Abstract
Taking into account various available experimental data, an improved internally consistent data set for the SiO 2 system is obtained by thermodynamic assessment. The volumetric properties for SiO 2 polymorphs are reassessed using the CALPHAD method. A two-coefficient expression is used to describe the thermal expansion and bulk modulus. For liquid phase, one equation is achieved in the temperature range of 298–4000 K either for thermal expansion or for bulk modulus. Phase diagrams have been calculated up to 40 GPa. It has been concluded that, in the pressure range lower than 20 GPa, there is no significant difference between the phase diagrams calculated by the Birch–Murnaghan equation of state (EOS) and by Murnaghan EOS.
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