Abstract

Quantum spins of mesoscopic size are a well-studied playground for engineering non-classical states. If the spin represents the collective state of an ensemble of qubits, its non-classical behavior is linked to entanglement between the qubits. In this work, we report on an experimental study of entanglement in dysprosium's electronic spin. Its ground state, of angular momentum $J=8$, can formally be viewed as a set of $2J$ qubits symmetric upon exchange. To access entanglement properties, we partition the spin by optically coupling it to an excited state $J'=J-1$, which removes a pair of qubits in a state defined by the light polarization. Starting with the well-known W and squeezed states, we extract the concurrence of qubit pairs, which quantifies their non-classical character. We also directly demonstrate entanglement between the 14- and 2-qubit subsystems via an increase in entropy upon partition. In a complementary set of experiments, we probe decoherence of a state prepared in the excited level $J'=J+1$ and interpret spontaneous emission as a loss of a qubit pair in a random state. This allows us to contrast the robustness of pairwise entanglement of the W state with the fragility of the coherence involved in a Schr\"odinger cat state. Our findings open up the possibility to engineer novel types of entangled atomic ensembles, in which entanglement occurs within each atom's electronic spin as well as between different atoms.

Highlights

  • Entanglement is a hallmark of nonclassical behavior in compound quantum systems

  • The virtual absorption of a photon is interpreted as the annihilation of a qubit pair in a state defined by the light polarization, leaving a set of 14 qubits in the excited electronic level [see Fig. 1(a)]

  • As shown in Ref. [48], the existence of a strictly negative value Z (n) constitutes a necessary and sufficient criterion of nonclassicality. To apply this criterion to our system, we use the connection between the mean values of spin projection and the Husimi function of qubit pairs extracted from the electronic spin J, Ln = Qpair(n) − Qpair(−n), Ln2 = Qpair(n) + Qpair(−n), leading to the expression Z (n) = α Cn, where we introduce the coefficient α = ( Qpair(−n) − Qpair(n))2 − 1 and the distribution

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Summary

INTRODUCTION

Entanglement is a hallmark of nonclassical behavior in compound quantum systems. Minimal entangled systems of qubit pairs, as realized with correlated photon pairs, play a central role in testing the foundations of quantum mechanics [1,2]. We study quantum entanglement between subsystems of the electronic spin of dysprosium atoms, of angular momentum J = 8 in its ground state and prepared in nonclassical spin states. The virtual absorption of a photon is interpreted as the annihilation of a qubit pair in a state defined by the light polarization, leaving a set of 14 qubits in the excited electronic level [see Fig. 1(a)]. This process realizes a partition of the electronic spin J in two subsystems—the excited electronic spin J = J − 1 and the photon angular momentum L = 1. Such systems would combine entanglement between atoms and within each electronic spin, allowing one to scale up entanglement depth and its application to quantumenhanced sensing

Probing pairs via light coupling
Application to Dicke states
Coherent and W states
Measure of nonclassicality via the concurrence
Pairwise correlations in a squeezed state
PROBING ENTANGLEMENT VIA THE SUBSYSTEM ENTROPY
Entanglement of the W state
Entanglement of a Schrödinger cat state
DECOHERENCE UPON QUBIT LOSS
Robustness of pairwise quantum correlations
Fragility of macroscopic coherence
Findings
SUMMARY AND OUTLOOK
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