Abstract

In this paper, we study the influence of time-dependent phase delay on the emission of few photons from a single molecule in a solid matrix. The results demonstrate that a time-dependent phase of the pulses can be used to control the photon emission and strongly affects the spectrum of single molecules. The spectrum of the photon emission probabilities reflects the fast dynamics of the states of the system when the duration of the driven laser pulses is short. Also, it is shown that the coupling between the system and the rf field strongly affects the spectrum of the photon emission probabilities in space.

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