Coherent Light Source Research Articles

Highly ordered graphite (HOPG) to hexagonal diamond (lonsdaleite) phase transition observed on picosecond time scales using ultrafast x-ray diffraction

The response of rapidly compressed highly oriented pyrolytic graphite (HOPG) normal to its basal plane was investigated at a pressure of ∼80 GPa. Ultrafast x-ray diffraction using ∼100 fs pulses at the Materials Under Extreme Conditions sector of the Linac Coherent Light Source was used to probe the changes in crystal structure resulting from picosecond timescale compression at laser drive energies ranging from 2.5 to 250 mJ. A phase transformation from HOPG to a highly textured hexagonal diamond structure is observed at the highest energy, followed by relaxation to a still highly oriented, but distorted graphite structure following release. We observe the formation of a highly oriented lonsdaleite within 20 ps, subsequent to compression. This suggests that a diffusionless martensitic mechanism may play a fundamental role in phase transition, as speculated in an early work on this system, and more recent static studies of diamonds formed in impact events.

The fluctuation-dissipation measurement instrument at the Linac Coherent Light Source.

The development of new modes at x-ray free electron lasers has inspired novel methods for studying fluctuations at different energies and timescales. For closely spaced x-ray pulses that can be varied on ultrafast time scales, we have constructed a pair of advanced instruments to conduct studies targeting quantum materials. We first describe a prototype instrument built to test the proof-of-principle of resonant magnetic scattering using ultrafast pulse pairs. This is followed by a description of a new endstation, the so-called fluctuation-dissipation measurement instrument, which was used to carry out studies with a fast area detector. In addition, we describe various types of diagnostics for single-shot contrast measurements, which can be used to normalize data on a pulse-by-pulse basis and calibrate pulse amplitude ratios, both of which are important for the study of fluctuations in materials. Furthermore, we present some new results using the instrument that demonstrates access to higher momentum resolution.

3D-Printed Möbius Microring Lasers: Topology Engineering in Photonic Microstructures.

Manipulating photons in artificially structured materials is highly desired in modern photonic technology. Nontrivial topological structures are rapidly emerging as a state-of-art platform for achieving unprecedented fascinating phenomena of photon manipulation. However, the current studies mainly focus on planar structures, and the fabrication of photonic microstructures with specific topological geometric features still remains a great challenge. Extending the topological photonics to 3Dmicroarchitectures is expected to enrich the photon manipulation capabilities and further advance the topological photonic devices. Here, a femtosecond laser direct writing technique is employed to fabricate 3D topological Möbius microring resonators from dye-doped polymer. The high-quality-factor Möbius microring resonator supports a unique spin-orbit coupled lasing at very low threshold. Due to the spin-orbit coupling induced geometric/Berry phase, the Möbius microrings, in striking contrast with ordinary microrings, output laser signals with all polarization states. The manipulation of miniaturized coherent light sources in the fabricated Möbius microrings represents a significant step forward toward 3D topological photonics that offers a novel design philosophy for functional photonic and optoelectronic devices.

Quasi-distributed fiber-optic acoustic sensor based on a low coherence light source.

A quasi-distributed acoustic sensor using in-line weak reflectors and a low coherence light source is presented. The dynamic strain is retrieved from the phase change of the two interfering light beams reflected by the same weak reflector. In the experiments, two vibrations at different channels along a weak reflector array are successfully detected simultaneously. A strain resolution of 50 pɛ/H z with 20-m interval is achieved in experiments, and no cross talk is observed. With simple system configuration and low cost, this approach provides a new, to the best of our knowledge, solution for quasi-distributed acoustic sensing.

White-Light Spectral Interferometry for Characterizing Inhomogeneity in Solutions and Nanocolloids.

