Coherence Peak Research Articles

Spin Seebeck effect mediated reversal of vortex-Nernst effect in superconductor-ferromagnet bilayers

We report on the observation of sign reversal of vortex-Nernst effect in epitaxial NbN/Fe bilayers deposited on MgO (001) substrates. Strong coupling between vortex magnetisation and ferromagnetic magnetisation at the NbN/Fe bilayer interface is presented. In NbN/Fe bilayer thin films an apparent sign reversal of vortex-Nernst signal under a temperature gradient with magnetic field and temperature is observed when the thickness of Fe is increased up to 5 nm. This reversal of the vortex-Nernst effect is associated with the enhancement of the spin Seebeck effects (SSE) near Tc due to coherence peak effect (CPE) and strong coupling of vortex magnetisation and ferromagnetic magnetisation at the interface of the NbN/Fe bilayer. The observed large SSE via inverse spin Hall effect (ISHE) is due to the CPE below and close to TC, highlighting the high spin to charge conversion efficiency of NbN in this region. This work may contribute to the development of superconducting spintronic devices by engineering the coupling of the superconductor/ferromagnet interface.

Observation of multigap and coherence peak in the noncentrosymmetric superconductor CaPtAs: As75 nuclear quadrupole resonance measurements

We present synthesis and $^{75}$As-nuclear quadrupole resonance (NQR) measurements for the noncentrosymmetric superconductor CaPtAs with a superconducting transition temperature $T_c$ of $\sim 1.5$ K. We discovered two different forms of CaPtAs during synthesis; one is a high-temperature tetragonal form that was previously reported, and the other is a low-temperature form consistent with the orthorhombic structure of CaPtP. According to the $^{75}$As-NQR measurement for superconducting tetragonal CaPtAs, the nuclear spin-lattice relaxation rate $1/T_1$ has an obvious coherence peak below $T_c$ and does not follow a simple exponential variation at low temperatures. These findings indicate that CaPtAs is a multigap superconductor and a large $s$-wave component.

Temperature dependence of the superconducting gap of single-layer FeSe/SrTiO3 : Direct comparison between transport and spectroscopic measurements

We studied the superconducting properties of the one-unit cell FeSe grown on high-doped ${\mathrm{SrTiO}}_{3}$(001) (STO) substrate by in situ transport and angle-resolved photoemission spectroscopy (ARPES) measurements. By comparing with previous data taken for the low-doped STO substrate [Phys. Rev. Lett. 124, 227002 (2020)], it was revealed that the onset of superconductivity occurs at $\ensuremath{\sim}40$ K irrespective of the STO doping level. Furthermore, from the temperature dependence of the critical current, we were able to deduce the superconducting gap that is relevant in the transport phenomena, which gradually increases by cooling the sample down from 40 K. In contrast, the coherent peak emerges at 60 K that likely corresponds to the Cooper pair formation, while the leading edge shift near the Fermi level is clearly observed at 40 K in the ARPES spectra. We speculate that the STO surface presumably acts as an effective ``disorder'' in this system and the Cooper pairs are preformed well above the onset of the resistance drop.

Temperature-dependent broadening of coherent current peaks in InAs double quantum dots

Quantum systems as used for quantum computation or quantum sensing are nowadays often realized in solid state devices as e.g. complex Josephson circuits or coupled quantum-dot systems. Condensed matter as an environment influences heavily the quantum coherence of such systems. Here, we investigate electron transport through asymmetrically coupled InAs double quantum dots and observe an extremely strong temperature dependence of the coherent current peaks of single-electron tunneling. We analyze experimentally and theoretically the broadening of such coherent current peaks up to temperatures of 20K and we are able to model it with quantum dissipation being due to two different bosonic baths. These bosonic baths mainly originate from substrate phonons. Application of a magnetic field helps us to identify the different quantum dot states through their temperature dependence.

In-plane electronic anisotropy revealed by interlayer resistivity measurements on the iron-based superconductor parent compound CaFeAsF

Both cuprates and iron-based superconductors demonstrate nematicity, defined as the spontaneous breaking of rotational symmetry in electron systems. The nematic state can play a role in the high-transition-temperature superconductivity of these compounds. However, the microscopic mechanism responsible for the transport anisotropy in iron-based compounds remains debatable. Here, we investigate the electronic anisotropy of CaFeAsF by measuring its interlayer resistivity under magnetic fields with varying field directions. Counterintuitively, the interlayer resistivity was larger in the longitudinal configuration ($B \parallel I \parallel c$) than in the transverse one ($B \perp I \parallel c$). The interlayer resistivity exhibited a so-called coherence peak under in-plane fields and was highly anisotropic with respect to the in-plane field direction. At $T$ = 4 K and $B$ = 14 T, the magnetoresistance $\Delta\rho/\rho_0$ was seven times larger in the $B \parallel b_o$ than in the $B \parallel a_o$ configuration. Our theoretical calculations of the conductivity based on the first-principles electronic band structure qualitatively reproduced the above observations but underestimated the magnitudes of the observed features. The proposed methodology can be a powerful tool for probing the nematic electronic state in various materials.

