Abstract

The optical detection technique is used to observe magnetic resonance in the triplet state 3 B 1 u of the self-trapped exciton in LiF, NaF, KF. The strong anisotropy of the hyperfine interaction in the x− y plane is related to the more localized character of the electronic wavefunction. The magnetic dipolar contribution to the fine structure can be described by a Mollwo-Ivey type law in alkali fluorides and chlorides.

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