We demonstrate the use of white-light spectral interferometry as an effective technique involving only linear optical interactions and a partially coherent light source to measure the complex transmission response function of optical resonance and to determine the corresponding variation in the refractive index relative to a reference. We also discuss experimental arrangements to increase the accuracy and sensitivity of the technique. The superiority of the technique over single-beam absorption measurements is demonstrated by the accurate determination of the response function of the chlorophyll-a solution. The technique is then applied to chlorophyll-a solutions of varying concentrations and gold nanocolloids to characterize inhomogeneous broadening. Results on the inhomogeneity of gold nanocolloids are also supported by transmission electron micrographs, showing distributions of the size and shape of the constituent gold nanorods.

Directional Laser from Solution‐Grown Grating‐Patterned Perovskite Single‐Crystal Microdisks

AbstractSolution‐processed, high‐gain, and wavelength‐tunable perovskite single‐crystal microdisk (PVKsc‐MD) lasers have emerged as prospective coherent light sources in advanced nanophotonic designs. However, the inevitable multi‐directional emission from a highly symmetrical cavity leads to low light collection efficiency which greatly hinders its application in integrated optical circuits. Here, we report on surface‐patterned MAPbBr3 PVKsc‐MDs synthesized by a cost‐efficient bottom‐up solution process employing spin‐coating and confined‐growth nanoimprinting. The patterned microdisks have high crystal quality with regular shape and sharp edges and nano‐grating structure on the upper surface. This straightforward process yields surface‐patterned PVKsc‐MD lasers with a low lasing threshold and high quality (Q) factor. In addition, the grating structure patterned on the PVKsc‐MDs reduces the original symmetry of the laser cavity, which improves the emission directionality four times.

Quasi‐Bound States in the Continuum Enhanced Second‐Harmonic Generation in Thin‐Film Lithium Niobate

AbstractThis work reports the second‐harmonic generation (SHG) in a z‐cut thin‐film lithium niobate (LN) under nearly normal‐incident linearly‐polarized pumping. To utilize the largest nonlinear term which is along the out‐of‐plane direction in the z‐cut LN film, the film is patterned with a 2D periodic array to support symmetry‐protected bound states in the continuum (BICs) bearing strong out‐of‐plane electric field component. Enabled by such optical resonances near the BIC condition at the pumping wavelength, significant enhancement in SHG compared to an unpatterned film is observed. This approach, combining transparent thin‐film nonlinear materials with tailored BICs, offers prospects for engineering compact coherent light sources in a broad wavelength range.

Demystifying speckle field interference microscopy

Dynamic speckle illumination (DSI) has recently attracted strong attention in the field of biomedical imaging as it pushes the limits of interference microscopy (IM) in terms of phase sensitivity, and spatial and temporal resolution compared to conventional light source illumination. To date, despite conspicuous advantages, it has not been extensively implemented in the field of phase imaging due to inadequate understanding of interference fringe formation, which is challenging to obtain in dynamic speckle illumination interference microscopy (DSI-IM). The present article provides the basic understanding of DSI through both simulation and experiments that is essential to build interference microscopy systems such as quantitative phase microscopy, digital holographic microscopy and optical coherence tomography. Using the developed understanding of DSI, we demonstrated its capabilities which enables the use of non-identical objective lenses in both arms of the interferometer and opens the flexibility to use user-defined microscope objective lens for scalable field of view and resolution phase imaging. It is contrary to the present understanding which forces us to use identical objective lenses in conventional IM system and limits the applicability of the system for fixed objective lens. In addition, it is also demonstrated that the interference fringes are not washed out over a large range of optical path difference (OPD) between the object and the reference arm providing competitive edge over low temporal coherence light source based IM system. The theory and explanation developed here would enable wider penetration of DSI-IM for applications in biology and material sciences.

Multi-moded high-index contrast optical waveguide for super-contrast high-resolution label-free microscopy.

