Fiber Angle Research Articles

Homogenised strength criterion for natural fibre-reinforced composite

A representative model for multilayer natural fibre composite (NFC) plates is introduced to investigate its homogenised strength criterion. A three-layer NFC plate model is used to analyse the local stress–strain characteristics in multi-layered NFC. Finite element analysis (FEA) is performed on the representative volume element (RVE) under various boundary conditions to investigate stress and strain at macroscopic and microscopic levels. The explicit assessment of homogenised strength requires calculating stress tensors and equivalent stresses to determine parameter values. The precise specification of homogenised strength requirements assists in comprehending the material's behaviour under various loading conditions, which affects composite application design and optimisation techniques. The study examined the effect of fibre orientation angles on NFC's mechanical behaviour. The results demonstrate that flax fibres have comparatively higher stress levels than coir fibres. This study improves the understanding of natural fibre laminate composites’ macroscopic and microscopic behaviours, that is, the material's response under different loadings. The definition of homogenised strength criterion on NFC improves their design evaluations.

Grinding performance investigation of multidirectional CF/PEEK composites—A comparative with unidirectional CF/PEEK

AbstractTo distinguish the grinding performance of the multidirectional (MD) and unidirectional (UD) carbon fiber‐reinforced thermoplastic (CFRTP) composites, MD and UD carbon fiber‐reinforced poly‐etherether‐ketone (CF/PEEK) composites were employed in this study. Different ply stacking sequences and process parameters were set for grinding experiments. Subsequently, the surface morphologies and roughness were observed and measured. Experimental results indicated that the variations of grinding forces with grinding parameters of MD‐CF/PEEK and UD‐CF/PEEK were consistent. However, the heat transfer mechanism and the effects of grinding parameters on the maximum grinding temperatures were different between the two composites. The grinding forces and temperatures of MD‐CF/PEEK were slightly lower than UD‐CF/PEEK, and MD‐CF/PEEK reached better surface quality under the same parameters, indicating that the grinding performance of MD‐CF/PEEK was not the simple superposition of UD‐CF/PEEK. In addition, the chip formation and material removal mechanism of CF/PEEK were investigated. The grinding performance of MD‐CF/PEEK was primarily dependent on the θ elements of laminate while the grinding performance of UD‐CF/PEEK was closely related to the fiber orientation angles during grinding. This study established a more in‐depth understanding into the grinding performance of MD‐CF/PEEK and provided technical guidance for high‐quality grinding of CFRTP.Highlights The grinding performance of the multidirectional (MD) and unidirectional (UD) carbon fiber‐reinforced poly‐etherether‐ketone (CF/PEEK) is compared. The grinding forces and temperatures of MD‐CF/PEEK are slightly lower than that of UD‐CF/PEEK, and the MD‐CF/PEEK reach a better surface quality under the same grinding parameters. The grinding performance of MD‐CF/PEEK is primarily dependent on the θ elements of laminate, and the change of layering order is not a critical factor. The grinding performance of UD‐CF/PEEK is closely related to the fiber orientation angles during the grinding process. The surface quality of MD‐CFRTP can be effectively improved by reducing the grinding depth and feed speed, and increasing the grinding wheel speed.

Multilayer modeling framework for analyzing thermo-mechanical properties and responses of twisted and coiled polymer actuators

The twisted and coiled polymer actuator (TCPA) has a complex multi-scale structure consisting of crystalline micro-fibrils and an amorphous matrix at the micro-scale, which are organized into a macro-scale fiber. When the polymer fiber undergoes twisting and coiling, its mechanical and thermal properties become variable. In this study, we developed a multi-layer modeling framework capable of accurately predicting the effective mechanical and thermal properties, as well as the thermo-mechanical responses of the TCPA. Our numerical results demonstrate that the effective mechanical and thermal properties of the TCPA are influenced by the radius and twisting angle of the polymer fiber. By analyzing the precise mechanical and thermal properties, the numerical calculated driving responses exhibit good agreement with experimental data. We also examined the influence of initial helical radius, helical pitch and fiber radius on the driving responses of the TCPA. The proposed numerical model can be further utilized to optimize the driving responses of the TCPA by adjusting geometric parameters and the twisting angle of the polymer fiber.

