Abstract
Sequential and iterative asymmetric reaction on achiral substrates with two prochiral centers caused an enantiomeric enhancement and its synthetic application to C2 symmetric azacycloalkanes and 2, 6 disubstituted piperidines is described. Repeated asymmetric dihydroxylation (AD) for terminal olefins also improved stereoselectivity (ee) and a number of syntheses of alkaloids are demonstrated.
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