The article elucidates the physical mechanism behind the generation of superior-contrast and high-resolution label-free images using an optical waveguide. Imaging is realized by employing a high index contrast multi-moded waveguide as a partially coherent light source. The modes provide near-field illumination of unlabeled samples, thereby repositioning the higher spatial frequencies of the sample into the far-field. These modes coherently scatter off the sample with different phases and are engineered to have random spatial distributions within the integration time of the camera. This mitigates the coherent speckle noise and enhances the contrast (2-10) × as opposed to other imaging techniques. Besides, the coherent scattering of the different modes gives rise to fluctuations in intensity. The technique demonstrated here is named chip-based Evanescent Light Scattering (cELS). The concepts introduced through this work are described mathematically and the high-contrast image generation process using a multi-moded waveguide as the light source is explained. The article then explores the feasibility of utilizing fluctuations in the captured images along with fluorescence-based techniques, like intensity-fluctuation algorithms, to mitigate poor-contrast and diffraction-limited resolution in the coherent imaging regime. Furthermore, a straight waveguide is demonstrated to have limited angular diversity between its multiple modes and therefore, for isotropic sample illumination, a multiple-arms waveguide geometry is used. The concepts introduced are validated experimentally via high-contrast label-free imaging of weakly scattering nanosized specimens such as extra-cellular vesicles (EVs), liposomes, nanobeads and biological cells such as fixed and live HeLa cells.

New method for the determination of photoabsorption from transmittance measurements in the extreme ultraviolet.

We have developed a new method for the determination of photoabsorption at extreme ultraviolet wavelengths longer than 20 nm, where reliable refractive index values are sparse or non-existent. Our method overcomes the obstacle of multiple reflections that occur inside thin films in this spectral range, which up until now has prevented the accurate determination of photoabsorption from transmittance measurements. We have derived a mathematical expression that is independent of internal reflection amplitudes, while taking advantage of the transmittance oscillations stemming from such reflections. The method is validated on measurements of aluminum thin films. This advance will enable accurate refractive index values for many important materials for optical instrumentation, thus facilitating high-priority research on topics including coherent light sources, planetary and solar physics, and semiconductor manufacturing.

Optical fiber optofluidic laser based on surfactant solubilization of rhodamine B gain in an aqueous solution.

We report a whispering gallery mode (WGM)-based fiber optofluidic laser (FOFL), in which rhodamine B (RhB) in an aqueous surfactant solution of sodium dodecylbenzene sulfonate (SDBS) is used as the laser gain medium. Here, the role of SDBS is to scatter the RhB dye molecules to effectively prevent its self-association in the aqueous solution. Therefore, the fluorescence quantum yield of the used RhB dye is improved due to the enhanced solubilization, which results in a low lasing threshold of ∼2.2 µJ/mm2 when the concentration of SDBS aqueous solution reaches up to 20 mM, on par with or even better than most of the optofluidic dye lasers using RhB as the gain medium in an organic solution. We then establish a model of solubilization capacity of SDBS micelles, which successfully addresses the mechanisms of dye-surfactant interactions in the proposed FOFL system. We further apply this FOFL platform to the case of concentration sensing of the used SDBS, which exhibits a 2-order-of-magnitude improvement in sensitivity compared to the fluorescence measurement due to the signal amplification inherent to the lasing process. The proposed FOFL platform in combination with surfactant solubilization gain medium in an aqueous solution promises to enable chip-scale coherent light sources for various environmental and bio-chemical sensing applications.

Fully integrated electrically driven optical frequency comb at communication wavelength

Abstract To meet the high demand of data transmission capacity, optical communications systems have been developed. In order to increase the channel numbers for larger communication bandwidth, multi-mode lasers and laser arrays can be used. As an alternative coherent light source, optical frequency comb (OFC) contains multi-wavelength signal, and hence enables communication with data stream of tens of terabit/s. Fully integrated electrically driven OFCs are expected as a compact, robust, and low-cost light source for data communication. In this review article, the recent development progress on fully integrated electrically driven OFC generators are reviewed, with focus on the demonstrations in the past five years. Based on comb generation approaches, the works are categorized into two main types: one is OFC generators based on four-wave mixing in high-Q resonator, and the other is OFC generators based on mode-locked laser. At the end, a summary and future outlook are provided.

