Target optimization for the photonuclear production of radioisotopes

Abstract

In this paper we discuss the optimum shape of a target for photonuclear production of radioisotopes using an electron linear accelerator. Different target geometries such as right cylinder, conical frustum, Gaussian volume of revolution and semi-ellipsoid have been considered for the production of 67Cu via 68Zn(γ,p)67Cu photonuclear reaction. The specific activity (SA) of 67Cu was simulated for each target shape. Optimum ratio of radius to height for cylindrical targets was found to be between 0.2 and 0.25 for target masses ranging from 20g to 100g. It was shown that while some unconventional target shapes, such as semi-elliptical volume of revolution, result in slightly higher specific activities than cylindrical targets, the advantage is not significant and is outweighed by the complexity of the target production and handling. Power deposition into the target was modeled and the trade-off between the maximization of 67Cu yield and the minimization of target heating has been discussed. The 67Cu case can easily be extended for production of many other isotopes.