Coherent Sources Research Articles

Barium Chalcogenide Crystals: A Review

In recent decades, new nonlinear optical materials have been actively developed to create coherent tunable light sources in the mid-infrared (mid-IR) part of the spectrum used in a variety of scientific fields. In the present review, the main attention is focused on barium chalcogenide crystals, including their linear and nonlinear optical properties, laser-induced damage threshold (LIDT), and frequency down-conversion.

Electric and magnetic metal-insulator-metal metasurfaces in the mid-infrared based on Babinet’s, Lorentz’s, and Kirchhoff’s principles

Metasurfaces can extend the optical properties of conventional materials by structuring surfaces at a subwavelength scale. These artificial subwavelength surfaces mimic the physics of conventional materials and can, in principle, be designed to provide novel optical material properties. Metal-insulator-metal (MIM) antenna metasurfaces are among the most widely used as ideal absorbers and emitters. In this work, we present MIM metasurfaces in the mid-infrared that comply in the electric and magnetic forms of Babinet’s, Lorentz’s, and Kirchhoff’s principles. To verify the validity of Babinet's, Lorentz's, and Kirchhoff's MIM metasurfaces, we computed their reflection and absorption spectra as well as electric and magnetic field maps. We found that even in the presence of graphene on top of the electric and magnetic MIM metasurfaces, these principles still hold qualitatively. However, the excitation of gap surface plasmon polaritons (SPPs) and graphene SPPs fails to comply quantitatively. Additionally, we fabricated the MIM metasurfaces and used imaging Fourier transform infrared spectroscopy in the mid infrared spectrum to validate them. Finally, we explore the potentials and limits of the use of graphene as tunability material, with a tunability bandwidth up to 0.6 µm. Our findings can be applied to the development of electric and magnetic frequency selectivity metasurfaces, polarizers, coherent thermal sources, and detectors.

Mean-field equation for phase-modulated optical parametric oscillator

The widely established techniques for the generation of ultrashort optical pulses rely on passive mode locking of lasers, with the output pulse duration and emission spectrum determined by the intrinsic lifetime of laser transition in the gain medium. Due to the instantaneous nature of nonlinear gain, optical parametric oscillators (OPOs) are capable of generating optical radiation in all timescales from continuous-wave (cw) to ultrashort femtosecond regime, if driven by laser pump sources in the corresponding time domain. In the ultrashort timescale, operation of OPOs conventionally relies on mode-locked pump lasers, with the concomitant disadvantages of large footprint and high cost. At the same time, the lack of gain storage mandates the use of synchronous pumping, resulting in increased complexity. In this paper, we present the concept of phase-modulated OPO driven by cw pump laser. The approach overcomes the traditional drawbacks of ultrafast OPOs, enabling femtosecond pulse generation without the need for synchronous pumping, resulting in a simplified, compact, and cost-effective architecture using cw input pump lasers. We derive a mean-field equation for a degenerate χ(2) OPO driven by a cw laser with intracavity electro-optic modulator (EOM), and also including dispersion compensation. The equation predicts the formation of stable femtosecond pulses (<200fs), in both normal and anomalous dispersion regimes, with a controllable repetition rate determined by the frequency of the EOM. The remarkable functionality of the proposed scheme paves the way for the development of an alternative class of widely tunable coherent femtosecond light sources in both bulk and integrated format based on χ(2) OPOs using cw pump lasers. Published by the American Physical Society 2024

Monolithic PMN-39PT nanograting-assisted second harmonic generation enhancement.

