A general mechanism is presented by which topological physics arises in strongly correlated systems without flat bands. Starting from a charge transfer insulator, topology emerges when the charge transfer energy between the cation and anion is reduced to invert the lower Hubbard band and the spin-degenerate charge transfer band. A universal low-energy theory is developed for the inversion of the charge transfer gap in a quantum antiferromagnet. The inverted state is found to be a quantum anomalous Hall (QAH) insulator with noncoplanar magnetism. Interactions play two essential roles in this mechanism: producing the insulating gap and quasiparticle bands prior to the band inversion, and causing the change of magnetic order necessary for the QAH effect after inversion. Our theory explains the electric-field-induced transition from a correlated insulator to a QAH state in AB-stacked transition-metal-dichalcogenides bilayer MoTe2/WSe2.3 MoreReceived 3 November 2021Revised 24 January 2022Accepted 9 March 2022DOI:https://doi.org/10.1103/PhysRevX.12.021031Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article’s title, journal citation, and DOI.Published by the American Physical SocietyPhysics Subject Headings (PhySH)Research AreasQuantum anomalous Hall effectPhysical SystemsBilayer filmsCharge-transfer insulatorsTransition metal dichalcogenidesTechniquesDensity matrix renormalization groupHartree-Fock methodsHubbard modelCondensed Matter, Materials & Applied Physics
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