Investigation of coherent/Compton scattering differential cross section ratios in Cu alloys as depending on chemical environment and scattering angle

In this study, seven alloys with a nominal composition of (CuO2)0.5 M0.5 (M = Fe, Co, Ni, Cu, Zn, Y, and Nb wt%) were produced via the powder mixed method. Alloys and pure metals were excited with 59.54 keV photon energy emitted from Am-241 radioactive source at 25°, 35°, 45°, 55°, 65°, 75′ and 85° scattering angles. The spectra of the coherent/Compton peaks were obtained by Si(Li) detector. First of all, chemical shift, (ΔE) peak energies, (E) asymmetry index (As) and full width half maximum (FWHM) values were found in the Compton/Coherent scattering spectra obtained depending on the scattering angle and the chemical environment of the transition metals. Then the ratios of the Coherent/Compton scattering differential cross-section (dσcoherent/dσCompton) were obtained experimentally. The experimental dσcoherent/dσCompton ratios of the selected 3d-4d transition metals were found to be compatible with the data in the literature. Asymmetry and chemical shifts were observed in almost all samples, especially in Compton peaks, with increasing scattering angles. The chemical shifts of Compton and Coherent peaks of the alloys were found in the range of 1–932 eV. The experimental dσkoherent/dσCompton ratios for the alloys obtained by adding Fe, Co, Ni, Cu, Zn, Y, and Nb to Cu2O were found as 0.697, 0.689 0.678, 0.698, 0.736, 0.755, 0.798, 0.835 at 45° scattering angle, respectively. It has been determined that the experimental dσcoherent/dσCompton ratio for each alloy increases with increasing atomic number, while it decreases with increasing scattering angle.

First commissioning results of the coherent scattering and imaging endstation at the Shanghai soft X-ray free-electron laser facility

The Shanghai soft X-ray free-electron laser (SXFEL) user facility project started in 2016 and is expected to be open to users by 2022. It aims to deliver ultra-intense coherent femtosecond X-ray pulses to five endstations covering a range of 100–620 eV for ultrafast X-ray science. Two undulator lines are designed and constructed, based on different lasing modes: self-amplified spontaneous emission and echo-enabled harmonic generation. The coherent scattering and imaging (CSI) endstation is the first of five endstations to be commissioned online. It focuses on high-resolution single-shot imaging and the study of ultrafast dynamic processes using coherent forward scattering techniques. Both the single-shot holograms and coherent diffraction patterns were recorded and reconstructed for nanoscale imaging, indicating the excellent coherence and high peak power of the SXFEL and the possibility of “diffraction before destruction” experiments at the CSI endstation. In this study, we report the first commissioning results of the CSI endstation.

Correlation of Magnetism and Disordered Shiba Bands in Fe Monolayer Islands on Nb(110).

Two-dimensional (2D) magnet–superconductor hybrid systems are intensively studied due to their potential for the realization of 2D topological superconductors with Majorana edge modes. It is theoretically predicted that this quantum state is ubiquitous in spin–orbit-coupled ferromagnetic or skyrmionic 2D spin–lattices in proximity to an s-wave superconductor. However, recent examples suggest that the requirements for topological superconductivity are complicated by the multiorbital nature of the magnetic components and disorder effects. Here, we investigate Fe monolayer islands grown on a surface of the s-wave superconductor with the largest gap of all elemental superconductors, Nb, with respect to magnetism and superconductivity using spin-resolved scanning tunneling spectroscopy. We find three types of islands which differ by their reconstruction inducing disorder, the magnetism and the subgap electronic states. All three types are ferromagnetic with different coercive fields, indicating diverse exchange and anisotropy energies. On all three islands, there is finite spectral weight throughout the substrate’s energy gap at the expense of the coherence peak intensity, indicating the formation of Shiba bands overlapping with the Fermi energy. A strong lateral variation of the spectral weight of the Shiba bands signifies substantial disorder on the order of the substrate’s pairing energy with a length scale of the period of the three different reconstructions. There are neither signs of topological gaps within these bands nor of any kind of edge modes. Our work illustrates that a reconstructed growth mode of magnetic layers on superconducting surfaces is detrimental for the formation of 2D topological superconductivity.

