Temperature-driven spin reorientation transition in van der Waals Cr1.7Te2 ferromagnet

Abstract

The phenomenon of spin reorientation transition in magnetic materials is truly captivating, as it involves a fascinating change in the direction of magnetic moments. However, the research on spin reorientation transition in two-dimensional (2D) magnetic materials has received limited attention, thus hindering its immense potential for significant advancements in various device applications. In this study, we present a discovery of a spin reorientation transition from an in-plane to an out-of-plane direction in the van der Waals ferromagnet Cr1.7Te2 (Tc = 300 K). This transition occurs at 70 K when the temperature ranges from 3 to 300 K, which is evidenced by the temperature-dependent Hall effect and magnetic anisotropy energy measurements. Notably, the anisotropic evolution observed reveals that the shape anisotropy effect surpasses the magnetocrystalline anisotropy in van der Waals ferromagnet at low temperatures, which is distinct from reported ferromagnetic materials. Furthermore, temperature-dependent x-ray diffraction characterizations confirm that no structural phase transition occurs during this intriguing spin reorientation transition process. These findings establish a strong and solid foundation, offering a promising platform for the design and development of cutting-edge 2D spintronic devices.