Abstract

We have investigated magnetic interactions between transition metal ions in bismuthene topological insulators with protected edge states. We find that these topological states have a crucial role in the magnetic interactions in 2D topological insulators. Using first-principles and model Hamiltonian, we make a comparative study of transition metal doped bulk and nanoribbon bismuthene. While a direct overlap between the transition metal prevails in gapped bulk bismuthene, at the borders of nanoribbons, a long-range magnetism is present. The exchange interactions are well described by a Ruderman–Kittel–Kasuya–Yosida-like Hamiltonian mediated by massive and topological states. Our results show a dominance of antiferromagnetism promoted by the topological states, preserving the spin-locked Dirac crossing states due to a global time-reversal symmetry preservation. This extended magnetic interactions mediated mainly by massless electrons can increase the spin diffusion length being promising for fast dissipationless spintronic devices.

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