Changes In Cloud Microphysics Research Articles

Buffering of Aerosol‐Cloud Adjustments by Coupling Between Radiative Susceptibility and Precipitation Efficiency

AbstractAerosol‐cloud interactions (ACI) in warm clouds are the primary source of uncertainty in effective radiative forcing (ERF) during the historical period and, by extension, inferred climate sensitivity. The ERF due to ACI (ERFaci) is composed of the radiative forcing due to changes in cloud microphysics and cloud adjustments to microphysics. Here, we examine the processes that drive ERFaci using a perturbed parameter ensemble (PPE) hosted in CAM6. Observational constraints on the PPE result in substantial constraints in the response of cloud microphysics and macrophysics to anthropogenic aerosol, but only minimal constraint on ERFaci. Examination of cloud and radiation processes in the PPE reveal buffering of ERFaci by the interaction of precipitation efficiency and radiative susceptibility.

Modulation of Tropical Convection‐Circulation Interaction by Aerosol Indirect Effects in Convective Self‐Aggregation Simulations of a Gray Zone Global Model

AbstractDisentangling the response of tropical convective updrafts to enhanced aerosol concentrations has been challenging. Leading theories for explaining the influence of aerosol concentrations on tropical convection are based on the dynamical response of convection to changes in cloud microphysics, neglecting possible changes in the environment. In recent years, global convection‐permitting models (GCPM) have been developed to circumvent problems arising from imposing artificial scale separation on physical processes associated with deep convection. Here, we use a global model in the convective gray zone that partially simulates deep convection to investigate how enhanced concentrations of aerosols that act as cloud condensate nuclei (CCN) impact tropical convection features by modulating the convection‐circulation interaction. Results from a pair of idealized non‐rotating radiative‐convective equilibrium simulations show that the enhanced CCN concentration leads to weaker large‐scale circulation, the closeness of deep convective systems to the moist cluster edges, and more mid‐level cloud water at an equilibrium state in which convective self‐aggregation occurred. Correspondingly, the enhanced CCN concentration modulates how the physical processes that support or oppose convective aggregation maintain the aggregated state at equilibrium. Overall, the enhanced CCN concentration facilitates the development of deep convection in a drier environment but reduces mean precipitation. Our results emphasize the importance of allowing atmospheric phenomena to evolve continuously across spatial and temporal scales in simulations when investigating the response of tropical convection to changes in cloud microphysics.

Solar Activity, Weather, and Climate: The Elusive Connection

Abstract The search for an explanation of correlations of weather and climate with solar activity has uncovered some subtle effects of the varying solar inputs, which include irradiance, energetic particles, electric fields induced by the solar wind, and the modulation of the galactic cosmic ray flux. Relevant phenomena have been identified in stratospheric chemistry and dynamics and in aerosols, atmospheric electricity, and clouds. The effects are small and appear intermittently in statistical analyses of observations. Correlations and theory permit responses to several solar inputs effective on the decadal time scales, making it difficult to distinguish them observationally. No mechanism for tropospheric decadal change can be considered to be definitely established, but for the day-to-day time scale there is clear observational evidence for clouds responding to solar wind–induced current flow (JZ) in the global electric circuit, due to changes in ionospheric potential, and independently from Forbush decreases of the cosmic ray flux. The responses to JZ also correlate separately with ionospheric potential changes due to changes in day-to-day thunderstorm activity. The identified mechanism is for electric charge effects on in-cloud scavenging, and this implies a decadal response, in view of decadal changes in JZ. However, a complete and quantitative model of the inferred electrically induced changes in cloud microphysics is not yet available. The failures, successes, and controversies of the search illustrate the somewhat chaotic process of scientific discovery.

