Abstract

We propose a versatile scheme to slow supersonically cooled molecules using a decelerating potential well, obtained by steering a focusing laser beam onto a pair of spinning reflective mirrors under a high-speed brake. The longitudinal motion of molecules in the moving red-detuned light field is analyzed and their corresponding phase-space stability is investigated. Trajectories of $\mathrm{C}{\mathrm{H}}_{4}$ molecules under the influence of the potential well are simulated using the Monte Carlo method. For instance, with a laser beam of power 20 kW focused onto a spot of waist radius 40--100 \ensuremath{\mu}m, corresponding to a peak laser intensity on the order of $\ensuremath{\sim}{10}^{8}\phantom{\rule{0.16em}{0ex}}\mathrm{W}/\mathrm{c}{\mathrm{m}}^{2}$, a $\mathrm{C}{\mathrm{H}}_{4}$ molecule of $\ensuremath{\sim}250\phantom{\rule{0.16em}{0ex}}\mathrm{m}/\mathrm{s}$ can be decelerated to $\ensuremath{\sim}10\phantom{\rule{0.16em}{0ex}}\mathrm{m}/\mathrm{s}$ over a distance of a few centimeters on a time scale of hundreds of microseconds.

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