Abstract
Criteria of interstitial hole size and H-H interatomic distance were used to predict the stoichiometries and the hydrogen-occupied sites in hydrides of the intermetallic compound ZrNi and other isostructural compounds. With only these simple considerations of geometry it was possible to rationalize most of the experimental observations available for such compounds. A number of neutron diffraction experiments are recommended to test some of the predictions presented.
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