Abstract
add a new member to the series of mononuclear complexes M(sacacen), M = Ni, Cu, Zn, whose structures were previously reported. The number of d electrons within the series is systematically varied from 7 to 10. The four structures are compared in detail to find the parameters that govern the deformation trends. An extended Huckel MO treatment has been applied to determine the relationships between the geometry and the number of d electrons at the metal. The results are compared with the esr and electrochemical experimental data that have been previously reported for these compounds.
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