Abstract
The variation-perturbation approach with a time-dependent electric field is used in order to obtain the third-order energy and to find the first hyperpolarizability with the first-order perturbed function. The function used is the same as the one described in a previous paper [M. R\'erat, M. Merawa, and C. Pouchan, Phys. Rev. A 45, 6263 (1992)] relative to dynamic-polarizability calculation from a time-dependent gauge-invariant method. Static-hyperpolarizability components are given for FH and LiH and discussed in comparison with previous calculations. Dynamic components are calculated for the electro-optic Pockels effect up to the first resonances.
Talk to us
Join us for a 30 min session where you can share your feedback and ask us any queries you have
Schedule a callDisclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.
