Abstract
We theoretically investigate the behavior of coherent optical phonons in an electron–phonon coupled system at moderate laser intensity: below GW/cm2. We calculate the coherent phonons from impulsive stimulated Raman scattering (ISRS) and impulsive absorption (IA) mechanisms with a nonperturbative model. The generation efficiency of coherent phonons in single-pulse excitation exhibits gradual nonlinear saturation with increasing optical intensity in a nonperturbative regime. The ISRS mechanism exhibits substantial saturation at relatively low pulse intensity, whereas the IA mechanism remains roughly linear. We further examine the influence of double-pulse excitation on quantum path interference. The ISRS mechanism exhibits a pronounced saturation effect near 0 fs of pump–pump delay, whereas the IA process exhibits negligible saturation behavior. These results reproduce well experimental data obtained by double-pulse excitation and support our proposal that ISRS is the primary quantum path for the observed coherent phonons in gallium arsenide.
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