Second harmonic generation plays a vital role in frequency conversion which mutually promotes the laser technology and allows the wavebands extension of new coherent source. The monolithic crystals are supposed to be a superior choice for harmonic generation due to long interaction distance, however, the phase-mismatch brought a sharp reduction in the conversion efficiency. Although birefringent phase-matching and quasi-phase-matching techniques are commonly utilized to fill the phase gap in monolithic crystals, these techniques are limited by the natural refractive index of crystal and the domain engineering, respectively. In recent years, subwavelength structures evolve as a flexible scheme to realize phase matching by engineering the geometry features of crystals. Here, structured nanogratings are designed and fabricated on a monolithic PMN-39PT (Pb(Mg1/3Nb2/3)O3-0.39PbTiO3) substrate, a novel ferroelectric crystal with promising optical prospect, for enhancing second harmonic generation, where birefringent or quasi phase-matching is hard to achieve. The nanograting-assisted second harmonic generation enhancement is observed which is not limited by the availability of thin crystalline films. Meanwhile, a boost in the second harmonic signal synchronously promotes the cascading third harmonic generation. This method may provide an alternative solution for enhanced harmonic generation on monolithic substrates and develop potential nonlinear optical materials for frequency conversion.

Spatially nonuniformly correlated vortex beams and their arrays

We introduce a class of partially coherent sources with spatially nonuniformly correlation properties and an off-axis helicoidal phase. It is shown that the unique correlation and phase properties of such sources lead to radiated fields with extraordinary propagation characteristics, such as dark hollow with zero central intensity, self-focusing and lateral self-shifting light intensity. Based on such novel random sources, two types of nonuniformly correlated vortex beam arrays with radial and rectangular symmetry are explored. Analytical and numerical investigations for the evolutions of such light fields are made by the model decomposition representation of correlation function and fast Fourier transform method. The results demonstrate new opportunities for modeling off-axis self-focusing vortex beams and other beam shaping applications by joint modulation of coherence and phase.

Ultrahigh-brightness 50 MeV electron beam generation from laser wakefield acceleration in a weakly nonlinear regime

We propose an efficient scheme to produce ultrahigh-brightness tens of MeV electron beams by designing a density-tailored plasma to induce a wakefield in the weakly nonlinear regime with a moderate laser energy of 120 mJ. In this scheme, the second bucket of the wakefield can have a much lower phase velocity at the steep plasma density down-ramp than the first bucket and can be exploited to implement longitudinal electron injection at a lower laser intensity, leading to the generation of bright electron beams with ultralow emittance together with low energy spread. Three-dimensional particle-in-cell simulations are carried out and demonstrate that high-quality electron beams with a peak energy of 50 MeV, ultralow emittance of ∼28 nm rad, energy spread of 1%, charge of 4.4 pC, and short duration less than 5 fs can be obtained within a 1-mm-long tailored plasma density, resulting in an ultrahigh six-dimensional brightness B6D,n of ∼2 × 1017 A/m2/0.1%. By changing the density parameters, tunable bright electron beams with peak energies ranging from 5 to 70 MeV, a small emittance of ≤0.1 mm mrad, and a low energy spread at a few-percent level can be obtained. These bright MeV-class electron beams have a variety of potential applications, for example, as ultrafast electron probes for diffraction and imaging, in laboratory astrophysics, in coherent radiation source generation, and as injectors for GeV particle accelerators.

Electrical polarization switching of perovskite polariton laser

Abstract Optoelectronic and spinoptronic technologies benefit from flexible and tunable coherent light sources combining the best properties of nano- and material-engineering to achieve favorable properties such as chiral lasing and low threshold nonlinearities. In this work we demonstrate an electrically wavelength- and polarization-tunable room temperature polariton laser due to emerging photonic spin–orbit coupling. For this purpose, we design an optical cavity filled with both birefringent nematic liquid crystal and an inorganic perovskite. Our versatile growth method of single CsPbBr3 inorganic perovskite crystals in polymer templates allows us to reach strong light–matter coupling and pump-induced condensation of exciton–polaritons resulting in coherent emission of light. The sensitivity of the liquid crystal to external voltage permits electrical tuning of the condensate energy across 7 nm; its threshold power, allowing us to electrically switch it on and off; and its state of polarization sweeping from linear to locally tilted circularly polarized emission.

Holographic Brain Theory: Super-Radiance, Memory Capacity and Control Theory.

