Abstract
The Raman spectrum of K 3InCl 6, H 2O single crystal is assigned on the basis of the crystal structure knowledge. The main feature is the splitting of the ν 1 vibrational band into two components, that are assigned in relation to the indium site occupation ratio. In Raman spectroscopy, the superposition of the internal mode frequency range (characteristic of different anionic species), does not contribute to any improvement of the ionic isomerisation found by X-ray investigation.
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