Abstract
Neutron diffraction measurements have been performed on highly concentrated LiCI solutions in D 2O over a wide temperature range covering their glassy and supercooled states and the supercritical temperature of water. The 6Li/ 7Li and 35Cl/ 37Cl isotopic substitution method was used to derive the Li- and Cl-related radial distribution functions. Both neutron data sets have revealed temperature-dependent microscopic structures of ionic hydration in terms of ion-water distances, hydration number, orientation of coordinated water molecules, and hydrogen bonding.
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