We investigate Quantum Electrodynamics corresponding to the holographic brain theory introduced by Pribram to describe memory in the human brain. First, we derive a super-radiance solution in Quantum Electrodynamics with non-relativistic charged bosons (a model of molecular conformational states of water) for coherent light sources of holograms. Next, we estimate memory capacity of a brain neocortex, and adopt binary holograms to manipulate optical information. Finally, we introduce a control theory to manipulate holograms involving biological water's molecular conformational states. We show how a desired waveform in holography is achieved in a hierarchical model using numerical simulations.

Sub‐Nominal Resolution Fourier Transform Spectrometry with Chip‐Based Combs

AbstractChip‐based optical frequency combs address the demand for compact, bright, coherent light sources of equidistant phase‐locked lines. Traditionally, the Fourier Transform Spectroscopy (FTS) technique is considered a suboptimal choice for resolving comb lines in chip‐based sensing applications due to the requirement of long optical delays, and spectral distortion from the instrumental line shape. Here, a sub‐nominal resolution FTS technique is developed that extracts the comb's offset frequency in any spectral region directly from the measured interferogram without resorting to nonlinear ‐to‐ interferometry. This in turn enables 10's of MHz resolution spectrometry with millimeter optical retardations currently limited by the emission linewidth and phase noise of the used lasers. Low‐pressure Doppler‐broadened absorption lines probed by widely‐tunable chip‐scale mid‐infrared optical frequen with electrical pumping are fully resolved over a span of tens of nanometers. This versatile technique paves the way for compact, electrostatically‐actuated, or even all‐on‐chip high‐fidelity FTS, and can be readily applied to boost the resolution of existing commercial instruments with compact interferometers several hundred times.

Optimizing microlens arrays for incoherent HiLo microscopy

HiLo microscopy is a powerful, low-cost, and easily configurable technique for acquiring high-contrast optically-sectioned images. However, traditional HiLo microscopes are based on coherent light sources with diffusive glass plates or incoherent light sources with digital mirror devices (DMD) and spatial light modulators (SLM), which are more expensive. Here, we propose a new low-cost HiLo microscopy technique using MLAs and incoherent LED light sources. We simulated structured illumination (SI) patterns and HiLo image generation. To observe how MLAs affect HiLo images, we used three common MLAs with specific microlens pitch and numerical aperture (NA) to generate periodic illumination patterns. Our simulations concluded that the MLA's NA does not significantly affect HiLo images, and a larger lens pitch can bring a higher image contrast. However, there is an optimized lens pitch. If the lens pitch is equal to or higher than 140 μm, artifacts are observed in HiLo images. Based on our simulations, employing the cross-type MLA with a 0.01NA and a period of 120 μm yields the optimal HiLo image (94.6 % contrast). In our quantitative analysis with the traditional HiLo, where SI patterns were set with the same period, we calculated the SSIM index between each HiLo-Ground Truth image pair. The cross-type MLA HiLo performed slightly better (SSIM = 0.9554) than the traditional HiLo (SSIM = 0.9396). However, when using the hexagon-type MLA, artifacts were evident in the final HiLo image (SSIM = 0.9054). The cylinder-type MLA HiLo result (SSIM = 0.9366) is similar to the traditional HiLo. To our knowledge, this is the first numerical study about MLA-based HiLo microscopy. This study can benefit researchers using MLAs and incoherent light sources to configure their low-cost HiLo microscopes.

Introducing Corrections to the Reflectance of Graphene by Light Emission

Monolayer graphene absorbs 2.3 percent of the incident visible light. This “small” absorption has been used to emphasize the visual transparency of graphene, but it in fact means that multilayer graphene absorbs a sizable fraction of incident light, which causes non-negligible fluorescence. In this paper, we formulate the light emission properties of multilayer graphene composed of tens to hundreds of layers using a transfer matrix method and confirm the method’s validity experimentally. We quantitatively explain the measured contrasts of multilayer graphene on SiO2/Si substrates and find sizable corrections, which cannot be classified as incoherent light emissions, to the reflectance of visible light. The new component originates from coherent emission caused by absorption at each graphene layer. Multilayer graphene thus functions as a partial coherent light source of various wavelengths, and it may have surface-emitting laser applications.