Detection of large-scale cloud microphysical changes within a major shipping corridor after implementation of the International Maritime Organization 2020 fuel sulfur regulations

Abstract. New regulations from the International Maritime Organization (IMO) limiting sulfur emissions from the shipping industry are expected to have large benefits in terms of public health but may come with an undesired side effect: acceleration of global warming as the climate-cooling effects of ship pollution on marine clouds are diminished. Previous work has found a substantial decrease in the detection of ship tracks in clouds after the IMO 2020 regulations went into effect, but changes in large-scale cloud properties have been more equivocal. Using a statistical technique that estimates counterfactual fields of what large-scale cloud and radiative properties within an isolated shipping corridor in the southeastern Atlantic would have been in the absence of shipping, we confidently detect a reduction in the magnitude of cloud droplet effective radius decreases within the shipping corridor and find evidence for a reduction in the magnitude of cloud brightening as well. The instantaneous radiative forcing due to aerosol–cloud interactions from the IMO 2020 regulations is estimated as O(1 W m−2) within the shipping corridor, lending credence to global estimates of O(0.1 W m−2). In addition to their geophysical significance, our results also provide independent evidence for general compliance with the IMO 2020 regulations.

Microphysical and thermodynamic phase analyses of Arctic low-level clouds measured above the sea ice and the open ocean in spring and summer

Abstract. Airborne in situ cloud measurements were carried out over the northern Fram Strait between Greenland and Svalbard in spring 2019 and summer 2020. In total, 811 min of low-level cloud observations were performed during 20 research flights above the sea ice and the open Arctic ocean with the Polar 5 research aircraft of the Alfred Wegener Institute. Here, we combine the comprehensive in situ cloud data to investigate the distributions of particle number concentration N, effective diameter Deff, and cloud water content CWC (liquid and ice) of Arctic clouds below 500 m altitude, measured at latitudes between 76 and 83∘ N. We developed a method to quantitatively derive the occurrence probability of their thermodynamic phase from the combination of microphysical cloud probe and Polar Nephelometer data. Finally, we assess changes in cloud microphysics and cloud phase related to ambient meteorological conditions in spring and summer and address effects of the sea ice and open-ocean surface conditions. We find median N from 0.2 to 51.7 cm−3 and about 2 orders of magnitude higher N for mainly liquid clouds in summer compared to ice and mixed-phase clouds measured in spring. A southerly flow from the sea ice in cold air outbreaks dominates cloud formation processes at temperatures mostly below −10 ∘C in spring, while northerly warm air intrusions favor the formation of liquid clouds at warmer temperatures in summer. Our results show slightly higher N in clouds over the sea ice compared to the open ocean, indicating enhanced cloud formation processes over the sea ice. The median CWC is higher in summer (0.16 g m−3) than in spring (0.06 g m−3), as this is dominated by the available atmospheric water content and the temperatures at cloud formation level. We find large differences in the particle sizes in spring and summer and an impact of the surface conditions, which modifies the heat and moisture fluxes in the boundary layer. By combining microphysical cloud data with thermodynamic phase information from the Polar Nephelometer, we find mixed-phase clouds to be the dominant thermodynamic cloud phase in spring, with a frequency of occurrence of 61 % over the sea ice and 66 % over the ocean. Pure ice clouds exist almost exclusively over the open ocean in spring, and in summer the cloud particles are most likely in the liquid water state. The comprehensive low-level cloud data set will help us to better understand the role of clouds and their thermodynamic phase in the Arctic radiation budget and to assess the performance of global climate models in a region of the world with the strongest anthropogenic climate change.

Effects of Cloud Microphysics on the Universal Performance of Neural Network Radiation Scheme

AbstractUnderstanding the effect of cloud microphysical changes on the stability of radiation emulator is essential in an operational weather forecasting model with frequent updates. This study examined the effect of 15 microphysics schemes on a radiation emulator for real and ideal cases. In the real case, although the forecast errors against the control run increased with varying microphysics schemes to the trained scheme, the forecast error of 2‐m temperature was rather improved by 0.9%–5.4% when compared with observations. The radiation emulator for the real case was applied to an ideal squall‐line simulation to test its universal application, resulting in increase of 8.6%–41.3% more forecast errors in heating rates and fluxes for 14 microphysics schemes more than the trained scheme. These errors could be reduced by 26.5%–50.4% with the use of a compound parameterization. Therefore, the stability and accuracy of radiation emulator on microphysics changes was confirmed.

