Abstract

Abstract. Although much effort has been put into studying air pollution, our knowledge of the mechanisms of frequently occurring intense haze episodes in China is still limited. In this study, using 3 years of measurements of air pollutants at three different height levels on a 325 m Beijing meteorology tower, we found that a positive aerosol–boundary layer feedback mechanism existed at three vertical observation heights during intense haze polluted periods within the mixing layer. This feedback was characterized by a higher loading of PM2.5 with a shallower mixing layer. Modelling results indicated that the presence of PM2.5 within the boundary layer led to reduced surface temperature, relative humidity and mixing layer height during an intensive haze episode. Measurements showed that the aerosol–boundary layer feedback was related to the decrease in solar radiation, turbulent kinetic energy and thereby suppression of the mixing layer. The feedback mechanism can explain the rapid formation of intense haze episodes to some extent, and we suggest that the detailed feedback mechanism warrants further investigation from both model simulations and field observations.

Highlights

  • With the rapid economic growth and urbanization, an increasing frequency of haze episodes along with the air pollution has become of great concern in China during the last decade

  • In this study, using 3 years of measurements of air pollutants at three different height levels on a 325 m Beijing meteorology tower, we found that a positive aerosol–boundary layer feedback mechanism existed at three vertical observation heights during intense haze polluted periods within the mixing layer

  • The development of a mixing layer height in an urban city is affected by the intensity of incoming solar radiation

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Summary

Introduction

With the rapid economic growth and urbanization, an increasing frequency of haze episodes along with the air pollution has become of great concern in China during the last decade During December 2016 a series of intense haze episodes took place in eastern China, characterized by surface PM2.5 concentrations exceeding 500 μg m−3 in several measurement sites in Beijing and its surrounding sites (http://www.mep.gov.cn/gkml/hbb/ qt/201701/t20170102_393745.htm, last access: 11 December 2019). A recent study reported that the particulate matter has significantly decreased the life span of residents by as many as 5.5 years in northern China (Chen et al, 2013). The air pollution was estimated to cause over 3 million premature deaths every year (Lelieveld et al, 2015)

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