Coherent Backscattering by Large Ice Crystals of Irregular Shapes in Cirrus Clouds

All elements of the scattering matrix have been numerically studied for particles of irregular shapes whose size is much larger than incident wavelength. The calculations are performed in the physical optics approximation for a particle size of 20 μm at a wavelength of 0.532 μm. Here the scattered intensity reveals the backscattering coherent peak. It is shown that the polarization elements of the matrix reveal the surges within the backscattering peak. The angular width of the surges does not practically depend on particle shape, but depends on the particle size. It is shown that these surges are created by interference between the conjugate scattered waves propagating in the inverse directions. The results obtained are of interest for interpretation of lidar measurements in cirrus clouds.

Tracking of magnetic helicity evolution in the inner heliosphere

Context. Magnetic helicity is one of the invariants in ideal magnetohydrodynamics, and its spectral evolution has a substantial amount of information to reveal the mechanism that are behind turbulence in space and astrophysical plasmas. Aims. The goal of our study is to observationally characterize the magnetic helicity evolution in the inner heliosphere by resolving the helicity transport in a scale-wise fashion in the spectral domain. Methods. The evolution of the magnetic helicity spectrum in the inner heliosphere was tracked using a radial alignment event achieved by Parker Solar Probe at a distance of 0.17 astronomical units (AU) from the Sun and BepiColombo at 0.58 AU with a delay of about 3.5 days. Results. The reduced magnetic helicity resolved in the frequency domain shows three main features: (1) a coherent major peak of a highly helical component at the lowest frequency at about 5 × 10−4 Hz, (2) a damping of helicity oscillation at the intermediate frequencies from 10−3 to 10−2 Hz when observed at 0.58 AU, and (3) a coherent nonhelical component in the ion-kinetic range at frequencies of about 0.1 − 1 Hz. Conclusions. Though limited in the frequency range, the main message from this work is that the solar wind develops into turbulence by convecting large-scale helicity components on the one hand and creating and annihilating helical wave components on the other hand. Excitation of waves can overwrite the helicity profile in the inner heliosphere. By comparing this with the typical helicity spectra at a distance of 1 AU (that is, a randomly oscillating helicity sign in the intermediate frequency range up to about 1 Hz), the helicity evolution reaches a nearly asymptotic state at the Venus orbit (about 0.7 AU) and beyond.

Acoustic, Phononic, Brillouin Light Scattering and Faraday Wave-Based Frequency Combs: Physical Foundations and Applications.

Frequency combs (FCs)—spectra containing equidistant coherent peaks—have enabled researchers and engineers to measure the frequencies of complex signals with high precision, thereby revolutionising the areas of sensing, metrology and communications and also benefiting the fundamental science. Although mostly optical FCs have found widespread applications thus far, in general FCs can be generated using waves other than light. Here, we review and summarise recent achievements in the emergent field of acoustic frequency combs (AFCs), including phononic FCs and relevant acousto-optical, Brillouin light scattering and Faraday wave-based techniques that have enabled the development of phonon lasers, quantum computers and advanced vibration sensors. In particular, our discussion is centred around potential applications of AFCs in precision measurements in various physical, chemical and biological systems in conditions where using light, and hence optical FCs, faces technical and fundamental limitations, which is, for example, the case in underwater distance measurements and biomedical imaging applications. This review article will also be of interest to readers seeking a discussion of specific theoretical aspects of different classes of AFCs. To that end, we support the mainstream discussion by the results of our original analysis and numerical simulations that can be used to design the spectra of AFCs generated using oscillations of gas bubbles in liquids, vibrations of liquid drops and plasmonic enhancement of Brillouin light scattering in metal nanostructures. We also discuss the application of non-toxic room-temperature liquid–metal alloys in the field of AFC generation.

Proximity-Effect-Induced Anisotropic Superconductivity in a Monolayer Ni-Pb Binary Alloy.