Low Threshold and Ultrastability of One-Step Air-Processed All-Inorganic CsPbX3 Thin Films toward Full-Color Visible Amplified Spontaneous Emission

All-inorganic perovskites (CsPbX3) with the merits of high stability and remarkable optical gain property are attractive for achieving on-chip coherent light sources. Unfortunately, traditional solution-processed CsPbX3 films suffer from inevitable poor surface integrity and pinhole defects, severely hindering their optical properties. Here, from the perspective of precursor solution chemistry, we use an ionic liquid solvent methylammonium acetate (MAAc) to fabricate compact, pinhole-free, and smooth CsPbX3 thin films in a one-step air process without antisolvent treatment. Optically pumped amplified spontaneous emission (ASE) with a straightforward visible spectral tunability (418-725 nm) is achieved under both nanosecond and femtosecond laser excitation. For the representative CsPbBr3 films, the threshold reaches down to 11.4 μJ cm-2 under nanosecond laser pumping, which is comparable to the value under one-photon femtosecond pumping. The long gain lifetime up to 258.2 ps is revealed by transient absorption spectroscopy. Most importantly, the films show excellent optical stability and humidity stability with no obvious degradation under the pulsed laser irradiation for more than 210 min, stable ASE output under 95% high humidity, and conspicuous ASE after 1000 h of storage in air condition without encapsulation. These results demonstrate that the method of fabricating inorganic perovskite films with an ionic liquid solvent is promising in developing high-performance full-color visible lasers.

Compact generation of robust Airy beam pattern with spatial coherence engineering.

We present a class of partially coherent light sources having Airy-type amplitude and Airy-correlated spatial coherence. We show that the light beam generated by such sources can preserve the Airy beam pattern well during its propagation from source to far field. We demonstrate the robustness of the Airy beam pattern by introducing a hard aperture to largely block the beam source. We find that the coherence-induced Airy beam pattern can still be well reconstructed during propagation. We successfully synthesize such partially coherent source using the principle of complex random modes decomposition by using a single phase-only spatial light modulator. The proposed robust Airy beam pattern may find applications in information transmission through complex media.

The time-resolved atomic, molecular and optical science instrument at the Linac Coherent Light Source.

The newly constructed time-resolved atomic, molecular and optical science instrument (TMO) is configured to take full advantage of both linear accelerators at SLAC National Accelerator Laboratory, the copper accelerator operating at a repetition rate of 120 Hz providing high per-pulse energy as well as the superconducting accelerator operating at a repetition rate of about 1 MHz providing high average intensity. Both accelerators power a soft X-ray free-electron laser with the new variable-gap undulator section. With this flexible light source, TMO supports many experimental techniques not previously available at LCLS and will have two X-ray beam focus spots in line. Thereby, TMO supports atomic, molecular and optical, strong-field and nonlinear science and will also host a designated new dynamic reaction microscope with a sub-micrometer X-ray focus spot. The flexible instrument design is optimized for studying ultrafast electronic and molecular phenomena and can take full advantage of the sub-femtosecond soft X-ray pulse generation program.

Early Days of SACLA XFEL

The SACLA (SPring-8 Angstrom compact laser) was designed to significantly downsize the SASE (self-amplified spontaneous emission) type XFEL (X-ray free-electron laser), in order to generate coherent light in the wavelength region of 0.1 nm by adopting an in-vacuum undulator that can shorten the magnetic field period length. In addition, a SASE XFEL facility with a total length of 700 m has become a reality by using a C-band RF accelerating tube that enables a high acceleration gradient. Although progress was initially slow, the small-scale, low-cost SACLA was smoothly constructed, and it became the second light source to lase in the 0.1 nm wavelength region, following the LCLS (linac coherent light source) in the United States. In this paper, we look back on the history leading up to SACLA. and describe the SCSS (SPring-8 compact SASE source) project as a preparatory stage and a part of the construction/commissioning of SACLA. Since March 2012, SACLA has been operating as a shared user facility. Just a few of the upgrade activities of the facility and advanced research conducted are introduced. Finally, we will discuss the future development of the SPring-8 site, which has co-located the third-generation synchrotron radiation facility SPring-8 and the X-ray free-electron laser facility SACLA.

Towards performing high-resolution inelastic X-ray scattering measurements at hard X-ray free-electron lasers coupled with energetic laser drivers.

