bosonic) representation. We show that any Lie algebra can be considered for this map by expressing the algebra generators in terms of the oscillator creation and annihilation operators acting in the Hilbert space of quantum oscillator states. Then, to describe quantum states in the probability representation of quantum oscillator states, we express their density operators in terms of conditional probability distributions (symplectic tomograms) or Husimi-like probability distributions. We illustrate this general scheme by examples of qubit states (spin-1/2 su(2)-group states) and even and odd Schrödinger cat states related to the other representation of su(2)-algebra (spin-j representation). The two-mode coherent-state superpositions associated with cyclic groups are studied, using the Jordan-Schwinger map. This map allows us to visualize and compare different properties of the mentioned states. For this, the su(2) coherent states for different angular momenta j are used to define a Husimi-like Q representation. Some properties of these states are explicitly presented for the cyclic groups C2 and C3. Also, their use in quantum information and computing is mentioned.

Symmetry Breaking: A Classic Example of Quantum Interference Captured by Mixed Quantum/Classical Theory.

The phenomena of propensity and inverse propensity are explored using time-dependent mixed quantum classical theory, MQCT, in which the rotational motion of the molecule is treated quantum mechanically, whereas the scattering process is described classically. Good agreement with the results of accurate full-quantum calculations is reported for a closed shell approximation to the NO + Ar system. It is shown that MQCT reproduces both phenomena in a broad range of the final states of the molecule and for various initial rotational states, offering a unique time-dependent insight. It permits seeing that both propensity and inverse propensity occur due to efficient depopulation of some states at the early postcollisional stage of the scattering process, when the molecule exists in a coherent superposition of many excited states that span a very broad range of angular momentum quantum numbers, populated by an efficient stepladder process of many consecutive transitions with small Δj.

Massive particle interferometry with lattice solitons

We discuss an interferometric scheme employing interference of bright solitons formed as specific bound states of attracting bosons on a lattice. We revisit the proposal of Castin and Weiss [Phys. Rev. Lett. vol. 102, 010403 (2009)] for using the scattering of a quantum matter-wave soliton on a barrier in order to create a coherent superposition state of the soliton being entirely to the left of the barrier and being entirely to the right of the barrier. In that proposal, it was assumed that the scattering is perfectly elastic, i.e. that the center-of-mass kinetic energy of the soliton is lower than the chemical potential of the soliton. Here we relax this assumption: By employing a combination of Bethe ansatz and DMRG-based analysis of the dynamics of the appropriate many-body system, we find that the interferometric fringes persist even when the center-of-mass kinetic energy of the soliton is above the energy needed for its complete dissociation into constituent atoms.

Feedback Control of Quantum Systems to Stabilize Superposition States

As a specific trait of quantum mechanics, quantum superposition is exploited in many applications such as quantum computation. This paper proposes a feedback scheme to stabilize the desired quantum superposition states. To this aim, a new factorization is derived for the stochastic master equation of a quantum system which is driven by the field in the superposition of coherent states. Then, a feedback scheme is proposed, which consists of a quantum system driven by the field in the superposition of coherent states and a classical feedback channel proportional to the observations of a Homodyne detector. Afterward, the quantum filter of the closed loop system is attained using the SLH framework. Finally, the factorization of the closed loop quantum filter is obtained and the control law is calculated such that the proposed factorization satisfies the stabilization condition. Finally, as an example, the control method is simulated for a two-level atom and the stabilization of the superposition states is achieved.

Spatially structured optical effects in semiconductor quantum dots via biexciton coherence

In this paper, we study the spatially structured optical effects that occur when weak laser lights interact with coherently prepared semiconductor quantum dots (SQDs). Initially, the SQD is prepared in a coherent superposition of the lower exciton states. By utilizing two weak optical vortex fields that couple to a biexciton state, we observe spatially dependent effects of the absorption of probe fields. Using the well-established Maxwell–Bloch equations, we analyze the generation of composite optical vortex beams within this system. Our investigation revolves around the formation of different types of spatially dependent beams, exploring their properties and characteristics. Additionally, the transfer of optical vortices through the parametric generation process is examined, for the case where only one vortex beam is present at the beginning of the medium. This study provides insights into the spatially structured optical phenomena in coherently prepared SQDs and contributes to the understanding of light–matter interactions in such systems.