A proximity effect facilitates the penetration of Cooper pairs that permits superconductivity in a normal metal, offering a promising approach to turn heterogeneous materials into superconductors and develop exceptional quantum phenomena. Here, we have systematically investigated proximity-induced anisotropic superconductivity in a monolayer Ni-Pb binary alloy by combining scanning tunneling microscopy/spectroscopy (STM/STS) with theoretical calculations. By means of high-temperature growth, the Ni-Pb surface alloy has been fabricated on Pb(111) and the appearance of a domain boundary as well as a structural phase transition can be deduced from a half-unit-cell lattice displacement. Given the high spatial and energy resolution, tunneling conductance (dI/dU) spectra have resolved the reduced but anisotropic superconducting gap ΔNiPb ≈ 1.0 meV, in stark contrast to the isotropic ΔPb ≈ 1.3 meV. In addition, the higher density of states at the Fermi energy (D(EF)) of the Ni-Pb surface alloy results in an enhancement of coherence peak height. According to the same Tc ≈ 7.1 K with Pb(111) from the temperature-dependent ΔNiPb and the short decay length Ld ≈ 3.55 nm from the spatially monotonic decrease of ΔNiPb, both results are supportive of a proximity-induced superconductivity. Despite a lack of a bulk counterpart, the atomically thick Ni-Pb bimetallic compound opens a pathway to engineer superconducting properties down to the two-dimensional limit, giving rise to the emergence of anisotropic superconductivity via a proximity effect.

Functional connectivity maps of theta/alpha and beta coherence within the subthalamic nucleus region

The subthalamic nucleus (STN) is a primary target for deep brain stimulation in Parkinson's disease (PD). Although small in size, the STN is commonly partitioned into sensorimotor, cognitive/associative, and limbic subregions based on its structural connectivity profile to cortical areas. We investigated whether such a regional specialization is also supported by functional connectivity between local field potential recordings and simultaneous magnetoencephalography. Using a novel data set of 21 PD patients, we replicated previously reported cortico-STN coherence networks in the theta/alpha and beta frequency ranges, and looked for the spatial distribution of these networks within the STN region. Although theta/alpha and beta coherence peaks were both observed in on-medication recordings from electrode contacts at several locations within and around the STN, sites with theta/alpha coherence peaks were situated at significantly more inferior MNI coordinates than beta coherence peaks. Sites with only theta/alpha coherence peaks, i.e. without distinct beta coherence, were mostly located near the border of sensorimotor and cognitive/associative subregions as defined by a tractography-based atlas of the STN. Peak coherence values were largely unaltered by the medication state of the subject, however, theta/alpha peaks were more often identified in recordings obtained after administration of dopaminergic medication. Our findings suggest the existence of a frequency-specific topography of cortico-STN coherence within the STN, albeit with considerable spatial overlap between functional networks. Consequently, optimization of deep brain stimulation targeting might remain a trade-off between alleviating motor symptoms and avoiding adverse neuropsychiatric side effects.

Magnetic field induced transition from a vortex liquid to Bose metal in ultrathin a -MoGe thin film

We identify a magnetic field induced transition from a vortex liquid to Bose metal in a 2-dimensional amorphous superconductor, a-MoGe, using a combination of magnetotransport and scanning tunnelling spectroscopy (STS). Below the superconducting transition, Tc ~ 1.36 K, the magnetoresistance isotherms cross at a nearly temperature independent magnetic field, H_c^*~ 36 kOe. Above this field, the temperature coefficient of resistance is weakly negative, but the resistance remains finite as T --> 0, as expected in a bad metal. From STS conductance maps at 450 mK we observe a very disordered vortex lattice at very low fields that melts into a vortex liquid above 3 kOe. Up to H_c^* the tunnelling spectra display superconducting gap and coherence peak over a broad background caused by electron-electron interactions, as expected in a vortex liquid. However, above H_c^* the tunnelling spectra continue to display the gap but the coherence peak gets completely suppressed, suggesting that Cooper pairs lose their phase coherence. We conclude that H_c^* demarcates a transition from a vortex liquid to Bose metal, that eventually transforms to a regular metal at a higher field H* where the gap vanishes in the electronic spectrum.

Particle–hole asymmetric superconducting coherence peaks in overdoped cuprates

To elucidate the superconductor to metal transition at the end of superconducting dome, the overdoped regime has stepped onto the center stage of cuprate research recently. Here, we use scanning tunneling microscopy to investigate the atomic-scale electronic structure of overdoped trilayer Bi-2223 and bilayer Bi-2212 cuprates. At low energies the spectroscopic maps are well described by dispersive quasiparticle interference patterns. However, as the bias increases to the superconducting coherence peak energy, a virtually non-dispersive pattern with sqrt(2)*sqrt(2) periodicity emerges. Remarkably, the position of the coherence peaks exhibits evident particle-hole asymmetry which also modulates with the same period. We propose that this is an extreme quasiparticle interference phenomenon, caused by pairing-breaking scattering between flat anti-nodal Bogoliubov bands, which is ultimately responsible for the superconductor to metal transition.