Effect of Fiber Orientation and Volume Fraction on Young's Modulus for Unidirectional Carbon Fiber Reinforced Composites: A Numerical Investigation

The modulus of elasticity of unidirectional fiber-reinforced composites greatly depends on the fiber orientation and the fiber volume fraction. This paper investigates the effects of fiber orientation and fiber volume fraction using the commercially available Finite Element Analysis (FEA) software Abaqus. Carbon fiber is the reinforcing material, while epoxy is used as the matrix. Representative Volume Element (RVE) of the unidirectional carbon fiber reinforced composites are modeled in Abaqus, and the unidirectional tensile test is simulated to determine the modulus of elasticity for different fiber orientations and fiber volume fractions. The numerical results are verified by previously published results and by experimental results. It is found that the modulus of elasticity of the composite is maximum when the fiber inclination angle is 0°, i.e., the fibers are placed along the loading direction. As the fiber orientation angle increases, the modulus of elasticity also decreases and is almost constant after 45°. A linear increase in modulus of elasticity is observed for an increase in fiber volume fraction. This model will help the researcher to select the appropriate fiber orientation and volume fraction for a specific application.

Optimization Of Hybrid Composite Laminates With Various Materials Using GA/GPSA Hybrid Algorithm for Maximum Dimensional Stability

In this study, it is aimed to obtain the highest dimensional stability against temperature changes in fiber-reinforced hybrid composite laminates considering eight different composite materials: Aramid/Epoxy, AS4/Epoxy, Boron/Epoxy, E-Glass/Epoxy, IM6/Epoxy, GY70/Epoxy, Kevlar49/Epoxy, and Spectra/Epoxy. The study focuses on finding the optimum continuous and traditional fiber angle orientations for the hybrid composite plates that would provide the lowest coefficients of thermal expansion. For this purpose, two different laminate sequences were investigated, each including two materials. A hybrid algorithm combining genetic algorithm and generalized pattern search algorithm was used in the optimization. A great number of hybrid design problems were solved repeatedly, and their results were compared both within themselves and to the optimum non-hybrid laminate results. Furthermore, the thermal durability of the selected optimum hybrid designs was evaluated by Tsai-Wu failure and Hashin-Rotem criteria. The results reveal that substantial increase in dimensional stability can be achieved by stacking sequence optimization of hybrid composite laminates with multiple material selection, and this hybrid design approach can offer the desired laminated composite structures for aerospace applications required to withstand extreme temperature changes.

Improving the Accuracy of the Evaluation Method for the Interfacial Shear Strength of Fiber-Reinforced Thermoplastic Polymers through the Short Beam Shear Test.

Short fiber-reinforced thermoplastic polymers (SFRTPs) are commonly used in various molding methods due to their high specific elasticity and strength. To evaluate the interfacial strength, several determination methods have been proposed, including the interfacial shear strength (IFSS). In previous research, an IFSS evaluation method based on the short beam shear method was proposed. However, this method is only applicable to micrometer-sized fibers with high stiffness levels that are not easily bent. When utilizing cellulose fiber, the interfacial shear strength (IFSS) results frequently exhibit significant deviations. To tackle this issue, we suggest an enhanced experimental technique that employs beam-shaped specimens with welding points based on the short beam shear test. Furthermore, we conducted a three-dimensional analysis of the original method to determine the fiber orientation angle and IFSS. The outcomes were compared with previously reported determinations. The IFSS achieved through the novel method proposed in this paper exhibits high precision and reliability, rendering it suitable for use with soft and flexible fibers.

An anisotropic topology optimization procedure for continuous fiber reinforced polymer structures with biaxial fiber layout for improved intersection point design

Fiber placement technologies allow for manufacturing of complex-shaped composite parts with load-adapted fiber orientation. For design of corresponding structures, topology optimization is well-established. However, anisotropic topology optimization approaches are often limited to unidirectional fiber orientations. In truss-like topology optimized structures, the intersections between the individual trusses are subject to multiaxial stress states. For those, a unidirectional fiber orientation is not appropriate and may not be suitable for manufacturing.In this work we propose a topology optimization procedure that allows for unidirectional but also biaxial fiber orientations. The choice between unidirectional and biaxial fiber layout is based on the stress state within the finite elements. For the biaxial fiber layout, the first fiber angle is aligned with the maximum absolute principal stress direction, while the second fiber orientation is calculated using composite net theory.Results show that considering biaxial fiber orientations leads to fiber orientations that can be better manufactured by fiber placement technologies and are considered suitable for automatic derivation of manufacturing-tolerant placement paths. Furthermore, the stress state at intersections is improved reducing the probability of inter fiber failure. In addition, consideration of biaxial fiber orientations could increase the stiffness at constant weight compared to purely unidirectional topology optimization.