Superoscillations and Fock spaces

In this paper we use techniques in Fock spaces theory and compute how the Segal-Bargmann transform acts on special wave functions obtained by multiplying superoscillating sequences with normalized Hermite functions. It turns out that these special wave functions can be constructed also by computing the approximating sequence of the normalized Hermite functions. First, we start by treating the case when a superoscillating sequence is multiplied by the Gaussian function. Then, we extend these calculations to the case of normalized Hermite functions leading to interesting relations with Weyl operators. In particular, we show that the Segal-Bargmann transform maps superoscillating sequences onto a superposition of coherent states. Following this approach, the computations lead to a specific linear combination of the normalized reproducing kernels (coherent states) of the Fock space. As a consequence, we obtain two new integral Bargmann-type representations of superoscillating sequences. We also investigate some results relating superoscillation functions with Weyl operators and Fourier transform.

Time evolution of quantum correlations induced by atomic state superpositions

In this article, we study the time evolution of Gaussian quantum correlations induced by the superposition of atomic states. Photon-based quantum information and communication are powerful and suitable because the relevant physical mechanisms, the high combination rate of photons, and the sources of coherence can be understood and easily modeled. To this end, coupled photon pairs produced by coherent superposition of atomic states in an atomic laser and influences of spontaneous atomic decay due to vacuum field fluctuations have been considered. The dynamics of the quantum system leads to temporal quantum correlations such as quantum discord, quantum entanglement, and quantum steering, which are treated by the density operator approach. It was found that the generated photon pairs are completely in a separable state in the initial phase of the dynamical processes. The quantum coherences must be given sufficient time to generate quantum correlations that saturate after very short time scales. The strength of these quantum correlations has been improved by increasing the number of superposed atoms per unit of time. In particular, two-way quantum steering, which is a guarantee for the existence of quantum discord and quantum entanglement, can be achieved by increasing the atom injection rate from 10 kHz to 100 kHz when the probability of finding atoms in the excited state is 45%.

Asynchronous measurement-device-independent quantum key distribution with hybrid source.

The linear constraint of secret key rate capacity is overcome by the twin-field quantum key distribution (QKD). However, the complex phase-locking and phase-tracking technique requirements throttle the real-life applications of the twin-field protocol. The asynchronous measurement-device-independent (AMDI) QKD, also called the mode-pairing QKD, protocol can relax the technical requirements and keep the similar performance of the twin-field protocol. Here, we propose an AMDI-QKD protocol with a nonclassical light source by changing the phase-randomized weak coherent state to a phase-randomized coherent-state superposition in the signal state time window. Simulation results show that our proposed hybrid source protocol significantly enhances the key rate of the AMDI-QKD protocol, while exhibiting robustness to imperfect modulation of nonclassical light sources.

Enhancement of dynamical entanglement in a dispersive two-mode Jaynes–Cummings model via superposition of photon-added pair coherent state

In this paper, we introduce a new non-Gaussian state called superposition of photon-added pair coherent state (SPAPCS) by superposition addition of photons to two modes of a pair coherent state (PCS). It is demonstrated that the SPAPCS has an enhanced non-Gaussian property by testing its Wigner function when increasing the number of photons added to two modes of the PCS. We use the field as a SPAPCS to study a dynamical entanglement in a dispersive two-mode Jaynes–Cummings model in dissipation atom-field interaction. We detect the dynamical entanglement degrees of the global system and subsystems by using the linear entropy criteria. The obtained results show the dynamical entanglement degrees can be enhanced by the phase damping effect as well as the superposition adding photons to two modes of the field in SPAPCS.