S-wave superconductivity in the noncentrosymmetric W3Al2C superconductor: an NMR study

We report on a microscopic study of the noncentrosymmetric superconductor W3Al2C (with T c = 7.6 K), mostly by means of 27Al- and 13C nuclear magnetic resonance (NMR). Since in this material the density of states at the Fermi level is dominated by the tungsten’s 5d orbitals, we expect a sizeable spin–orbit coupling (SOC) effect. The normal-state electronic properties of W3Al2C resemble those of a standard metal, but with a Korringa product 1/(T 1 T) significantly smaller than that of metallic Al, reflecting the marginal role played by s-electrons. In the superconducting state, we observe a reduction of the Knight shift and an exponential decrease of the NMR relaxation rate 1/T 1, typical of s-wave superconductivity (SC). This is further supported by the observation of a small but distinct coherence peak just below T c in the 13C NMR relaxation-rate, in agreement with the fully-gapped superconducting state inferred from the electronic specific-heat data well below T c. The above features are compared to those of members of the same family, in particular, Mo3Al2C, often claimed to exhibit unconventional SC. We discuss why, despite the enhanced SOC, W3Al2C does not show spin-triplet features in its superconducting state and consider the broader consequences of our results for noncentrosymmetric superconductors in general.

Pallidal and Cortical Oscillations in Freely Moving Patients With Dystonia

ObjectivesTo evaluate the correlation between the pallidal local field potentials (LFPs) activity and the cortical oscillations (at rest and during several motor tasks) in two freely moving patients with generalized dystonia and pallidal deep brain stimulation (DBS). Materials and MethodsTwo women with isolated generalized dystonia were selected for bilateral globus pallidus internus (GPi) DBS. After the electrodes' implantation, cortical activity was recorded by a portable electroencephalography (EEG) system simultaneously with GPi LFPs activity, during several motor tasks, gait, and rest condition. Recordings were not performed during stimulation. EEG and LFPs signals relative to each specific movement were coupled together and grouped in neck/upper limbs movements and gait. Power spectral density (PSD), EEG-LFP coherence (through envelope of imaginary coherence operator), and 1/f exponent of LFP-PSD background were calculated. ResultsIn both patients, the pallidal LFPs PSD at rest was characterized by prominent 4–12 Hz activity. Voluntary movements increased activity in the theta (θ) band (4–7 Hz) compared to rest, in both LFPs and EEG signals. Gait induced a drastic raise of θ activity in both patients' pallidal activity, less marked for the EEG signal. A coherence peak within the 8–13 Hz range was found between pallidal LFPs and EEG recorded at rest. ConclusionsNeck/upper limbs voluntary movements and gait suppressed the GPi-LFPs—cortical-EEG coherence and differently impacted both EEG and LFPs low frequency activity. These findings suggest a selective modulation of the cortico-basal ganglia network activity in dystonia.

Surface topography measurement of microstructures near the lateral resolution limit via coherence scanning interferometry

As a non-destructive method, coherence scanning interferometry is widely utilized for surface topography measurement of step microstructures in optical and integrated circuit fields. The measurements are always implemented near the lateral resolution limit of the system because the critical dimension of these microstructures is at the micron or sub-micron scale. However, in this case, not only is the image of microstructures blurred, but also the diffraction effects distort the measured topography near the step edges. The magnitude of distortion at a certain position appears to be related to its distance from the edges and the duty cycle of the microstructures. Therefore, it is necessary, although difficult, to improve the accuracy of topography measurement for microstructures if their images are blurred owing to the lateral resolution limit. When located far away from the step edges of microstructures, the coherence signals are normal and contain a single envelope with its peak corresponding to the surface height. However, the anomalous coherence signals containing two envelopes appear near the step edges. The peaks of these envelopes correspond to the top and bottom surfaces of step structures, thus distorting the coherence peak detection for topography measurement. Therefore, the primary issue is the determination of the correct envelope in the anomalous coherence signals that is achieved by distinguishing the current surface of step structures for each position. In this paper, we propose a binarization method based on edge localization to achieve surface distinguishment through the analysis of the contrast and intensity of the coherence signals. After determining the correct envelope, we construct a new form of wavelet family and employ the Morlet wavelet transform to calculate a split point for dividing the anomalous coherence signals. Finally, the effective coherence signals corresponding to the correct envelope are extracted. Surface topography measurement of the nanopillars on the metasurface is obtained from the extracted signals. These nanopillars are distributed with a varying duty cycle and their diameters range from 590 to 1350 nm, near the lateral resolution limit of 501.9 nm of the system. The topography of nanopillars is recovered from the field of view, while the diameter and height of different types of nanopillars are measured. The mean value and standard deviation of these two parameters are consistent with the results obtained via scanning electron microscopy.

