Roads towards fault-tolerant universal quantum computation.

Quantum gates are essential for the realization of quantum computer and have been implemented in various types of two-level systems. However, high-dimensional quantum gates are rarely investigated both theoretically and experimentally even that high-dimensional quantum systems exhibit remarkable advantages over two-level systems for some quantum information and quantum computing tasks. Here we experimentally demonstrate the four-dimensional X gate and its unique higher orders with the average conversion efficiency 93%. All these gates are based on orbital-angular-momentum degree of freedom (DoF) of single photons. Besides, a set of controlled quantum gates is implemented by use of polarization DoF. Our work is an important step toward the goal of achieving arbitrary high-dimensional quantum circuit and paves a way for the implementation of high-dimensional quantum communication and computation.

Quantum information science has extensive applications in various research fields, such as information, physics and computer science. It is well known that the quantum properties of a system exhibit many unique advantages in the security of information transmission and processing, computation, and the improvement of channel capacity. Quantum information includes several research fields, for example, quantum communication, quantum computing and so on. In the past 30 years, the development of quantum communication, quantum computing and quantum information processing has made great progress in both theory and experiments. As a fundamental resource for quantum information processing, entanglement is a key element for many applications, such as quantum key distribution, quantum teleportation, quantum dense coding, quantum secure direct communication and quantum metrology. Because of the weak interaction with the environment and the degrees of freedom, entangled photons are the excellent candidates as the quantum-information carrier. Several remarkable experiments have been performed with the photonic entanglement. However, it is necessary to share a pair of entangled photons between the communicating parties in advance in these quantum information processes. Furthermore, the application of hyperentanglement, the entanglement of photon pairs simultaneously existing in more than one degree of freedom, has been widely studied for the reason that it can improve the channel capacity of quantum communications and implement hyperparallel computing, such as the quantum error-correcting code, quantum repeater and deterministic entanglement purification. Moreover, the quantum logic gates play an essential role in quantum information processing which attracts much attention on the designing of the quantum logic gates. Depending on the coherent dynamics of the cavity quantum electrodynamical system, deterministic quantum gate operations between the quantum systems can be realized. Here in this review, by considering high-dimensional quantum systems, several high-dimensional quantum protocols are presented. They can greatly improve the capacity of quantum channel and noise immunity, which exhibits potential applications in quantum information processing. This review describes the development of quantum computing and quantum information processing using hyperentanglement. And the entangled photons in single degree of freedom and multi-degrees of freedom are used to illustrate the two-dimensional and high-dimensional quantum information processing schemes. Finally, the latest progress and further applications of quantum computing and quantum information processing are introduced.

Quantum light sources are one of key devices for quantum information processing, and they are also the important foundation for applications such as in quantum computing, quantum communication, and quantum simulation. Improving the capacity of quantum information coding by using the quantum light source is a major challenge in the development of quantum information technology. Photons with a helical phase front can carry a discrete, unlimited but quantized amount of orbital angular momentum (OAM). The infinite number of states with different OAMs can greatly increase the capacity of optical communication and information processing in quantum regimes. To date photons carrying OAM have mainly been generated by using bulk crystals, which limits the efficiency and the scalability of the source. With the advancement of quantum photonic technology, many significant quantum photonic devices can now be realized on integrated chips. However, creating high-dimensional OAM quantum states at a micro-nano scale is still a challenge. And the research of harnessing high-dimensional OAM mode by using integrated quantum photonic technologies is still in its infancy. Here, the authors review the recent progress and discuss the integrated quantum light sources with OAM. The authors introduce the research progress of using OAM for both single photons and entangled photons and emphasize the exciting work on pushing boundaries in high-dimensional quantum states. This may pave the way for the research and practical applications of high-dimensional quantum light sources.

The spatial modes of light, carrying a quantized amount of orbital angular momentum (OAM), is one of the excellent candidates that provides access to high-dimensional quantum states, which essentially makes it promising towards building high-dimensional quantum networks. Quantum memory with efficiency above 50% is an essential condition for beating the no-cloning limit or in the one-way quantum computation. However, up till now, the highest storage efficiencies achieved for OAM states are below 30%, which is an obstacle towards practical applications. In this paper, we report the storage and retrieval of photonic qubits encoded with OAM state in an elongated cold rubidium atomic ensemble, achieving a storage efficiency around 65% with an average conditional fidelity above 98%. Our work constitutes an efficient node that is needed towards high dimensional and large scale quantum networks.