Physical processes driving intensification of future precipitation in the mid- to high latitudes

Precipitation is changing as the climate warms, and downpours can become more intense due to the increased water holding capacity of the atmosphere. However, the exact nature of the precipitation response and its characteristics is still not well understood due to the complex nature of the physical processes underlying the formation of clouds and precipitation. In this study, present and future Norwegian climate is simulated at convection-permitting scales with a regional climate model. The future climate is a high emission scenario at the middle of the century. Hourly precipitation is separated into three categories (convective, stratiform, and orographically enhanced stratiform) using a physically-based algorithm. We investigate changes in the frequency, intensity and duration of precipitation events for each category, delivering a more nuanced insight into the precipitation response to a changing climate. Results show very strong seasonality, with significant intensification of autumn precipitation. An increase in convective precipitation frequency and intensity dominates the climate change signal regardless of season. While changes in winter and summer are well explained by thermodynamical theory, the precipitation response in autumn and spring deviates from the idealised thermodynamic response, partly owing to changes in cloud microphysics. These results show that changes in the precipitation distribution are affected in complex ways by the local climatology, terrain, seasonality and cloud processes. They illustrate the need for further and more detailed investigations about physical processes underlying projected precipitation changes and their seasonal and regional dependence.

Limited Regional Aerosol and Cloud Microphysical Changes Despite Unprecedented Decline in Nitrogen Oxide Pollution During the February 2020 COVID-19 Shutdown in China.

Following the emergence of a novel coronavirus in Wuhan, China instituted shutdown measures starting in late January and continuing into February 2020 to arrest the spread of disease. This resulted in a sharp economic contraction unparalleled in recent Chinese history. Satellite retrievals show that nitrogen dioxide pollution declined by an unprecedented amount (~50% regionally) from its expected unperturbed value, but regional‐scale column aerosol loadings and cloud microphysical properties were not detectably affected. The disparate impact is tied to differential economic impacts of the shutdown, in which transportation, a disproportionate source of nitrogen oxide emissions, underwent drastic declines (~90% reductions in passenger traffic), whereas industry and power generation, responsible for >90% of particulate emissions, were relatively less affected (~20% reductions in electricity and thermal power generation). A combination of anomalously warm and humid meteorological conditions and complex chemical interactions further decreased nitrogen dioxide concentrations but likely enhanced secondary aerosol formation.

Parameterization of In‐Cloud Aerosol Scavenging Due to Atmospheric Ionization: Part 4. Effects of Varying Altitude

AbstractWe have verified that the modified analytic solution (MAS) for aerosol scavenging designed in our previous work to parameterize in‐cloud collision rate coefficients between aerosol particles and droplets can be extended to altitudes ranging from 0 to 20.6 km, and droplet radii up to 100 μm. The MAS deals separately with the short‐range effects and long‐range effects involved in the collisions, with the short‐range effects including image electric forces, the intercept effect, and the weight effect; and the long‐range effects including Brownian diffusion, the Coulomb electric force, and phoretic forces. The effects of Brownian diffusion and Coulomb electric force increase as height increases, while the change of phoretic forces with altitude is complicated. The effects of image electric force and intercept change slightly with altitude, while the weight effect increases significantly at higher altitudes. When the short‐range effects include the irregular shape of particles, the MAS also works well. The calculations of collision rate coefficients by our Monte Carlo trajectory model for varying droplet radius, droplet charges, particle radius, particle charges, particle density, relative humidity, pressure and temperature have now been completed, and we parameterize them by the simple MAS method which makes the results user friendly and easily applicable for cloud models. Based on our results, it is now possible to build cloud models to investigate the hypothesized link between the downward current flow in the global electric circuit current and cloud microphysical changes affecting cloud development.