High-resolution inelastic X-ray scattering is an established technique in the synchrotron community, used to investigate collective low-frequency responses of materials. When fielded at hard X-ray free-electron lasers (XFELs) and combined with high-intensity laser drivers, it becomes a promising technique for investigating matter at high temperatures and high pressures. This technique gives access to important thermodynamic properties of matter at extreme conditions, such as temperature, material sound speed, and viscosity. The successful realization of this method requires the acquisition of many identical laser-pump/X-ray-probe shots, allowing the collection of a sufficient number of photons necessary to perform quantitative analyses. Here, a 2.5-fold improvement in the energy resolution of the instrument relative to previous works at the Matter in Extreme Conditions (MEC) endstation, Linac Coherent Light Source (LCLS), and the High Energy Density (HED) instrument, European XFEL, is presented. Some aspects of the experimental design that are essential for improving the number of photons detected in each X-ray shot, making such measurements feasible, are discussed. A careful choice of the energy resolution, the X-ray beam mode provided by the XFEL, and the position of the analysers used in such experiments can provide a more than ten-fold improvement in the photometrics. The discussion is supported by experimental data on 10 µm-thick iron and 50 nm-thick gold samples collected at the MEC endstation at the LCLS, and by complementary ray-tracing simulations coupled with thermal diffuse scattering calculations.

Simultaneous beam-based alignment measurement for multiple magnets by correcting induced orbit shift

We propose a method to simultaneously determine the magnetic centers of multiple quadrupoles in a transport line or a storage ring. The method finds the magnet centers by correcting the induced orbit shift due to a change of the quadrupole gradient strengths, with the goal of eliminating or minimizing such orbit shifts. The correction of the induced orbit shift is done by steering the orbit toward the quadrupole centers with correctors, using the response matrix of the induced orbit shift with respect to the correctors. The quadrupoles are selected with orbit corrector magnets and beam position monitors in between to ensure that orbit correction at the quadrupole locations can be achieved. The response matrix can be measured or calculated. Simulations with a section of the Linac Coherent Light Source II and the Stanford Positron Electron Asymmetric Ring (SPEAR3) storage ring are done to demonstrate the feasibility and performance of the method. It is also experimentally tested on SPEAR3. The method can be extended for beam-based alignment measurement of nonlinear magnets.

DUV coherent light emission from ultracompact microcavity wavelength conversion device.

A unique design of our ultracompact microcavity wavelength conversion device exploits the simple principle that the wavelength conversion efficiency is proportional to the square of the electric field amplitude of enhanced pump light in the microcavity, and expands the range of suitable device materials to include crystals that do not exhibit birefringence or ferroelectricity. Here, as a first step toward practical applications of all-solid-state ultracompact deep-ultraviolet coherent light sources, we adopted a low-birefringence paraelectric SrB4O7 crystal with great potential for wavelength conversion and high transparency down to 130 nm as our device material, and demonstrated 234 nm deep-ultraviolet coherent light generation, whose wavelength band is expected to be used for on-demand disinfection tools that can irradiate the human body.

LOEN: Lensless opto-electronic neural network empowered machine vision

Machine vision faces bottlenecks in computing power consumption and large amounts of data. Although opto-electronic hybrid neural networks can provide assistance, they usually have complex structures and are highly dependent on a coherent light source; therefore, they are not suitable for natural lighting environment applications. In this paper, we propose a novel lensless opto-electronic neural network architecture for machine vision applications. The architecture optimizes a passive optical mask by means of a task-oriented neural network design, performs the optical convolution calculation operation using the lensless architecture, and reduces the device size and amount of calculation required. We demonstrate the performance of handwritten digit classification tasks with a multiple-kernel mask in which accuracies of as much as 97.21% were achieved. Furthermore, we optimize a large-kernel mask to perform optical encryption for privacy-protecting face recognition, thereby obtaining the same recognition accuracy performance as no-encryption methods. Compared with the random MLS pattern, the recognition accuracy is improved by more than 6%.