Magnetoencephalography Studies of the Envelope Following Response During Amplitude-Modulated Sweeps: Diminished Phase Synchrony in Autism Spectrum Disorder.

Prevailing theories of the neural basis of at least a subset of individuals with autism spectrum disorder (ASD) include an imbalance of excitatory and inhibitory neurotransmission. These circuitry imbalances are commonly probed in adults using auditory steady-state responses (ASSR, driven at 40 Hz) to elicit coherent electrophysiological responses (EEG/MEG) from intact circuitry. Challenges to the ASSR methodology occur during development, where the optimal ASSR driving frequency may be unknown. An alternative approach (more agnostic to driving frequency) is the amplitude-modulated (AM) sweep in which the amplitude of a tone (with carrier frequency 500 Hz) is modulated as a sweep from 10 to 100 Hz over the course of ∼15 s. Phase synchrony of evoked responses, measured via intra-trial coherence, is recorded (by EEG or MEG) as a function of frequency. We applied such AM sweep stimuli bilaterally to 40 typically developing and 80 children with ASD, aged 6–18 years. Diagnoses were confirmed by DSM-5 criteria as well as autism diagnostic observation schedule (ADOS) observational assessment. Stimuli were presented binaurally during MEG recording and consisted of 20 AM swept stimuli (500 Hz carrier; sweep 10–100 Hz up and down) with a duration of ∼30 s each. Peak intra-trial coherence values and peak response frequencies of source modeled responses (auditory cortex) were examined. First, the phase synchrony or inter-trial coherence (ITC) of the ASSR is diminished in ASD; second, hemispheric bias in the ASSR, observed in typical development (TD), is maintained in ASD, and third, that the frequency at which the peak response is obtained varies on an individual basis, in part dependent on age, and with altered developmental trajectories in ASD vs. TD. Finally, there appears an association between auditory steady-state phase synchrony (taken as a proxy of neuronal circuitry integrity) and clinical assessment of language ability/impairment. We concluded that (1) the AM sweep stimulus provides a mechanism for probing ASSR in an unbiased fashion, during developmental maturation of peak response frequency, (2) peak frequencies vary, in part due to developmental age, and importantly, (3) ITC at this peak frequency is diminished in ASD, with the degree of ITC disturbance related to clinically assessed language impairment.

Single-domain perpendicular magnetization induced by the coherent O 2p -Ru 4d hybridized state in an ultra-high-quality SrRuO3 film

We investigated the Ru $4d$ and O $2p$ electronic structure and magnetic properties of an ultrahigh-quality $\mathrm{SrRu}{\mathrm{O}}_{3}$ film on $\mathrm{SrTi}{\mathrm{O}}_{3}$ grown by machine-learning assisted molecular-beam epitaxy. The high itinerancy and long quantum lifetimes of the quasiparticles in the Ru $4d$ ${t}_{2g}$-O $2p$ hybridized valence band are confirmed by observing the prominent well-screened peak in the Ru $3d$ core-level photoemission spectrum, the coherent peak near the Fermi energy in the valence-band spectrum, and quantum oscillations in the resistivity. The element-specific magnetic properties and the hybridization between the Ru $4d$ and O $2p$ orbitals were characterized by Ru ${M}_{2,3}$-edge and O $K$-edge soft x-ray absorption spectroscopy and x-ray magnetic circular dichroism measurements. The ultrahigh-quality $\mathrm{SrRu}{\mathrm{O}}_{3}$ film with the residual resistivity ratio of 86 shows the large orbital magnetic moment of oxygen ions induced by the strong orbital hybridization of the O $2p$ states with the spin-polarized Ru $4d$ ${t}_{2g}$ states. The film also shows single-domain perpendicular magnetization with an almost ideal remanent magnetization ratio of 0.97. These results provide detailed insights into the relevance between orbital hybridization and the perpendicular magnetic anisotropy in $\mathrm{SrRu}{\mathrm{O}}_{3}/\mathrm{SrTi}{\mathrm{O}}_{3}$ systems.