Abstract
The interest in belite (Ca2SiO4 + impurities or dopants) phase increases significantly since new types of clinkers based essentially on this phase become promising alternatives to Portland clinker for reducing CO2 emission. Belite is also of interest as a biomedical cement. For the cement industry, stabilization of the β-polymorph is essential since the γ-polymorph has no hydraulic activity. In order to understand the mechanism of β-polymorph stabilization, this paper explores the addition of three dopants, namely P, B and S. It turns out that these dopants can modify the lattice parameters of Ca2SiO4 and induce specific twinning morphologies and surface relief, as well as grain boundaries deformations. A link between the addition of dopant leading to significant microstructural changes and the stabilization of β-polymorph has been established.
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