The high-dimensional quantum system greatly improve the quantum channel capacity and information storage space, and achieve high-dimensional quantum information transmission, which enhance the speed of quantum computing and quantum information processing. In this paper, a high-dimensional quantum teleportation protocol without information loss is proposed. We consider pre-sharing a high-dimensional non-maximum entangled state as a quantum channel between sender and receiver. By adding auxiliary particle and performing high-dimensional local operations, it is possible to achieve high-dimensional quantum teleportation without information loss. Simultaneously, we apply the protocol to butterfly network, and propose a novel high-dimensional quantum network coding based on prediction mechanism. In our scheme, we use Z-{|0⟩, |1⟩} basis to predict the transmission of high dimensional states over the butterfly network. When the prediction is successful, the deterministic transmission of high-dimensional quantum states can be realized over the butterfly network. Our scheme greatly saves the usage of quantum and classical channels, which improves the utilization efficiency of both channels.

Connecting multiple smaller qubit modules by generating high-fidelity entanglement is a promising path for scaling quantum computing hardware. The performance of such a modular quantum computer depends on the quality and rate of entanglement generation. However, identifying optimal architectures and entanglement generation protocols remains an open question. How can modular quantum architectures be designed to achieve fault tolerance while requiring only feasible entanglement rates and hardware? Focusing on solid-state quantum hardware, we investigate the threshold and logical failure rate of a fully distributed surface code. We consider both emission-based and scattering-based entanglement schemes between the modules to link the performance to the physical hardware and identify the regime for fault tolerance. We compare architectures with one or two data qubits per module. For some entanglement schemes, thresholds nearing the thresholds of non-distributed implementations (~ 0.4%) appear feasible with future parameters minimizing the performance gap between modular and monolithic quantum processors.

Quantum error correction and fault-tolerance have provided the possibility for large scale quantum computations without a detrimental loss of quantum information. A very natural class of gates for fault-tolerant quantum computation is the Clifford gate set and as such their usefulness for universal quantum computation is of great interest. Clifford group gates augmented by magic state preparation give the possibility of simulating universal quantum computation. However, experimentally one cannot expect to perfectly prepare magic states. Nonetheless, it has been shown that by repeatedly applying operations from the Clifford group and measurements in the Pauli basis, the fidelity of noisy prepared magic states can be increased arbitrarily close to a pure magic state~\cite{Bravyi}. We investigate the robustness of magic state distillation to perturbations of the initial states to arbitrary locations in the Bloch sphere due to noise. Additionally, we consider a depolarizing noise model on the quantum gates in the decoding section of the distillation protocol and demonstrate its effect on the convergence rate and threshold value. Finally, we establish that faulty magic state distillation is more efficient than fault-tolerance-assisted magic state distillation at low error rates due to the large overhead in the number of quantum gates and qubits required in a fault-tolerance architecture. The ability to perform magic state distillation with noisy gates leads us to conclude that this could be a realistic scheme for future small-scale quantum computing devices as fault-tolerance need only be used in the final steps of the protocol.

