Abstract

Magneto‐electric (ME) ceramic composites of cobalt ferrite (CoF) and lead zirconate titanate (PZT) were prepared by mechanical mixing of the constituent powders followed by cosintering. The cosintering conditions for nano‐sized CoF and submicrometer‐sized PZT powders were studied in detail. It was found that the CoF powder needs to be presintered at 700°C for 2 h to minimize the differences in the sintering kinetics of the constituent powders. Despite the low cosintering temperatures (900°C–1000°C) the interdiffusion of the cations from both phases was confirmed with energy‐dispersive X‐ray analysis and X‐ray diffraction. Efforts were made to optimize the cosintering conditions to prepare dense ceramic ME composites, which showed the converse ME effect.

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