Abstract 5571: Collagen stabilization directs immune suppression in the head and neck squamous cell carcinoma hypoxic subtype

Abstract Head & neck squamous cell carcinoma (HNSCC) show limited clinical benefit to immune checkpoint inhibitors (ICI). Interactions between extracellular matrix (ECM), tumor, and immune cells underly the mechanisms leading to immunosuppression and resistance to ICIs. Collagen matrix remodeling within tumor stroma can influence accessibility and function of immune cells. Specifically, telopeptidyl lysine residues in fibrillar collagen can be hydroxylated by Lysyl hydroxylase 2 (LH2) prior to cross-linking which leads to stiffened, stable collagen. We previously showed that this LH2-modified tumor microenvironment (TME) drives HNSCC invasion and metastasis. Here, we elucidate the interplay between LH2-modified collagen and the immune landscape within TME of hypoxic and immunosuppressive HNSCC. Bioinformatics analyses of RNAseq datasets were performed to assess pathways regulating collagen deposition and stabilization. Tissue microarray having 81 primary, 28 recurrent primary, and 3 lymph node metastases tumor cores was analyzed. Cores were classified according to our published Hypoxia-Immune signature (Chaudhary R. et al. 2023, Can Res Comm). We performed Second Harmonic Generation imaging of H&E stained TMA section to analyze the orientation and length of collagen fibrils. Picrosirius red (PSR) staining allowed quantification of total collagen and collagen maturation was assessed by polarized light imaging of birefringence. Further, we performed multiplex immunofluorescence staining for CD3+ (T-cell); CD14+ (Monocyte & Macrophage); CD11c+ (Dendritic); Pax5+ (B-cell); Pan-Cytokeratin+ (tumor), and LH2. Low (0-1) LH2 expression was seen in 29.5% of analyzed cores whereas 70.5% of cores scored high (2-3) for LH2 expression. Cores classified under the hypoxia subtype exhibit high LH2 and enrichment of collagen stability signature. Late-stage tumors have highly oriented collagen fibers compared to normal tissue or early-stage tumors which have randomly distributed fibers. CT-Fire-based measurements revealed that LH2hi cores have significantly increased fiber length and lower coefficient of variance for fiber angles. The area of collagen measured by PSR staining had no correlation with tumor stage or subtype indicating that collagen deposition is similarly high in HNSCCs. However, birefringence measurements showed that a higher fraction of mature fibrillar collagen is associated with late-stage LH2hi tumors. Interestingly, LH2 expression positively correlated with increased CD3+ T cells in stroma suggesting that anti-tumor T cells are physically obstructed by the presence of LH2-stabilized and stiffened collagen fibers. LH2 expression influences the quality of collagen but not the quantity. Understanding the effect of LH2-mediated collagen modifications on the TIME may have implications for therapeutic strategies to enhance anti-tumor immune response in HNSCC. Citation Format: Sonal Srivastava, John Powers, Ritu Chaudhary, Sadegh Marzban, Robbert J. Slebos, Jeffrey West, Xiaofei Song, Jose A. Guevara-Patino, Christine H. Chung, Antonio L. Amelio. Collagen stabilization directs immune suppression in the head and neck squamous cell carcinoma hypoxic subtype [abstract]. In: Proceedings of the American Association for Cancer Research Annual Meeting 2024; Part 1 (Regular Abstracts); 2024 Apr 5-10; San Diego, CA. Philadelphia (PA): AACR; Cancer Res 2024;84(6_Suppl):Abstract nr 5571.

Improving fatigue characteristics of ply drop-off in composite laminate with ply curving termination

Ply drop-off is a weak point of a tapered composite laminate, where stress concentration occurs and delamination initiates. By suppressing delamination from the ply drop-off, more optimized structural design and further weight reduction are possible. Ply Curving Termination (PCT), which locally changes the fiber direction at the edge of the dropped ply, is one of the promising delamination suppression mechanisms. To improve the technical maturity of PCT, this study conducted tensile fatigue tests using asymmetric taper configuration. Damage initiation, delamination propagation, and final failure were evaluated in detail by changing the PCT fiber angle and loading level, confirming that large PCT angles are effective in improving the fatigue properties of tapered laminates and that controlling the location of initial damage is necessary to maximize the effectiveness of PCT. Based on the findings, an effective design guideline for tapered laminates with PCT was presented.

