Thermoluminescent dosimetry (TLD) was successfully evaluated as an in-core thermal-neutron-flux determinant. The LiF crystals enriched with either /sup 6/Li or /sup 7/Li provided two effective neutron-gamma discrimination techniques. The first method used both types of crystals. The /sup 6/LiF dosimeters, which have large thermal-neutron cross sections, detected both neutrons and gamma radiation, while the /sup 7/LiF dosimeters, possessing negligible thermal-neutron attenuation characteristics, monitored the gamma component only. The dosimeters were inserted into a reactor for a known time interval and read on a commercially available detection system, and the difference in dosimeter exposure yielded a direct measure of neutron flux. The second technique used bare and cadmium-covered /sup 7/LiF dosimeters. The bare crystals detected reactor gammas, while those encapsulated in cadmium measured reactor gammas plus capture gammas from the Cd(n,..gamma..) reaction. The difference in exposures provided the capture-gamma contribution, which was proportional to reactor flux. Experiments using a subcritical and a TRIGA reactor revealed exposure rate to neutron flux sensitivities of 1.4 x 10/sup -7/ R/sec per phi and 2.6 x 10/sup -8/ R/sec per phi for the respective techniques. Accurate flux measurements were obtained over a range spanning 10/sup 2/ to 10/sup 12/ n/(cm/sup 2/ sec). At higher fluxes, more » the dosimeters experienced radiation damage and readings became unreliable. The TLD results were compared against BF/sub 3/ detection, foil activation, and fission chambers to derive an empirical exposure rate to the flux conversion factor. « less
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