Planar laser-induced fluorescence of O 2 has been performed in a turbulent nonpremixed flame using a broadband argon-fluoride source. For a given oxygen concentration, laser absorption and subsequent fluorescence emission increase strongly with temperature. The reverse configuration of the investigated flame with an axial injection of liquid oxygen in a fast coflow of hydrogen at ambient temperature is particularly well suited to this laser diagnostic. The liquid dart is quickly vaporized and no fluorescence is emitted from the liquid phase making it possible to investigate the concentration field of oxygen vapor in the flame. In addition, the laser irradiance has not been altered by cumulative absorption when it reaches the reaction zone where the hot and the weak amounts of O 2 are quantitatively detected with a maximum sensitivity. Assuming a fast direct reaction, the conditioned dissipation rate is derived from the gradient of the fluorescence signal at the stoichiometric surface. A two-dimensional map of the average rate of reaction is obtained showing a bimodal structure in the early stages of the flow development where the conditioned dissipation reaches high levels. These conditioned data have been spatially integrated to provide the cumulative oxygen consumption as a function of the distance to the injector. The results indicate that about 40% of the injected oxygen is consumed before the turbulent flame reaches the walls of the burner. To our knowledge, these are the first experimental data on quantitative reactant consumption in such a turbulent flame. The technique opens promising perspectives for detailed investigation of scalar dissipation and reaction rate in turbulent jet flames.
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