Flexural performance of nature-inspired 3D-printed strain-hardening cementitious composites (3DP-SHCC) with Bouligand structures

Inspired by nature, this study employed the Bouligand structures, as observed in the dactyl club of mantis shrimp, to enhance the performance of 3D-printed Strain-Hardening Cementitious Composites (3DP-SHCC). Twenty sets of printed and mold-cast specimens were prepared to investigate the effects of Bouligand structures on the flexural performance of 3DP-SHCC. Three printing patterns (parallel, cross, and Bouligand printing) and five pitch angles (15°, 30°, 45°, 60°, 75°) were used for the Bouligand printing pattern. The results showed that the flexural performance of parallel-printed SHCC exhibited significant directionality. The flexural strength and toughness of parallel-printed SHCC in the X direction were 1.28 times and 3.27 times greater than the mold-cast SHCC. However, the flexural strength and toughness in the Y direction were 0.58 times and 0.25 times those of the mold-cast SHCC. The cross-printed and Bouligand-printed SHCC alleviated the directionality. The flexural performance of cross-printed SHCC was lower than that of the mold-cast SHCC. Compared to parallel-printed SHCC, the flexural strength and toughness of Bouligand-printed SHCC increased by 1.25 to 1.73 times and 3.48 to 5.10 times, respectively, in the Y direction. Bouligand-printing twisted the fiber angles, enabling effective crack bridging across multiple directions and endowing the SHCC with uniform mechanical properties in various directions. The Bouligand structures provided valuable inspiration for optimizing 3DP-SHCC structures.

In-situ monitoring of carbon fiber/epoxy composite with FBG sensors under curing and thermal cycling conditions

Residual strains from curing process as well as thermal expansion behaviors in application process are critical to structural design of composites. Here we demonstrate the applicability of fiber Bragg grating (FBG) sensors for in-situ measurements of strain evolution in epoxy resin and unidirectional (UD) laminate under curing and thermal cycling conditions. The validity of the FBG sensors was verified by the TMA tests. From the data recorded by the sensors, the information about real-time gel point, strain/temperature evolution and residual strains during curing can be obtained. The epoxy resin and UD laminates have distinct curing histories and characteristics under the same curing conditions because of the exothermic reaction. During thermal cycling, we found that the coefficient of thermal expansion (CTE) of the UD laminate is directional dependent as is the residual strain, i.e., it increases with fiber orientation angle. In addition, the relaxation of partial residual strains, attributed to the mismatch in CTE between the specimen and the mold, was captured by FBG sensors around the glass transition temperature during the first thermal cycle.

Effect of the filling pattern in 3D-printed polylactic acid scaffolds on mechanical properties and cell proliferation for bone tissue regeneration

3D printing technology can control the shape and filling pattern of the scaffold very well and has been widely used in the preparation of bone repair scaffolds. Modifying the filling pattern of scaffolds to alter their mechanical properties and cellular adhesion holds immense significance. In this study, 3D-printed polylactic acid (PLA) scaffolds with different fibre angles (15°-90°) were prepared. The 90° scaffold showed the best mechanical properties and was suitable for repairing long bones. The 60° scaffold has balanced mechanical properties and is suitable for maxillofacial bone repair. The scaffold with a 30° angle was the best for cell adhesion and proliferation and was suitable for cancellous bone repair.

Formulation and free vibration analysis of spinning Timoshenko composite beams using nonlinear geometrically exact theory

AbstractIn this study, a set of generalized nonlinear equations of motion for Timoshenko composite shafts is derived using the geometrically exact approach. These partial differential equations of motion are discretized by Galerkin method and the free vibration of an orthotropic spinning shaft with hinged‐hinged boundary conditions is investigated using the multiple‐scale method. We find that in the case of two mode discretization, composite couplings can have significant linear and nonlinear effects on the behavior of the shaft and that these effects were not predictable in the classical model. Also, in the investigating of composite layering we find that the effects of the fibers angle as well as the composite couplings can be noticeable, and these effects are greater in the case of the asymmetrical layering.