Abstract: This research volume offers a comprehensive and academically rigorous examination of the intersection between high-dimensional artificial intelligence (AI) and quantum computing, with a focus on their combined potential to transform scientific discovery, genomic analysis, and economic modeling. The book constructs an integrated conceptual and computational framework that synthesizes tensor-based AI architectures with quantum state formalism, enabling scalable solutions to complex, multi-dimensional problems that are intractable with classical methods alone. The study begins by analyzing the theoretical underpinnings of high-dimensional data spaces, manifold learning, and quantum mechanical principles such as superposition and entanglement. From this foundation, the volume explores hybrid quantum-AI methodologies applied to dynamic systems modeling in the sciences, precision diagnostics in genomics, and macroeconomic forecasting. Methodologically, the work employs a combination of variational quantum algorithms, quantum kernel methods, and tensor factorization, supported by simulations, real-world datasets, and benchmarking. Key results highlight improvements in model efficiency, predictive accuracy, and scalability across all domains explored. In genomics, quantum-AI models enable multi-omic integration and improved variant detection; in economics, they provide enhanced risk modeling and policy simulation. The implications extend to both theory and application, offering pathways for advancing scientific inquiry, personalizing medicine, and shaping resilient economic systems. The book concludes with a critical assessment of ethical, epistemological, and governance considerations, ensuring responsible and equitable development of quantum-AI technologies. Keywords High-dimensional AI, quantum computing, quantum machine learning, tensor factorization, quantum kernel methods, genomic intelligence, economic forecasting, hybrid quantum-classical systems, quantum reinforcement learning, multi-omic data integration, macroeconomic modeling, quantum algorithms, data scalability, scientific simulation, epistemological implications, algorithmic ethics, responsible AI, quantum explainability, federated quantum learning, quantum cloud infrastructure.

Although qubits are the leading candidate for the basic elements in a quantum computer, there are also a range of reasons to consider using higher dimensional qudits or quantum continuous variables (QCVs). In this paper we use a general `quantum variable' formalism to propose a method of quantum computation in which ancillas are used to mediate gates on a well-isolated `quantum memory' register and which may be applied to the setting of qubits, qudits (for $d>2$) or QCVs. More specifically, we present a model in which universal quantum computation may be implemented on a register using only: repeated applications of a single fixed two-body ancilla-register interaction gate, ancillas prepared in a single state, and local measurements of these ancillas. In order to maintain determinism in the computation, adaptive measurements via a classical-feedforward of measurement outcomes are used, with the method similar to that in measurement-based quantum computation (MBQC). We show that our model has the same hybrid quantum-classical processing advantages as MBQC, including the power to implement any Clifford circuit in essentially one layer of quantum computation. In some physical settings, high-quality measurements of the ancillas may be highly challenging or not possible, and hence we also present a globally unitary model which replaces the need for measurements of the ancillas with the requirement for ancillas to be prepared in states from a fixed orthonormal basis. Finally, we discuss settings in which these models may be of practical interest.

High-dimensional entanglement with larger Hilbert spaces enable an encoding of more bits per photon and thus promise increased communication capacities over quantum channels. Quantum frequency combs, which are intrinsically multimode in the temporal and frequency degrees of freedom within a single spatial mode, naturally facilitating the generation and measurement of high-dimensional entanglement. Current challenges include the extension of well-known methods for two qubits to high-dimensional quantum systems and their application in entanglement experiments with photons. More specifically, the major challenge is the certification of high-dimensional entanglement by a number of accessible experimental measurements. In this paper, we increase the Hilbert space dimensionality and provide versatile tools for quantifying and certifying high-dimensional entanglement in a biphoton frequency comb. We quantify the time binned Schmidt number up to 18 and certify entanglement of formation with 1.89 ebits. We have demonstrated a 648- dimensional Hilbert spaces with time-frequency entanglement in a biphoton frequency comb, enabling a computational space up to 13 photonic qubits, and 6.28 bits/photon classical information capacity. This high-dimensional time frequency multimode quantum states of biphoton frequency comb significantly boosting the photon information capacity that is critical for large-scale quantum information processing. Biphoton frequency comb has indeed demonstrated an attractive and powerful approach towards achieving this fundamental goal with applications in high-dimensional quantum information processing, time-frequency cluster-state quantum computation, high-dimensional encoding in quantum networks, and high-dimensional quantum simulations.

Realizing universal fault-tolerant quantum computation is a key goal in quantum information science1-4. By encoding quantum information into logical qubits using quantum error correcting codes, physical errors can be detected and corrected, enabling a substantial reduction in logical error rates5-11. However, the set of logical operations that can be easily implemented on these encoded qubits is often constrained1,12, necessitating the use of special resource states known as 'magic states'13 to implement universal, classically hard circuits14. A key method to prepare high-fidelity magic states is to perform 'distillation', creating them from multiple lower-fidelity inputs13,15. Here we present the experimental realization of magic state distillation with logical qubits on a neutral-atom quantum computer. Our approach uses a dynamically reconfigurable architecture8,16 to encode and perform quantum operations on many logical qubits in parallel. We demonstrate the distillation of magic states encoded in d = 3 and d = 5 colour codes, observing improvements in the logical fidelity of the output magic states compared with the input logical magic states. These experiments demonstrate a key building block of universal fault-tolerant quantum computation and represent an important step towards large-scale logical quantum processors.