Change of polarization degree of light beams on propagation in curved space

Even in free space, which is commonly considered of as a flat space–time in most settings, the degree of polarization of a partially spatially coherent light beam changes as it travels. Similarly, the polarization degree would change when a partially spatially coherent light beam propagates in a curved space–time. The difference of the polarization degree between the curved space and flat space can reveal the essential structure of the curved space. In this work, we consider a simplest case of curved space known as Schwarzschild spacetime. We can simulate the Schwarzschild space–time as an optical material with an effective refractive index. The difference of the polarization degree of a light beam propagating in curved space and flat space can be achieved up to 5%, which is detectable in practical measurement. In addition, we have found that the partially spatially coherent light source is necessary for obtaining significant changes in polarization degree. Our results provide an alternative method to estimate the Schwarzschild radius of a massive object with the optical polarization degree measurement.

All-carbon heterostructures self-assembly during field electron emission from diamond nanotip

In this study we demonstrate formation of all-carbon heterostructures induced by field electron emission from diamond needle-shaped crystallites with nanoscale tips. We show that at certain experimental conditions a carbon nanoprotrusion can be formed at the apex of a diamond emitter. Staircase-like current-voltage curves observed for such emitters indicated the presence of the Coulomb blockade effect in the self-assembled all-carbon heterostructures. The mechanism of nanoprotrusion formation via the field-induced surface diffusion of carbon atoms is revealed by observing the structural transformation of the emitter material using transmission electron microscopy. We also explore how the properties of the formed heterostructures evolve with the field emission current, and show that the characteristic size of the formed nanoprotrusion depends on the dimensions of the diamond nanotip. The developed approach offers a way to reproducible fabrication of heterostructured emitters which can be applied as coherent single-electron sources in vacuum nanoelectronics and electron quantum optics.

Efficient Third Harmonic Generation from Magnetic Resonance in Low-Index Dielectric Nanopillars

Boosting the harmonic generation of light in nanostructures through efficiently enhancing the light–matter interaction has received enormous attention and applications. Low-index dielectric nanoparticles, as one of the crucial members of nanophotonics, have not been successful in nonlinear enhancement due to weak Mie resonance and poor light confinement. Here, we designed efficient third harmonic generation (THG) in low-index dielectric nanopillars sandwiched by double layers of metal dressing (Au/polymer/Au), where the polymer offers essential nonlinear susceptibility. The resonance of the low-index nanopillars significantly enhanced the scattering and had a strong magnetic response that could boost the THG effect. We predict that the THG efficiency reaches up to 3 × 10−6 (six orders of enhancement) at a third harmonic wavelength of 300 nm. The efficient THG in low-index dielectric nanopillars may open the possibility for the development of a new type of efficient nonlinear coherent source.

Single-photon counting detectors for diffraction-limited light sources

When first introduced, single-photon counting detectors reshaped crystallography at synchrotrons. Their fast readout speed enabled, for example, shutter-less data collection and fine slicing of the rotation angle and boosted the development of new experimental techniques like ptychography. Under optimal conditions, single-photon counting detectors provide an unlimited dynamic range with image noise only limited by the Poisson statistics of the incoming photons. Counting the pulses from individual photons, essentially what made the detectors so successful, also causes the main drawback, which is the loss of efficiency at high photon fluxes due to pulse pileup in the analog front end. To fully take advantage of diffraction-limited light sources, the next-generation single-photon counters need to improve their count rate capabilities in the same order of magnitude as the increased flux. Moreover, fast frame rates (a few kHz) are required to cope with the shorter dwell time achievable, thanks to the higher flux. Detector architecture with multiple comparators and counters can open new possibilities for energy-resolved imaging, while interpixel communication can overcome the issues arising from charge sharing and reduce the loss of efficiency at the pixel corners. Coupling single-photon counting detectors to high-Z sensors for hard X-ray detection (>20 keV) and to low-gain avalanche diodes (LGADs) for soft X-rays is also necessary to make use of the increased coherence of the new light sources over the full radiation spectrum. In this paper, we present possible strategies to improve the performance of single-photon counting detectors at the fourth-generation synchrotron sources and compare them to charge integrating detectors.

