Abstract

The strong confinement of light in planar-optical waveguides has been used to measure the two-photon absorption coefficient, β, in 4-butoxycarbonylmethylurethane polydiacetylene (4BCMU) thin films. Prisms were used to couple the 30–60 ps pulses (up to 10 μJ) from a mode-locked YAG laser (λ=1.06 μm) into the thin-film waveguides. A simple analytical theory is compared with the experimental results to give a value of β≊4×10−3 cm/MW.

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