Abstract
Two manganese phosphate-oxalates, namely, H2aep·Mn2(H2PO4)2(C2O4)2·H2O (1) and H2epip·Mn2(H2PO4)2(C2O4)2 (2), were prepared under solvent-free conditions, where aep=1-(2-aminoethyl)piperazine and epip=1-ethylpiperzaine. The two hybrid solids have three-dimensional open-framework structures with 12-, and 16-ring channels, respectively. Topological analysis reveals that they have 4-connected lon and mog nets. The magnetic properties of the two compounds were also investigated.
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