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Evidence of the Quantum Optical Nature of High-Harmonic Generation

High-harmonic generation is a light up-conversion process occurring in a strong laser field, leading to coherent bursts of extreme ultrashort broadband radiation [Lewenstein , Phys. Rev. A , 2117 (1994)]. As a new perspective, we propose that ultrafast strong-field electronic or photonic processes such as high-harmonic generation can potentially generate nonclassical states of light well before the decoherence of the system occurs [Gorlach , Nat. Commun. , 4598 (2020); Stammer ., Phys. Rev. Lett. , 123603 (2022)]. This could address fundamental challenges in quantum technology such as scalability, decoherence, or the generation of massively entangled states [Lewenstein , Luca Argenti Michael Chini, 27 (2024)]. Here, we report experimental evidence of the nonclassical nature of the harmonic emission in several semiconductors excited by a femtosecond infrared laser. By investigating single- and double-beam intensity cross-correlation [Loudon, Rep. Prog. Phys. , 913 (1980)], we measure characteristic nonclassical features in the single-photon statistics. We observe two-mode squeezing in the generated harmonic radiation, which depends on the laser intensity that governs the transition from super-Poissonian to Poissonian photon statistics. The measured violation of the Cauchy-Schwarz inequality realizes a direct test of multipartite entanglement in high-harmonic generation [Wasak, Phys. Rev. A , 033616 (2014)]. This result is supported by the theory of multimodal detection and the Hamiltonian from which the effective squeezing modes of the harmonics can be derived [Gonoskov , Phys. Rev. B , 125110 (2024); Christ New J. Phys. , 033027 (2011)]. With this work, we show experimentally that high-harmonic generation is a new quantum bosonic platform that intrinsically produces nonclassical states of light with unique features such as multipartite broadband entanglement or multimode squeezing. The source operates at room temperature, using standard semiconductors and a standard commercial fiber laser, opening up new routes for the quantum industry, such as optical quantum computing, communication, and imaging. Published by the American Physical Society 2024

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Fracture as an Emergent Phenomenon

The mechanics of fracture propagation provides essential knowledge for the risk tolerance design of devices, structures, and vehicles. Techniques of free energy minimization provide guidance, but have limited applicability to material systems evolving away from equilibrium. Experimental evidence shows that the material response depends on driving forces arising from mechanical fields. Recent years have witnessed the development of new methods for modeling complex dynamic and quasistatic fracture. New approaches may differ remarkably from previous ones, as they involve implicit coupling between damaged and undamaged states, allowing fracture to be modeled as emergent phenomena.The focus of this workshop is on the most advanced techniques for modeling fracture, represented by eigenerosion methods, variational approaches, phase field fracture models, and non-local approaches. Technical progress is contingent on the further development of the mathematical framework underlying these techniques. This is necessary for accurate and reliable computational modeling of fracture for multiple freely propagating cracks. The objective of this workshop is to mathematically identify and discuss open issues related to fracture modeling and to highlight recent advances. Addressing fundamental issues will foster exchange between the different communities, essential for advancing the field.

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