Abstract

In this work, tension and fracture behaviors of cellulose nanopaper (CNP) made from two different preparation approaches are comparatively studied. The CNP are prepared by casting (or C-CNP) and filtration (or F-CNP) of CNF suspension. The resulting CNP are mechanically characterized using the vision-based full-field optical method of Digital Image Correlation. Tension tests show that F-CNP has a higher strength and greater nonlinearity than the C-CNP. The crack initiation and growth characteristics of the two types of CNP are investigated using optical measurements. The data are analyzed under small-scale-yielding conditions to quantify the fracture parameters such as stress intensity factors and energy release rates at crack initiation as well as during crack growth. The results indicate that both C-CNP and F-CNP show significant crack growth resistance in the post-crack initiation regime. The F-CNP particularly offers substantial resistance to crack growth relative to the C-CNP demonstrating that filtration is the preferred method to make CNP with higher tensile strength and better fracture properties.

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