Optical generation and detection of GHz longitudinal and transverse acoustic waves in solids assisted by two-dimensional metallic grating structure

Abstract

Absorption of laser pulses with picosecond temporal width in a two-dimensional nano-scale metallic grating deposited on a transparent substrate launches both longitudinal and transverse acoustic waves in to the sample. The periodic metallic structure makes the generated acoustic waves propagate several different directions. The propagating acoustic waves are monitored optically by the delayed light pulses (probe light) as the transient reflectivity change which is known as the Brillouin oscillation. The probe light is also diffracted by the metallic grating, allowing the detection of the acoustic waves propagating in the multiple directions efficiently. The analysis of the Brillouin oscillation frequencies brings the longitudinal and transverse sound velocities and the optical refractive index simultaneously from a single measurement. We verify the above mentioned scheme using a sample with two-dimensional square lattice (period 380 nm) of aluminum square islands of lateral dimension 200 × 200 nm2 and thickness of 50 nm on a fused silica substrate of thickness 1 mm. From the obtained Brillouin oscillation frequencies in several tens GHz, the acoustic and optical properties of the substrate material are successfully retrieved. The technique would be applicable to investigate the acoustic and optical properties of more complicated systems, such as anisotropic and/or inhomogeneous medium.