Temperature and polarization dependence of low-energy magnetic fluctuations in nearly optimally doped NaFe0.9785Co0.0215As

Abstract

We use unpolarized and polarized neutron scattering to study the temperature and polarization dependence of low-energy magnetic fluctuations in nearly-optimal-doped NaFe$_{0.9785}$Co$_{0.0215}$As, with coexisting superconductivity ($T_{\rm c}\approx19$ K) and weak antiferromagnetic order ($T_{\rm N}\approx30$ K, ordered moment $\approx0.02$ $\mu_{\rm B}$/Fe). A single spin resonance mode with intensity tracking the superconducting order parameter is observed, although energy of the mode only softens slightly on approaching $T_{\rm c}$. Polarized neutron scattering reveals that the single resonance is mostly isotropic in spin space, similar to overdoped NaFe$_{0.935}$Co$_{0.045}$As but different from optimal electron-, hole-, and isovalent-doped BaFe$_2$As$_2$ compounds, all featuring an additional prominent anisotropic component. Spin anisotropy in NaFe$_{0.9785}$Co$_{0.0215}$As is instead present at energies below the resonance, which becomes partially gapped below $T_{\rm c}$, similar to the situation in optimal-doped YBa$_2$Cu$_3$O$_{6.9}$. Our results indicate that anisotropic spin fluctuations in NaFe$_{1-x}$Co$_x$As appear in the form of a resonance in the underdoped regime, become partially gapped below $T_{\rm c}$ near optimal doping and disappear in overdoped compounds.