Time-Dependent Resonant Inelastic X-ray Scattering of Pyrazine at the Nitrogen K-Edge: A Quantum Dynamics Approach.

We calculate resonant inelastic X-ray scattering spectra of pyrazine at the nitrogen K-edge in the time domain including wavepacket dynamics in both the valence and core-excited state manifolds. Upon resonant excitation, we observe ultrafast non-adiabatic population transfer between core-excited states within the core-hole lifetime, leading to molecular symmetry distortions. Importantly, our time-domain approach inherently contains the ability to manipulate the dynamics of this process by detuning the excitation energy, which effectively shortens the scattering duration. We also explore the impact of pulsed incident X-ray radiation, which provides a foundation for state-of-the-art time-resolved experiments with coherent pulsed light sources.

Nonadiabatic dynamics with classical trajectories: The problem of an initial coherent superposition of electronic states.

Advances in coherent light sources and development of pump-probe techniques in recent decades have opened the way to study electronic motion in its natural time scale. When an ultrashort laser pulse interacts with a molecular target, a coherent superposition of electronic states is created and the triggered electron dynamics is coupled to the nuclear motion. A natural and computationally efficient choice to simulate this correlated dynamics is a trajectory-based method where the quantum-mechanical electronic evolution is coupled to a classical-like nuclear dynamics. These methods must approximate the initial correlated electron-nuclear state by associating an initial electronic wavefunction to each classical trajectory in the ensemble. Different possibilities exist that reproduce the initial populations of the exact molecular wavefunction when represented in a basis. We show that different choices yield different dynamics and explore the effect of this choice in Ehrenfest, surface hopping, and exact-factorization-based coupled-trajectory schemes in a one-dimensional two-electronic-state model system that can be solved numerically exactly. This work aims to clarify the problems that standard trajectory-based techniques might have when a coherent superposition of electronic states is created to initialize the dynamics, to discuss what properties and observables are affected by different choices of electronic initial conditions and to point out the importance of quantum-momentum-induced electronic transitions in coupled-trajectory schemes.

Operation model of a skew-symmetric split-crystal neutron interferometer.

The observation of neutron interference using a triple Laue interferometer formed by two separate crystals opens the way to the construction and operation of skew-symmetric interferometers with extended arm separation and length. The specifications necessary for their successful operation are investigated here: most importantly, how the manufacturing tolerance and crystal alignments impact the interference visibility. In contrast with previous studies, both incoherent sources and the three-dimensional operation of the interferometer are considered. It is found that, with a Gaussian Schell model of an incoherent source, the integrated density of the particles leaving the interferometer is the same as that yielded by a coherent Gaussian source having a radius equal to the coherence length.

Single-photon superradiance in individual caesium lead halide quantum dots.

The brightness of an emitter is ultimately described by Fermi's golden rule, with a radiative rate proportional to its oscillator strength times the local density of photonic states. As the oscillator strength is an intrinsic material property, the quest for ever brighter emission has relied on the local density of photonic states engineering, using dielectric or plasmonic resonators1,2. By contrast, a much less explored avenue is to boost the oscillator strength, and hence the emission rate, using a collective behaviour termed superradiance. Recently, it was proposed3 that the latter can be realized using the giant oscillator-strength transitions of a weakly confined exciton in a quantum well when its coherent motion extends over many unit cells. Here we demonstrate single-photon superradiance in perovskite quantum dots with a sub-100 picosecond radiative decay time, almost as short as the reported exciton coherence time4. The characteristic dependence of radiative rates on the size, composition and temperature of the quantum dot suggests the formation of giant transition dipoles, as confirmed by effective-mass calculations. The results aid in the development of ultrabright, coherent quantum light sources and attest that quantum effects, for example, single-photon emission, persist in nanoparticles ten times larger than the exciton Bohr radius.

Two-pion interferometry for partially coherent sources in relativistic heavy-ion collisions in a multiphase transport model

Two-pion interferometry for partially coherent sources in relativistic heavy-ion collisions in a multiphase transport model