Abstract
A coralloid 3D g-C3N4 supported VO2 catalyst was successfully synthesized in-situ by one-pot method, avoiding the agglomeration of VO2 during the reaction. The morphological and compositional information of the supported catalyst were investigated detailedly. 30% VO2/3D g-C3N4 revealed excellent catalytic activity in aerobic oxidative desulfurization, the oxidative of DBT, 4-MDBT and 4,6-DMDBT reached 98.6%, 99% and 99.4%, respectively, under the same mild conditions. The recycling performance and the mechanism on the oxidative of DBT were studied as well.
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