Buckling variability analysis in damaged composite laminates subjected to thermally varying environment

The present study investigates the effect of internal defects on the composite laminated (CL) plates comprised of two distinct graphite-epoxy materials (AS4/3501-6 and T300/5208). The centrally damaged laminates stacked in two distinct lamination sequences are exposed in thermally varying environments. The CL plates are considered to experience damage in two different combinations of damage parameters. The improved first-order shear deformation theory (IFSDT) based finite element (FE) model is employed to estimate the thermal buckling of CL plates comprised of multiple fiber orientation angles and constrained to C-S-C-S and S-C-S-C boundary restrictions. The implementation of a Radial basis function network (RBFN) surrogate model has demonstrated its potential as a feasible substitute for the computationally demanding Monte-Carlo simulations (MCS) in the context of stochastic exploration. The present investigation scrutinizes the probabilistic properties of diverse materials and their associated damage characteristics. Subsequently, the RBFN-based surrogate model is employed to evaluate the likelihood of failure.

Structural parameters defining distribution of collagen fiber directions in human carotid arteries

Collagen fiber arrangement is decisive for constitutive description of anisotropic mechanical response of arterial wall. In this study, their orientation in human common carotid artery was investigated using polarized light microscopy and an automated algorithm giving more than 4·106 fiber angles per slice. In total 113 slices acquired from 18 arteries taken from 14 cadavers were used for fiber orientation in the circumferential-axial plane. All histograms were approximated with unimodal von Mises distribution to evaluate dominant direction of fibers and their concentration parameter. 10 specimens were analyzed also in circumferential-radial and axial-radial planes (2-4 slices per specimen in each plane); the portion of radially oriented fibers was found insignificant. In the circumferential-axial plane, most specimens showed a pronounced unimodal distribution with angle to circumferential direction μ = 0.7° ± 9.4° and concentration parameter b = 3.4 ± 1.9. Suitability of the unimodal fit was confirmed by high values of coefficient of determination (mean R2 = 0.97, median R2 = 0.99). Differences between media and adventitia layers were not found statistically significant. The results are directly applicable as structural parameters in the GOH constitutive model of arterial wall if the postulated two fiber families are unified into one with circumferential orientation.

Optimization of infill density, fiber angle, carbon fiber layer position in 3D printed continuous carbon-fiber reinforced nylon composite

Composite materials have gained much attention in various industries, such as aerospace, automotive, sports, marine, and construction, as these sectors rely on high-performance, durable, and cost-effective materials. Such materials offer high strength, stiffness and heat resistance. However, the influence of printing parameters especially the position of carbon fiber layer on such material is rarely found in literature. The current study focuses on optimizing different printing and testing parameters such as carbon fiber layer position, infill density, fiber angle, and strain rate in 3D printed carbon-fiber reinforced nylon composite. The study also recommended the optimal combination of these parameters for maximizing the mechanical strength and energy absorption of related 3D printed parts. The investigation revealed that the most optimum condition was 80% infill density, fiber angle of 0°, carbon fiber layer position of 12–13, and strain rate of 10 mm/min. It has been found in the study that fiber angle was the most dominant input parameter with a contribution of 54.13%, whereas infill density was the second dominant parameter with a contribution of 16.25%. The study also found that the position of the carbon fiber layer has comparatively less effect on the final mechanical properties of 3D printed parts, with a contribution of 10.12%. To facilitate the optimization, the outcomes will be helpful for designing and manufacturing 3D printed carbon-fiber reinforced nylon composite parts.

Tensile properties of banana fiber reinforced recycled high‐density polyethylene composites: An experimental investigation

AbstractNatural fiber‐reinforced polymer composites (NFRCs) are increasingly favored over synthetic fiber‐reinforced alternatives due to their beneficial properties and environmental sustainability. Mechanical properties of composites are critical to ensure optimized utilization of NFRCs. Here, this research explores the effects of different fiber parameters on the tensile strength of high‐density polymer composites reinforced with banana fiber and utilizes the Taguchi method for both experimental and statistical analysis of the outcomes. Three different parameters are considered here: weight fractions, fiber orientation angle, and plasma treatment to fabricate the composites using the compression molding process. Taguchi analysis revealed that fiber orientation angle has the greatest influence among the three variables, with plasma treatment and weight fraction following in impact on tensile strength. The composite that exhibited the highest tensile strength was determined to have a weight fraction of 10%, a fiber orientation angle of 90°, and a plasma treatment period of 5 min. This combination yielded a strength of 30.351 MPa. The analysis of the interaction between any two factors was done using contour plots. In order to compare the experimental tensile strength values with the anticipated values derived from the regression equation, regression analysis was carried out.Highlights Composites were made up of recycled HDPE (rHDPE) from plastic bottles using a compression molding technique. The Taguchi method is applied to achieve an experimental design employing an L4 orthogonal array. Contour plot analysis is conducted to identify points of minimum and maximum responses, as anticipated from the results. Tensile strength was optimized to a maximum of 30.351 MPa.

