Abstract

Measurements are presented of the proton relaxation time in Cu x Zn 1− x Cs 2(SO 4) 26H 2O at liquid-helium temperatures. The results are explained by a thermodynamic model which distinguishes various electron Zeeman systems, and a dipolar interaction system strongly coupled to the proton spin system. The theory gives a quantitatively satisfactory explanation of the complicated behaviour of the proton spin relaxation time as a function of magnetic field and temperature.

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