Relating large-scale subsidence to convection development in Arctic mixed-phase marine stratocumulus

Abstract. Large-scale subsidence, associated with high-pressure systems, is often imposed in large-eddy simulation (LES) models to maintain the height of boundary layer (BL) clouds. Previous studies have considered the influence of subsidence on warm liquid clouds in subtropical regions; however, the relationship between subsidence and mixed-phase cloud microphysics has not specifically been studied. For the first time, we investigate how widespread subsidence associated with synoptic-scale meteorological features can affect the microphysics of Arctic mixed-phase marine stratocumulus (Sc) clouds. Modelled with LES, four idealised scenarios – a stable Sc, varied droplet (Ndrop) or ice (Nice) number concentrations, and a warming surface (representing motion southwards) – were subjected to different levels of subsidence to investigate the cloud microphysical response. We find strong sensitivities to large-scale subsidence, indicating that high-pressure systems in the ocean-exposed Arctic regions have the potential to generate turbulence and changes in cloud microphysics in any resident BL mixed-phase clouds.Increased cloud convection is modelled with increased subsidence, driven by longwave radiative cooling at cloud top and rain evaporative cooling and latent heating from snow growth below cloud. Subsidence strengthens the BL temperature inversion, thus reducing entrainment and allowing the liquid- and ice-water paths (LWPs, IWPs) to increase. Through increased cloud-top radiative cooling and subsequent convective overturning, precipitation production is enhanced: rain particle number concentrations (Nrain), in-cloud rain mass production rates, and below-cloud evaporation rates increase with increased subsidence.Ice number concentrations (Nice) play an important role, as greater concentrations suppress the liquid phase; therefore, Nice acts to mediate the strength of turbulent overturning promoted by increased subsidence. With a warming surface, a lack of – or low – subsidence allows for rapid BL turbulent kinetic energy (TKE) coupling, leading to a heterogeneous cloud layer, cloud-top ascent, and cumuli formation below the Sc cloud. In these scenarios, higher levels of subsidence act to stabilise the Sc layer, where the combination of these two forcings counteract one another to produce a stable, yet dynamic, cloud layer.

Regional modelling of rainfall erosivity: sensitivity of soil erosion to aerosol emissions

A rainfall erosivity scheme is implemented into the widely used regional atmosphere–land model, WRF. Rainfall erosivity is parametrized from hourly precipitation and surface runoff in a high resolution (4 km) convection‐permitting model. The scheme is used to examine the potential effects of changes in atmospheric aerosol concentrations on soil erosion in a case‐study of northern India and the surrounding countries for the 2010 monsoon season, using a model which isolates the indirect effect on cloud microphysics only. This study offers a preliminary investigation into this emerging topic, but longer simulations would be needed to establish a robust signal.Summer precipitation is reduced in most areas and the monsoon circulation weakens for increases in cloud condensation nuclei concentrations. This can be attributed to localised cloud microphysical changes in the northeast of India, which induce a dynamic response opposing the monsoon circulation. The two regions of greatest decrease in erosion with increasing aerosol are in the Western Ghats and the Ganges Delta, both significant cropland areas. However, the effect is not uniform, with isolated local increases in soil erosion. These results suggest that, while efforts to reduce anthropogenic aerosol emissions may improve water availability for crops through enhanced rainfall, these benefits are likely to be tempered by an increase in soil erosion, though robust local changes were difficult to predict.

Observed microphysical changes in Arctic mixed-phase clouds when transitioning from sea ice to open ocean

Abstract. In situ airborne observations of cloud microphysics, aerosol properties, and thermodynamic structure over the transition from sea ice to ocean are presented from the Aerosol-Cloud Coupling And Climate Interactions in the Arctic (ACCACIA) campaign. A case study from 23 March 2013 provides a unique view of the cloud microphysical changes over this transition under cold-air outbreak conditions. Cloud base lifted and cloud depth increased over the transition from sea ice to ocean. Mean droplet number concentrations, Ndrop, also increased from 110 ± 36 cm−3 over the sea ice to 145 ± 54 cm−3 over the marginal ice zone (MIZ). Downstream over the ocean, Ndrop decreased to 63 ± 30 cm−3. This reduction was attributed to enhanced collision-coalescence of droplets within the deep ocean cloud layer. The liquid water content increased almost four fold over the transition and this, in conjunction with the deeper cloud layer, allowed rimed snowflakes to develop and precipitate out of cloud base downstream over the ocean. The ice properties of the cloud remained approximately constant over the transition. Observed ice crystal number concentrations averaged approximately 0.5–1.5 L−1, suggesting only primary ice nucleation was active; however, there was evidence of crystal fragmentation at cloud base over the ocean. Little variation in aerosol particle number concentrations was observed between the different surface conditions; however, some variability with altitude was observed, with notably greater concentrations measured at higher altitudes ( > 800 m) over the sea ice. Near-surface boundary layer temperatures increased by 13 °C from sea ice to ocean, with corresponding increases in surface heat fluxes and turbulent kinetic energy. These significant thermodynamic changes were concluded to be the primary driver of the microphysical evolution of the cloud. This study represents the first investigation, using in situ airborne observations, of cloud microphysical changes with changing sea ice cover and addresses the question of how the microphysics of Arctic stratiform clouds may change as the region warms and sea ice extent reduces.