Stable quantum information in topological systems

Recent improvements in control of quantum systems make it seem feasible to finally build a quantum computer within a decade. While it has been shown that such a quantum computer can in principle solve certain small electronic structure problems and idealized model Hamiltonians, the highly relevant problem of directly solving a complex correlated material appears to require a prohibitive amount of resources. Here, we show that by using a hybrid quantum-classical algorithm that incorporates the power of a small quantum computer into a framework of classical embedding algorithms, the electronic structure of complex correlated materials can be efficiently tackled using a quantum computer. In our approach, the quantum computer solves a small effective quantum impurity problem that is self-consistently determined via a feedback loop between the quantum and classical computation. Use of a quantum computer enables much larger and more accurate simulations than with any known classical algorithm, and will allow many open questions in quantum materials to be resolved once a small quantum computer with around one hundred logical qubits becomes available.

Quantum entanglement is essential for the realization of distributed computing and has been implemented in various types of two-level systems. However, high-dimensional quantum protocols are rarely investigated both theoretically and experimentally, despite the remarkable advantages that high-dimensional quantum systems exhibit over two-level systems for certain quantum information and computing tasks. Here, we propose asymmetric protocols that utilize different dimensional systems to prepare the stator and achieve remote state operations with the assistance of shared N-partite graph states. Our protocols demonstrate convincing control power and security, with all implementations achievable through local operations and classical communications. The experimental realization of high-dimensional quantum systems and operations is presented using current technology. Our work contributes towards achieving arbitrary high-dimensional quantum protocols and paves the way for implementing high-dimensional quantum communication and computation.

Hyperentanglement, as a high-dimensional quantum entanglement phenomenon with multiple degrees of freedom, plays a critical role in quantum communication, quantum computing, and high-dimensional quantum state manipulation. Unlike entangled states in a single degree of freedom, hyperentangled states establish entanglement relationships simultaneously in multiple degrees of freedom, such as polarization, path, and orbital angular momentum. Through entanglement-based distribution techniques, high-dimensional quantum information networks can be constructed. On this basis, a fully connected quantum network with hyperentanglement is constructed in this work, and the polarization and time-bin degree-of-freedom hyperentanglement is realized through the process of second-harmonic generation and spontaneous parametric down-conversion in periodically poled lithium niobate (PPLN) waveguide cascades. The hyperentangled state is then multiplexed into a single-mode fiber by using dense wavelength division multiplexing (DWDM) technology for transmission to terminal users. The quality of the entangled states in the two degrees of freedom is characterized using Franson-type interference and photon-pair coincidence measurement techniques. Polarization entangled states are subjected to quantum state tomography, and entanglement distribution technology is employed to achieve long-distance distribution and quantum key transmission within the network. Experimental results show that the two-photon interference visibility of both polarization and time-bin entanglement is greater than 95%, demonstrating the high quality of the hyperentanglement in the network. After 100-km-entanglement distribution, the fidelity of the quantum states in both degrees of freedom remains above 88%, indicating the effectiveness of long-distance entanglement distribution in this network. Additionally, it is verified that this network supports the distribution of quantum keys over a distance of more than 50 km between users. These results confirm the feasibility of a fully connected quantum network with hyperentanglement and demonstrate the potential for constructing large-scale metropolitan networks by using hyperentanglement. As a higher-dimensional entanglement, hyperentangled states can significantly enhance the capacity and efficiency of quantum information processing. Although the quantum communication is still in its early stages of development, achieving stable storage and transmission of entangled states in large-scale metropolitan networks remains a great challenge. By utilizing the frequency conversion properties and high integration characteristics of the periodically poled lithium niobate waveguides, the three-user hyperentangled quantum network constructed in this work provides a new solution for developing the large-scale metropolitan networks with high-dimensional quantum information networks. It is expected to provide a new platform for quantum tasks such as superdense coding and quantum teleportation.