Grey wolf optimizer based-natural frequency optimization of laminated composite shells carrying distributed mass

In this study, a grey wolf optimizer is proposed to find the optimum stacking sequence to maximize the fundamental frequency of shells. The vibration analysis of the shells is done using first-order shear deformation theory and a nine-node isoparametric element with five degrees of freedom per node. A mass lumping scheme with rotary inertia is considered in the finite element formulation to include the rotary inertia effect. The design variable considered is the fiber angle orientation of the shells. The present approaches are compared with previously published results using layerwise optimization theory, the Ritz method, and classical lamination theory. A comparison study is also performed, comparing the GWO-based finite element model against six different metaheuristic approaches, and it demonstrates that the Grey Wolf Optimizer consistently outperforms these competing algorithms. The optimum fiber angle orientation of shells carrying distributed mass for various boundary conditions and shell types is analyzed for the first time, to the best of the author’s knowledge. This novel discovery will benefit future studies.

Numerical investigation on orthogonal cutting and damage response of CFRP/Ti6Al4V stacks

CFRP/Ti6Al4V stacks are widely employed in aerospace, automotive and marine applications owing to their superior properties. However, machining these stacked structures pose challenges due to the intrinsic difference in the mechanical properties of CFRP and Ti6Al4V. Such difference can induce distinct failure mechanisms and chip formation processes compared to those observed in individual materials. This paper presents an explicit finite element (FE) modeling to predict the cutting forces and analyze the induced damage during the orthogonal cutting process. The proposed FE model is validated using available experimental data for separate CFRP and Ti6Al4V conditions before being applied to simulate the cutting behavior of CFRP/Ti6Al4V stacks. The effects of fiber angles, cutting sequences and cutting parameters on the cutting performance and damage mechanism of CFRP/Ti6Al4V stacks are investigated in detail. This work provides insights into the cutting behavior of CFRP/Ti6Al4V stacks and facilitates the optimization of machining process for such composite system.

Mechanically enhanced battery separator prepared by hot‐pressing electrospun polyvinylidene fluoride@polymethyl methacrylate membranes with different fiber orientations in adjacent layers

AbstractCompared with commercial polyolefin membranes, electrospun polymeric membranes have the advantages of higher porosity and better electrolyte wettability, but their poor mechanical performance limits their industrial use as battery separators. In this work, a layer‐to‐layer electrospinning is used for fabrication of PVdF@PMMA membranes, in which fibers in adjacent layers are arranged at a certain angle (0°, 30°, 60°, 90°). The as‐electrospun membranes are further hot‐pressed to boost their mechanical strength. Various techniques are employed to evaluate the membranes, such as scanning electron microscopy, differential scanning calorimetry, contact angle measurement, electrochemical impedance spectroscopy, and linear sweep voltammetry. The results show that polymethyl methacrylate partially melts during the hot‐pressing treatment, causing adjacent fibers in the membranes to bridge. The obtained membranes show different tensile strength values with the various angles between fibers. When the angle is 30°, the tensile strength can reach 22.09 MPa and higher porosity (74.68%), greater liquid electrolyte absorption (612.36%) than that of commercial polyolefin membrane are harvested. The lithium‐ion cell assembly with the membrane separator exhibits a discharge capacity reaching 142 mAh g−1 and an excellent capacity retention of 90.7%. This present study provides an innovative and promising approach for the fabrication of high‐performance battery separator by electrospinning.Highlights PVdF@PMMA membranes are prepared by a layer‐to‐layer electrospinning. In the membranes, fiber orientation in adjacent layers is kept at a certain angle. Hot‐pressing further boosts mechanical performance of the membranes. Membranes with different angle of fibers show various mechanical strengths.