Effects of Urban Plume Aerosols on a Mesoscale Convective System

Abstract This study examines the effects of urban aerosols on a mesoscale convective system (MCS) in the central Great Plains with the Weather Research and Forecasting Model coupled with chemistry (WRF-Chem). Urban emissions from Kansas City, Missouri, were scaled by factors of 0.5, 1.0, and 2.0 to investigate the impact of urban aerosol load on MCS propagation and strength. The first half of the storm development is characterized by a stationary front to the north of Kansas City (phase I; 1800 UTC 26 May–0600 UTC 27 May), which develops into a squall line south of the urban area (phase II; 0600–1800 UTC 27 May). During phase I, doubling urban emissions shifts the precipitation accumulation, with enhancement downwind of the storm propagation and suppression upwind. During phase II, a squall line develops in the baseline and doubled emissions scenarios but not when emissions are halved. These changes in MCS propagation and strength are a function of cold pool strength, which is determined by microphysical processes and directly influenced by aerosol load. Overall, changes in urban emissions drive changes in cloud microphysics, which trigger large-scale changes in storm morphology and precipitation patterns. These results show that urban emissions can play an important role in mesoscale weather systems.

Thermodynamical and cloud microphysical response during the transition from southwest to northeast monsoon

The thermodynamical and microphysical response during the transition from southwest to northeast monsoon season is studied. Unique mixed phase cloud observations from the Cloud Aerosol Interaction and Precipitation Enhancement Experiment (CAIPEEX) and ground based observations from Integrated Ground Observation Campaign (IGOC), high resolution (3km) mesoscale forecasts with the nested Weather Research and Forecasting (WRF) model are used in the study. Convective available potential energy (CAPE), liquid water path (LWP) and precipitable water (PW) increased 3days before the onset and further enhanced with the onset of the northeast monsoon. A systematic decrease in lifting condensation level (LCL) height and increase in midlevel moisture before and during the onset period are observed, which resulted in increase in moist static energy in the midlayer for supporting deeper convection during the onset. Cloud microphysical response is noted with the mixed phase cloud observations of liquid water and ice water content. The model has simulated the mixed phase clouds in the area of detailed observations. Major cloud microphysical changes observed are (a) shallow warm clouds before the onset, (b) elevated supercooled liquid water content at the tops of clouds and (c) low ice water content during the onset period compared to subsequent periods after the onset with more ice water content.

The AgI Seeding Cloud Impact Investigation (ASCII) campaign 2012: overview and preliminary results

The ASCII campaign was conducted in early 2012 over the Sierra Madre, a Continental Divide range in Wyoming, to examine cloud microphysical changes resulting from the ground-based injection of silver iodide (AgI) into shallow orographic clouds. The campaign included a dual-polarization Doppler-On-Wheels radar on the mountain pass, the University of Wyoming King Air aircraft with profiling mm-wave radar and polarization backscatter lidar, two Ka-band profiling radars, one upstream of the AgI generators, and one downstream, and a number of instruments on the ground to characterize the cloud liquid water content and the in situ snow particle characteristics. The experimental design supported both simultaneous (upstream/ downstream) and non-simultaneous (before/ during) comparisons, in order to tease out the impact of glaciogenic seeding on cloud and precipitation. Unfortunately, suitably cold cloud base temperatures rarely occurred during the campaign. Nevertheless, profiling radar data collected on flights with a no-seeding period followed by a seeding period, as well as simultaneous ground-based profiling radar data, indicate that under suitable conditions AgI seeding can significantly increase radar reflectivity in the boundary layer, and thus snowfall rate near the ground.

