Abstract
Abstract A method for studying dissociation of diatomic molecules by isotope spectroscopy is presented both theoretically and practically. A theory based on combinatorial analysis is presented for molecules of the form B 2 and BC. Molecular dissociation rates can be calculated from measurements of isotope exchange provided the isotopes in the molecules can be considered as chemically equivalent. Dissociation measurements of O 2 on Pt, RuO 2 , Ir and Ni–Zr–Sm as well as CO on Pt and Al are presented in the temperature range 400–900 °C.
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