Abstract
Abstract Lithium–sulfur (Li–S) batteries are great candidates for energy storage systems, but need to overcome the issues of low sulfur utilization and polysulfide shuttling for use in large-scale commercial applications. Recently, quaternized polymers have received much attention for their polysulfide trapping properties due to electrostatic interaction. In this work, we report a series of polyarylether sulfone (PSF) binders with different cation structures including imidazolium (Im), triethylammonium (Tr), and morpholinium (Mo). The ability of the these quaternized binders and the conventional poly(vinylidene fluoride) or PVDF binder to capture polysulfide increases in the order of PVDF
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