The first aerosol indirect effect quantified through airborne remote sensing during VOCALS-REx

Abstract. The first aerosol indirect effect (1AIE) is investigated using a combination of in situ and remotely-sensed aircraft (NCAR C-130) observations acquired during VOCALS-REx over the southeast Pacific stratocumulus cloud regime. Satellite analyses have previously identified a high albedo susceptibitility to changes in cloud microphysics and aerosols over this region. The 1AIE was broken down into the product of two independently-estimated terms: the cloud aerosol interaction metric ACIτ =dlnτ/dlnNa|LWP , and the relative albedo (A) susceptibility SR-τ =dA/3dlnτ|LWP, with τ and Na denoting retrieved cloud optical thickness and in situ aerosol concentration respectively and calculated for fixed intervals of liquid water path (LWP). ACIτ was estimated by combining in situ Na sampled below the cloud, with τ and LWP derived from, respectively, simultaneous upward-looking broadband irradiance and narrow field-of-view millimeter-wave radiometer measurements, collected at 1 Hz during four eight-hour daytime flights by the C-130 aircraft. ACIτ values were typically large, close to the physical upper limit (0.33), with a modest increase with LWP. The high ACIτ values slightly exceed values reported from many previous in situ airborne studies in pristine marine stratocumulus and reflect the imposition of a LWP constraint and simultaneity of aerosol and cloud measurements. SR-τ increased with LWP and τ, reached a maximum SR-τ (0.086) for LWP (τ) of 58 g m−2 (~14), and decreased slightly thereafter. The 1AIE thus increased with LWP and is comparable to a radiative forcing of −3.2– −3.8 W m−2 for a 10% increase in Na, exceeding previously-reported global-range values. The aircraft-derived values are consistent with satellite estimates derived from instantaneous, collocated Clouds and the Earth's Radiant Energy System (CERES) albedo and MOderate resolution Imaging Spectroradiometer (MODIS)-retrieved droplet number concentrations at 50 km resolution. The consistency of the airborne and satellite estimates, despite their independent approaches, differences in observational scales, and retrieval assumptions, is hypothesized to reflect the ideal remote sensing conditions for these homogeneous clouds. We recommend the southeast Pacific for regional model assessments of the first aerosol indirect effect on this basis. This airborne remotely-sensed approach towards quantifying 1AIE should in theory be more robust than in situ calculations because of increased sampling. However, although the technique does not explicitly depend on a remotely-derived cloud droplet number concentration (Nd), the at-times unrealistically-high Nd values suggest more emphasis on accurate airborne radiometric measurements is needed to refine this approach.

A working hypothesis for connections between electrically-induced changes in cloud microphysics and storm vorticity, with possible effects on circulation

This paper outlines, and explores the uncertainties in, hypothesized connections between a series of processes that could explain two long-standing puzzles; those of (1) the observed winter storm vorticity responses to atmospheric energy inputs that change the ionosphere–earth current density, Jz, that appear to involve storm invigoration, and (2) changes in anti-cyclonic blocking and circulation that include the observed colder winters in Great Britain and western Europe at solar minima, and especially at extended solar minima. A working hypothesis for the mechanism responsible for (1) is that the flow of Jz through conductivity gradients, as in stratified cloud layers and fog, especially with sea-salt aerosol haze over the high latitude winter oceans, deposits electric changes on droplets and aerosol particles; most importantly on cloud condensation nuclei (CCN). These electric charges modulate scavenging of the particles in clouds and haze layers, increasing the concentration of small CCN and decreasing the concentration of large CCN. When further cloud formation occurs there is increased concentration of small droplets and decreased concentration of large ones, reducing coalescence and the production of rain. Thus updrafts carry more liquid water above the freezing level, and there the increased production of ice releases more latent heat and invigorates the updraft (the Rosenfeld mechanism), leading to increased vorticity. Here we explore the major uncertainties for the reality of the above chain of physical processes. A consequence of cumulative cyclonic vorticity increases is increases in downstream anti-cyclonic blocking. A further working hypothesis for (2) is that the invigoration may be large enough to contribute to the observed increases in blocking in winters at solar minima (high Jz) in the North Atlantic, that result in colder winters in the UK and northern Europe.

