Abstract
Syn and anti conformational isomers of 3-furylchlorocarbene were characterized in low-temperature matrixes by IR, UV/vis, chemical trapping, and calculational modeling. Displaying significantly different electronic spectra, the two isomeric carbenes could be photochemically interconverted. At shorter wavelengths, the carbene rearranges to a conjugated methylenecyclopropene.
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