Long-term impacts of aerosols on the vertical development of clouds and precipitation

Aerosols alter cloud density and the radiative balance of the atmosphere. This leads to changes in cloud microphysics and atmospheric stability, which can either suppress or foster the development of clouds and precipitation. The net effect is largely unknown, but depends on meteorological conditions and aerosol properties. Here, we examine the long-term impact of aerosols on the vertical development of clouds and rainfall frequencies, using a 10-year dataset of aerosol, cloud and meteorological variables collected in the Southern Great Plains in the United States. We show that cloud-top height and thickness increase with aerosol concentration measured near the ground in mixed-phase clouds—which contain both liquid water and ice—that have a warm, low base. We attribute the effect, which is most significant in summer, to an aerosol-induced invigoration of upward winds. In contrast, we find no change in cloud-top height and precipitation with aerosol concentration in clouds with no ice or cool bases. We further show that precipitation frequency and rain rate are altered by aerosols. Rain increases with aerosol concentration in deep clouds that have a high liquid-water content, but declines in clouds that have a low liquid-water content. Simulations using a cloud-resolving model confirm these observations. Our findings provide unprecedented insights of the long-term net impacts of aerosols on clouds and precipitation.

Radiative effects of African dust and smoke observed from Clouds and the Earth's Radiant Energy System (CERES) and Cloud‐Aerosol Lidar with Orthogonal Polarization (CALIOP) data

Cloud and aerosol effects have a significant impact on the atmospheric radiation budget in the tropical Atlantic because of the spatial and temporal extent of desert dust and smoke from biomass burning in the atmosphere. The influences of African dust and smoke aerosols on cloud radiative properties over the tropical Atlantic Ocean were analyzed for the month of July for 3 years (2006–2008) using colocated data collected by the Cloud‐Aerosol Lidar with Orthogonal Polarization (CALIOP) and Clouds and the Earth's Radiant Energy System (CERES) instruments on the Cloud‐Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) and Aqua satellites. Aerosol layer height and type can be accurately determined using CALIOP data through directly measured parameters such as optical depth, volume depolarization ratio, attenuated backscatter, and color ratio. On average, clouds below 5 km had a daytime instantaneous shortwave (SW) radiative flux of 270.2 ± 16.9 W/m2 and thin cirrus clouds had a SW radiative flux of 208.0 ± 12.7 W/m2. When dust aerosols interacted with clouds below 5 km, as determined from CALIPSO, the SW radiative flux decreased to 205.4 ± 13.0 W/m2. Similarly, smoke aerosols decreased the SW radiative flux of low clouds to a value of 240.0 ± 16.6 W/m2. These decreases in SW radiative flux were likely attributed to the aerosol layer height and changes in cloud microphysics. CALIOP lidar observations, which more accurately identify aerosol layer height than passive instruments, appear essential for better understanding of cloud‐aerosol interactions, a major uncertainty in predicting the climate system.

Possible influences of Asian dust aerosols on cloud properties and radiative forcing observed from MODIS and CERES

The effects of dust storms on cloud properties and Radiative Forcing (RF) are analyzed over Northwestern China from April 2001 to June 2004 using data collected by the MODerate Resolution Imaging Spectroradiometer (MODIS) and Clouds and the Earth's Radiant Energy System (CERES) instruments on the Aqua and Terra satellites. On average, ice cloud effective particle diameter, optical depth and ice water path of cirrus clouds under dust polluted conditions are 11%, 32.8%, and 42% less, respectively, than those derived from ice clouds in dust‐free atmospheric environments. Due to changes in cloud microphysics, the instantaneous net RF is increased from −161.6 W/m2 for dust‐free clouds to −118.6 W/m2 for dust‐contaminated clouds.